Abstract.
The dynamics of the surface plasmon in laser-driven metallic nanoparticles is described by means of a master-equation formalism. Within the Markov approximation, the dynamics is studied for different regimes ranging from weak excitation in photoabsorption experiments to strong excitation in pump-probe spectroscopy. It is shown that two collective levels are sufficient to describe the dynamics of the surface plasmon. On this basis, we predict the appearance of sidebands in the absorption spectrum of the probe laser field in pump-probe experiments.
Similar content being viewed by others
References
W.A. de Heer, Rev. Mod. Phys. 65, 611 (1993)
M. Brack, Rev. Mod. Phys. 65, 677 (1993)
T. Tokizaki, A. Nakamura, S. Kaneko, K. Uchida, S. Omi, H. Tanji, Y. Asahara, Appl. Phys. Lett. 65, 941 (1994)
J.-Y. Bigot, J.-C. Merle, O. Cregut, A. Daunois, Phys. Rev. Lett. 75, 4702 (1995)
M. Perner, P. Bost, U. Lemmer, G. von Plessen, J. Feldmann, U. Becker, M. Mennig, M. Schmitt, H. Schmidt, Phys. Rev. Lett. 78, 2192 (1997)
V. Halté, J. Guille, J.-C. Merle, I. Perakis, J.-Y. Bigot, Phys. Rev. B 60, 11738 (1999)
J.-Y. Bigot, V. Halté, J.-C. Merle, A. Daunois, Chem. Phys. 251, 181 (2000)
N. Del Fatti, F. Vallée, C. Flytzanis, Y. Hamanaka, A. Nakamura, Chem. Phys. 251, 215 (2000)
C. Voisin, N. Del Fatti, D. Christofilos, F. Vallée, J. Phys. Chem. B 105, 2264 (2001)
G. Weick, D. Weinmann, G.-L. Ingold, R.A. Jalabert, Europhys. Lett. 78, 27002 (2007)
L.G. Gerchikov, C. Guet, A.N. Ipatov, Phys. Rev. A 66, 053202 (2002)
G. Weick, R.A. Molina, D. Weinmann, R.A. Jalabert, Phys. Rev. B 72, 115410 (2005)
G. Weick, G.-L. Ingold, R.A. Jalabert, D. Weinmann, Phys. Rev. B 74, 165421 (2006)
C. Cohen-Tannoudji, J. Dupont-Roc, G. Grynberg, Atom-photon interactions: Basic processes and applications (Wiley-VCH, New York, 1992)
K. Hagino, Phys. Rev. B 60, R2197 (1999)
C. Yannouleas, R.A. Broglia, Ann. Phys. (N.Y.) 217, 105 (1992)
C. Seoanez, G. Weick, R.A. Jalabert, D. Weinmann, Eur. Phys. J. D 44, 351 (2007)
See, e.g., U. Weiss, Quantum Dissipative Systems (World Scientific, Singapore, 1993) which can also serve as a guide to the recent literature in this field
W.E. Lamb, R.C. Retherford, Phys. Rev. 72, 241 (1947); W.E. Lamb, Rep. Prog. Phys. 14, 19 (1951)
R. Schlipper, R. Kusche, B. von Issendorff, H. Haberland, Phys. Rev. Lett. 80, 1194 (1998); R. Schlipper, R. Kusche, B. von Issendorff, H. Haberland, Appl. Phys. A: Mater. Sci. Process. 72, 255 (2001)
D.F. Walls, G.J. Milburn, Quantum Optics (Springer-Verlag, Berlin, 1994)
C. Cohen-Tannoudji, S. Reynaud, J. Phys. B: At. Mol. Phys. 10, 345 (1977); C. Cohen-Tannoudji, S. Reynaud, in: Proc. Int. Conf. on Multiphoton Processes, edited by J.H. Eberly, P. Lambropoulos (Wiley, New York, 1978), p. 103
F.Y. Wu, S. Ezekiel, M. Ducloy, B.R. Mollow, Phys. Rev. Lett. 38, 1077 (1977)
C. Wei, N.B. Manson, Phys. Rev. A 49, 4751 (1994)
B.R. Mollow, Phys. Rev. A 5, 2217 (1972)
Y.-H. Liau, A.N. Unterreiner, Q. Chang, N.F. Scherer, J. Phys. Chem. B, 105, 2135 (2001)
R.A. Molina, D. Weinmann, R.A. Jalabert, Phys. Rev. B 65, 155427 (2002); R.A. Molina, D. Weinmann, R.A. Jalabert, Eur. Phys. J. D 24, 127 (2003)
G. Lindblad, Commun. Math. Phys. 48, 119 (1976); V. Gorini, A. Kossakowski, E.C.G. Sudarshan, J. Math. Phys. 17, 821 (1976)
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Weick, G., Ingold, GL., Weinmann, D. et al. Sidebands in the light absorption of driven metallic nanoparticles. Eur. Phys. J. D 44, 359–366 (2007). https://doi.org/10.1140/epjd/e2007-00197-2
Received:
Published:
Issue Date:
DOI: https://doi.org/10.1140/epjd/e2007-00197-2