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Emergent mechanical properties in highly filled additively manufactured polymer composites

  • Additive Manufacturing of Functional and Smart Composites Research Letter
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Abstract

In this work, we investigate additively manufactured composites with populations of coarse and fine glass microspheres that are functionalized using silane coupling agents to explore how and why different functionalization of the fine and coarse fractions leads to vastly different mechanics. Combining strong interfaces on fine particles with weak interfaces on coarse particles leads to enhancements in elongation to break and toughness, whereas combining two types of strong interfaces leads to enhancement in elongation to break and reduction or maintenance of other measured tensile properties. These results can inform future work in tailoring mechanics of highly filled additively manufactured composites.

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Data not included already in the manuscript and supporting information will be made available upon reasonable request to the corresponding author.

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Acknowledgments

This research was sponsored by DEVCOM Army Research Laboratory and was accomplished under Cooperative Agreement Number W911NF-19-2-0100. The views and conclusions contained in this document are those of the authors and should not be interpreted as representing the official policies, either expressed or implied, of DEVCOM ARL or the U.S. Government. The U.S. Government is authorized to reproduce and distribute reprints for Government purposes notwithstanding any copyright notation herein. The team is grateful to Mr. John Vericella and Autodesk for the donation of the Ember printers used in this work.

Funding

This research was sponsored by DEVCOM Army Research Laboratory and was accomplished under Cooperative Agreement Number W911NF-19–2-0100.

Author information

Authors and Affiliations

  1. Department of Plastics Engineering, University of Massachusetts Lowell, 1 University Ave, Lowell, MA, 01854, USA

    Tahamina Nasrin, Ahmed O. Adisa & Amy M. Peterson

  2. Department of Mechanical & Industrial Engineering, University of Massachusetts Lowell, 1 University Ave, Lowell, MA, 01854, USA

    Christopher J. Hansen

  3. Department of Mathematical and Statistical Sciences, University of Colorado Denver, 1201 Larimer St, Denver, CO, 80204, USA

    Farhad Pourkamali-Anaraki

  4. DEVCOM Army Research Laboratory, Aberdeen Proving Ground, Adelphi, MD, 21005, USA

    Robert E. Jensen

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  1. Tahamina Nasrin
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  2. Ahmed O. Adisa
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Contributions

Tahamina Nasrin: conceptualization, data curation, formal analysis, investigation, methodology, writing – original draft preparation; Ahmed Adisa: investigation, methodology, writing—review & editing; Christopher Hansen: conceptualization, funding acquisition, resources, writing – review & editing; Farhad Pourkamali-Anaraki: conceptualization, funding acquisition, writing – review & editing; Robert Jensen: conceptualization, writing – review & editing; Amy Peterson: conceptualization, methodology, project administration, resources, supervision, writing – original draft preparation.

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Correspondence to Amy M. Peterson.

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Nasrin, T., Adisa, A.O., Hansen, C.J. et al. Emergent mechanical properties in highly filled additively manufactured polymer composites. MRS Communications (2024). https://doi.org/10.1557/s43579-024-00530-x

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  • DOI: https://doi.org/10.1557/s43579-024-00530-x

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