Skip to main content
Log in

Multilevel memory and synaptic characteristics of a-IGZO thin-film transistor with atomic layer–deposited Al2O3/ZnO/Al2O3 stack layers

  • Invited Feature Paper
  • Published:
Journal of Materials Research Aims and scope Submit manuscript

Abstract

A multilevel nonvolatile memory based on an amorphous indium–gallium–zinc oxide thin-film transistor is successfully demonstrated by using an atomic layer–deposited ZnO film as a charge trapping layer. The memory device shows a much higher erasing efficiency at a negative bias, i.e., after erasing at −13 V for 1 µs, the threshold voltage shift is as large as −7.4 V. In the case of 13 V/1 µs programming (P) and −12 V/1 µs erasing (E), the device demonstrates an ON/OFF readout drain current (IDS) ratio of 103 after 105 s, and a large and stable ON/OFF IDS ratio of 106 till 104 of P/E cycles. Furthermore, multilevel memory characteristics are also demonstrated on the device, showing an IDS ratio of >102 for 4 different states. Additionally, the device also successfully demonstrates typical synaptic behaviors, such as excitatory and inhibitory postsynaptic current with different memory times at different memory states.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Figure 1
Figure 2
Figure 3
Figure 4
Figure 5
Figure 6

Similar content being viewed by others

References

  1. T. Iwasaki, N. Itagaki, T. Den, H. Kumomi, K. Nomura, T. Kamiya, and H. Hosono: Combinatorial approach to thin-film transistors using multicomponent semiconductor channels: An application to amorphous oxide semiconductors in In–Ga–Zn–O system. Appl. Phys. Lett. 90, 488 (2007).

    Article  Google Scholar 

  2. J. Jang, J.C. Park, D. Kong, M.K. Dong, J.S. Lee, B.H. Sohn, H. Cho, and D.H. Kim: Endurance characteristics of amorphous-InGaZnO transparent flash memory with gold nanocrystal storage layer. IEEE Trans. Electron Devices 58, 3940 (2011).

    Article  CAS  Google Scholar 

  3. A. Suresh, S. Novak, P. Wellenius, V. Misra, and J.F. Muth: Transparent indium gallium zinc oxide transistor based floating gate memory with platinum nanoparticles in the gate dielectric. Appl. Phys. Lett. 94, 123501 (2009).

    Article  Google Scholar 

  4. W.T. Chen and H.W. Zan: High-performance light-erasable memory and real-time ultraviolet detector based on unannealed indium–gallium–zinc–oxide thin-film transistor. IEEE Electron Device Lett. 33, 77 (2012).

    Article  Google Scholar 

  5. K. Nomura, T. Kamiya, H. Yanagi, E. Ikenaga, K. Yang, K. Kobayashi, M. Hirano, and H. Hosono: Subgap states in transparent amorphous oxide semiconductor, In–Ga–Zn–O, observed by bulk sensitive X-ray photoelectron spectroscopy. Appl. Phys. Lett. 92, 202117 (2008).

    Article  Google Scholar 

  6. Y. Li, Y. Pei, R. Hu, Z. Chen, Y. Ni, J. Lin, X. Zhang, Z. Chen, J. Liang, B. Fan, G. Wang, and H. Duan: Charge trapping memory characteristics of amorphous-indium–gallium–zinc oxide thin-film transistors with defect-engineered alumina dielectric. IEEE Trans. Electron Devices 62, 1184 (2015).

    Article  CAS  Google Scholar 

  7. S. Chen, W.P. Zhang, X.M. Cui, Q.Q. Sun, and W. Zhang: Monochromatic light-assisted erasing effects of In–Ga–Zn–O thin film transistor memory with Al2O3/Zn-doped Al2O3/Al2O3 stacks. Appl. Phys. Lett. 104, 143502 (2014).

    Article  Google Scholar 

  8. X.M. Cui, S. Chen, S.J. Ding, Q.Q. Sun, T. Nyberg, S.L. Zhang, and W. Zhang: Unique UV-erasable In–Ga–Zn–O TFT memory with self-assembled Pt nanocrystals. IEEE Electron Device Lett. 34, 1011 (2013).

    Article  CAS  Google Scholar 

  9. S. Chen, X.M. Cui, S.J. Ding, and Q.Q. Sun: Novel Zn-doped Al2O3 charge storage medium for light-erasable In–Ga–Zn–O TFT memory. IEEE Electron Device Lett. 34, 1008 (2013).

    Article  CAS  Google Scholar 

  10. D.J. Yun, H.B. Kang, and S.M. Yoon: Process optimization and device characterization of nonvolatile charge trap memory transistors using In–Ga–ZnO thin films as both charge trap and active channel layers. IEEE Trans. Electron Devices 63, 3128 (2007).

    Article  Google Scholar 

  11. S.J. Kim, M.J. Park, D.J. Yun, W.H. Lee, G.H. Kim, and S.M. Yoon: High performance and stable flexible memory thin-film transistors using In–Ga–Zn–O channel and ZnO charge-trap layers on poly(ethylene naphthalate) substrate. IEEE Trans. Electron Devices 64, 1557 (2016).

    Article  Google Scholar 

  12. J.Y. Bak, M.K. Ryu, S.H.K. Park, C.S. Hwang, and S.M. Yoon: Impact of charge-trap layer conductivity control on device performance of top-gate memory thin-film transistors using IGZO channel and ZnO charge-trap layer. IEEE Trans. Electron Devices 61, 2404 (2014).

    Article  CAS  Google Scholar 

  13. H. Yin, S. Kim, H. Lim, Y. Min, C.J. Kim, I. Song, J. Park, S.W. Kim, A. Tikhonovsky, J. Hyun, and Y. Park: Program/erase characteristics of amorphous gallium indium zinc oxide nonvolatile memory. IEEE Trans. Electron Devices 55, 2071 (2008).

    Article  CAS  Google Scholar 

  14. L.F. Abbott and W.G. Regehr: Synaptic computation. Nature 431, 796 (2004).

    Article  CAS  Google Scholar 

  15. H. Tian, Q. Guo, Y. Xie, H. Zhao, C. Li, J.J. Cha, F. Xia, and H. Wang: Anisotropic black phosphorus synaptic device for neuromorphic applications. Adv. Mater. 28, 4991 (2016).

    Article  CAS  Google Scholar 

  16. J.H. Li and F. Yang: Solution-processable low-voltage and flexible floating-gate memories based on an n-type polymer semiconductor and high-k polymer gate dielectrics. ACS Appl. Mater. Interfaces 6, 12815 (2014).

    Article  CAS  Google Scholar 

  17. G.H. Seo, D.J. Yun, W.H. Lee, and S.M. Yoon: Atomic-layer-deposition-assisted ZnO nanoparticles for oxide charge-trap memory thin-film transistors. Nanotechnology 28, 075202 (2016).

    Article  Google Scholar 

  18. J.Y. Bark, S.J. Kim, C.W. Byun, S.H. Chi, J.E. Pi, M.K. Ryu, and S.M. Yoon: Effects of thickness and geometric variations in the oxide gate stack on the nonvolatile memory behaviors of charge-trap memory thin-film transistors. Solid-State Electron. 111, 153 (2015).

    Article  Google Scholar 

  19. Z. Ye, Y. Yuan, H. Xu, Y. Liu, J. Luo, and M. Wang: Mechanism and origin of hysteresis in oxide thin-film transistor and its application on 3-D nonvolatile memory. IEEE Trans. Electron Devices 64, 438 (2017).

    Article  CAS  Google Scholar 

  20. H.K. Noh, K.J. Chang, B. Ryu, and W.J. Lee: Electronic structure of oxygen-vacancy defects in amorphous In–Ga–Zn–O semiconductors. Phys. Rev. B 84, 115205 (2011).

    Article  Google Scholar 

Download references

Acknowledgments

The authors would like to acknowledge the financial support in part by the National Natural Science Foundation of China (Grant No. 61874029), and in part by the National Key Technologies Research and Development Program of China (Grant No. 2015ZX02102-003).

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Shi-Jin Ding.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Liu, DD., Pei, J., Li, L. et al. Multilevel memory and synaptic characteristics of a-IGZO thin-film transistor with atomic layer–deposited Al2O3/ZnO/Al2O3 stack layers. Journal of Materials Research 35, 732–737 (2020). https://doi.org/10.1557/jmr.2019.355

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1557/jmr.2019.355

Navigation