Abstract
Recent nuclear forensics cases have focused primarily on plutonium (Pu) and uranium (U) materials. By definition however, nuclear forensics can apply to any diverted nuclear material. This includes neptunium (Np), an internationally safeguarded material like Pu and U, that could offer a nuclear security concern if significant quantities were found outside of regulatory control. This case study couples scanning electron microscopy (SEM) with quantitative analysis using newly developed specialized software, to evaluate a non-traditional nuclear forensic sample of Np. The results of the morphological analyses were compared with another Np sample of known pedigree, as well as other traditional actinide materials in order to determine potential processing and point-of-origin.
Similar content being viewed by others
References
D. K. Smith, M. J. Kristo, S. Niemeyer, G. B. Dudder, J. Radioanal. Nucl. Chem. 276 (2), 415–419 (2008).
M. J. Kristo, S. J. Tumey, Nucl. Instrum. Methods Phys. Res. Sect. B 294, 656–661 (2013).
K. J. Moody, I. D. Hutcheon, M. P. Grant, Nuclear Forensic Analysis. (CRC Press, Boca Raton, FL, 2005).
K. Mayer, M. Wallenius, I. Ray, Analyst 130, 433–441 (2005).
A. L. Tamasi, L. J. Cash, T. Mullen, A. R. Ross, C. E. Ruggerio, B. L. Scott, G. L. Wagner, J. R. Walensky, S. A. Zerkle, M. P. Wilkerson, J. Radioanal. Nucl. Chem. (2016).
J. Plaue, Ph.D., University of Nevada, Las Vegas, 2013.
M. Wallenius, K. Mayer, I. Ray, Forensic Sci. Int. 156, 55–62 (2006).
K. Mayer, M. Wallenius, T. Fanghanel, J. Alloys. Compd. 444–445, 50–56 (2007).
L. Tandon, et. al., J. Radioanal. Nucl. Chem. 276 (2), 467–473 (2008).
T. A. Nothwang, A. D. Neuman, C. C. Davis, S. L. Voit, M. R. Lopez, A. C. Martinez, JOM, 1667–1672 (2008).
C. Anderson-Cook, T. Burr, M. S. Hamada, C. Ruggerio, E. V. Thomas, Chemom. Intell. Lab. Syst. 149, 107–117 (2015).
D. Ho Mer Lin, Ph.D. Thesis, Ruperto-Carola University of Heidelberg, 2015.
I. Hutcheon, M. Kristo, K. Knight, Report No. LLNL-CONF-679869, 2015.
T. Burr, W. D. Stanbro, W. Charlton, J. Nuc. Sci. Technol. 38 (3), 209–216 (2001).
(Center for Nonproliferation Studies, Nuclear Threat Initiative, 2011), Vol. 2015.
M. Wallenius, K. Lutzenkirchen, K. Mayer, I. Ray, L. Aldave de las Heras, M. Betti, O. Cromboom, M. Hild, B. Lynch, A. Nicholl, H. Ottmar, G. Rasmussen, A. Schubert, G. Tamborini, H. Thiele, W. Wagner, C. Walker, E. Zuleger, J. Alloys. Compd. 444–445, 57–62 (2007).
J. M. Duffey, R. R. Livingston, Report No. WSRC-TC-2003-00388-R0, 2003.
D. T. Rankin, G. A. Burney, P. K. Smith, R. D. Sisson, in American Ceramic Society Bulletin (1977), Vol. 56, pp. 478–483.
D. T. Rankin, G. A. Burney, P. K. Smith, R. D. Sisson, Report No. DP-MS-75-119, 1976.
B. C. Hill, R. R. Livingston, Report No. WSRC-TR-2004-00296, 2004.
G. A. Burney, E. K. Dukes, Report No. DP-594, 1961.
S. L. Yarbro, S. L. Dunn, S. B. Schreiber, Report No. LA-11890, 1991.
W. E. Daniel, Report No. SRNL-TR-2011-00334, 2012.
X. Machuron-Mandard, C. Madic, J. Alloys. Compd. 235, 216–224 (1996).
J. A. Fahey, in The Chemistry of the Actinide Elements, edited by J. J. Katz, G. T. Seaborg, L. R. Morss, (Springer, Netherlands, 1986), Vol. 1, pp. 443–498.
Z. Yoshida, S. G. Johnson, T. Kimura, J. R. Krsul, in The Chemistry of the Actinide and Transactinide Elements, edited by L. R. Morss, N. M. Edelstein, J. Fuger, (Springer, The Netherlands, 2006).
C. E. Ruggiero, R. B. Porter, Report No. LA-UR-14-23586, 2014.
C. E. Ruggiero, R. B. Porter, Report No. LA-UR-14-23579, 2014.
P. K. Smith, G. A. Burney, D. T. Rankin, D. F. Bickford, R. D. Sisson, presented at the Sixth International Materials Symposium, Berkely, California, 1976 (unpublished).
J. L. Doyle, K. Kuhn, B. Byerly, L. Colletti, J. Fulwyler, K. Garduno, R. Keller, E. Lujan, A. Martinez, D. Porterfield, K. Spencer, F. Stanley, L. Townsend, M. Thomas, L. Walker, N. Xu, L. Tandon, (2016) Submitted
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Doyle, J.L., Schwartz, D. & Tandon, L. Nuclear Forensics of a Non-Traditional Sample: Neptunium. MRS Advances 1, 2999–3005 (2016). https://doi.org/10.1557/adv.2016.353
Published:
Issue Date:
DOI: https://doi.org/10.1557/adv.2016.353