Skip to main content
Log in

Preparation, characterization, and micropatterning of laser-dye-doped sol-gel films

  • Articles
  • Published:
Journal of Materials Research Aims and scope Submit manuscript

Abstract

Planar thin films of dye-doped silica were prepared by sol-gel synthesis. The optical properties of the films were characterized by transmittance measurements in the visible-infrared range and by photoluminescence. Micropatterns whose feature size was on the order of 2.4 μm, were imprinted on the film surface by a simple soft lithography approach. An optical microscope interfaced to a charge-coupled device camera was used to image the imprinted patterns and to analyze the patterned films photoluminescence. A sensitive spectral narrowing of the emission, which occurred only in micropatterned films, was attributed to the lateral confinement of the luminescence due to the micrometer-scale modulation of refractive index produced by the embossing procedure.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. S. Toyoda, N. Ooba, M. Hikita, T. Kurihara, and S. Imamura, Thin Solid Films 370, 311 (2000).

    Article  CAS  Google Scholar 

  2. X. Orignac, B. Barbieri, X.M. Du, R.M. Almeida, O. McCarthy, and E. Yeatman, Optical Mater. 12, 1 (1999).

    Article  CAS  Google Scholar 

  3. P. Innocenzi, A. Martucci, M. Guglielmi, L. Armelao, S. Pelli, G.C. Righini, and G.C. Battaglin, J. Non-Cryst. Solids 259, 182 (1999).

    Article  CAS  Google Scholar 

  4. J.T. Remillard, J.R. Jones, B.D. Poindexter, C.K. Narula, and W.H. Weber, Appl. Optics 38, 5306 (1999).

    Article  CAS  Google Scholar 

  5. Y. Ren, P. Mormile, L. Petti, and G.H. Cross, Sens. Actuators B 75, 76 (2001).

    Article  CAS  Google Scholar 

  6. K.M. Chen, A.W. Sparks, H-C. Luan, D.R. Lim, K. Wada, and L.C. Kimerling, Appl. Phys. Lett. 75, 24 (1999).

    Google Scholar 

  7. D. Blanc and S. Pelissier, Thin Solid Films 384, 251 (2001).

    Article  CAS  Google Scholar 

  8. J. Livage and D. Ganguli, Solar Energy Mater. Solar Cells 68, 365 (2000).

    Article  Google Scholar 

  9. Q.Y. Zhang and Z.H. Jiang, Mater. Chem. Phys. 69, 95 (2001).

    Article  CAS  Google Scholar 

  10. D. Lo, S.K. Lam, C. Ye, and K.S. Lam, Opt. Commun. 156, 316 (1998).

    Article  CAS  Google Scholar 

  11. R. Reisfeld, Opt. Mater. 16, 1 (2001).

    Article  CAS  Google Scholar 

  12. S.K. Lam, X.L. Zhu, and D. Lo, Appl. Phys. B 68, 1151 (1999).

    Article  CAS  Google Scholar 

  13. Y. Xia and G.M. Whitesides, Angew. Chem. Int. Ed. 37, 550 (1998).

    Article  CAS  Google Scholar 

  14. D.A. Doshi, N.K. Huesing, M. Lu, H. Fan, Y. Lu, K. Simmons-Potter, B.G. Potter, Jr., A.J. Hurd, and C.J. Brinker, Science 290, 107 (2000).

    Article  CAS  Google Scholar 

  15. J. Eang, X. Sun, L. Chen, and S. Chou, Appl. Phys. Lett. 75, 2767 (1999).

    Article  Google Scholar 

  16. P. Yang, G. Wirnsberger, H.C. Huang, S.R. Cordero, M.D. McGehee, B. Scott, T. Deng, G.M. Whitesides, B.F. Chmelka, S.K. Buratto, and G.D. Stucky, Science 287, 465 (2000).

    Article  CAS  Google Scholar 

  17. R. Reisfeld, E. Yariv, and H. Minti, Opt. Mater. 8, 31 (1997).

    Article  CAS  Google Scholar 

  18. T. Kawase, D.J. Pinner, R.H. Friend, and T. Shimoda, Synth. Met. 111, 583 (2000).

    Article  Google Scholar 

  19. A.N. Safonov, M. Jory, B.J. Matterson, J.M. Lupton, M.G. Salt, J.A.E. Wasey, W.L. Bernes, and I.D.W. Samuel, Synth. Met. 116, 145 (2001).

    Article  CAS  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Rights and permissions

Reprints and permissions

About this article

Cite this article

Arena, A., Patanè, S., Saitta, G. et al. Preparation, characterization, and micropatterning of laser-dye-doped sol-gel films. Journal of Materials Research 17, 2095–2098 (2002). https://doi.org/10.1557/JMR.2002.0309

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1557/JMR.2002.0309

Navigation