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Coupling of magnetism and structural phase transitions by interfacial strain

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Abstract

Proximity effects and exchange coupling across interfaces of hybrid magnetic heterostructures present unique opportunities for functional material design. In this review, we present an overview of recent experiments on magnetic hybrid materials in which magnetism was controlled by proximity to an active material. In particular, we discuss interfacial strain coupling of ferromagnetic materials in contact with a material undergoing a structural deformation. Bilayers containing VO2 and V2O3 as active materials are shown to strongly affect the magnetization and coercivity of ferromagnetic materials due to stress anisotropy caused by a temperature-dependent structural displacement in the oxide. The possibilities of tuning the system by sample morphology and materials choice are discussed in detail. In addition, we highlight a length-scale competition between magnetic and structural domains which leads to a maximum change in the coercivity in a narrow temperature window of the vanadium oxide phase transition.

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ACKNOWLEDGMENTS

The magnetism aspects of this work were supported by the Office of Basic Energy Science, U.S. Department of Energy, BES-DMS funded by the Department of Energy’s Office of Basic Energy Science, DMR under grant DE FG03 87ER-45332 and the oxide related science by the AFOSR (Grant No. FA9550-12-1-0381).

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Authors and Affiliations

  1. Department of Physics and Center for Advanced Nanoscience, University of California San Diego, La Jolla, California, 92093, USA

    Thomas Saerbeck, Siming Wang, Juan Gabriel Ramírez, Mikhail Erekhinsky, Ilya Valmianski & Ivan K. Schuller

  2. Department of Physics, Colorado State University, Fort Collins, Colorado, 80523, USA

    Jose de la Venta

  3. Materials Science and Engineering Program, University of California San Diego, La Jolla, California, 92093, USA

    Siming Wang

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  1. Thomas Saerbeck
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Saerbeck, T., de la Venta, J., Wang, S. et al. Coupling of magnetism and structural phase transitions by interfacial strain. Journal of Materials Research 29, 2353–2365 (2014). https://doi.org/10.1557/jmr.2014.253

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