# A multi-isotope \(0\nu 2\beta \) bolometric experiment

## Abstract

There are valuable arguments to perform neutrinoless double beta (\(0\nu 2\beta \)) decay experiments with several nuclei: the uncertainty of nuclear-matrix-element calculations; the possibility to test these calculations by using the ratio of the measured lifetimes; the unpredictability of possible breakthroughs in the detection technique; the difficulty to foresee background in \(0\nu 2\beta \) decay searches; the limited amount of isotopically enriched materials. We propose therefore approaches to estimate the Majorana neutrino mass by combining experimental data collected with different \(0\nu 2\beta \) decay candidates. In particular, we apply our methods to a next-generation experiment based on scintillating and Cherenkov-radiation bolometers. Current results indicate that this technology can effectively study up to four different isotopes simultaneously (\(^{82}\)Se, \(^{100}\)Mo, \(^{116}\)Cd and \(^{130}\)Te), embedded in detectors which share the same concepts and environment. We show that the combined information on the Majorana neutrino mass extracted from a multi-candidate bolometric experiment is competitive with that achievable with a single isotope, once that the cryogenic experimental volume is fixed. The remarkable conceptual and technical advantages of a multi-isotope investigation are discussed. This approach can be naturally applied to the proposed CUPID project, follow-up of the CUORE experiment that is currently taking data in the Gran Sasso underground laboratory.

## 1 Introduction

Neutrinoless double beta (\(0\nu 2\beta \)) decay is considered as one of the most promising ways to investigate the properties of neutrino and weak interactions, to test lepton number conservation, and in general to probe the Standard Model (SM) of particle physics [1, 2, 3, 4, 5, 6, 7]. Despite the almost 70-year-long history of \(0\nu 2\beta \) decay search, this elusive process is still not observed: the most sensitive experiments provide limits on the effective Majorana neutrino mass of the electron neutrino on the level of \(\lim \langle m_{\nu }\rangle \sim 0.1\)–1 eV (see the status of the \(0\nu 2\beta \) decay search in the reviews [2, 3, 4, 5, 6, 7, 8, 9, 10, 11, 12] and the recent experimental results [13, 14, 15, 16, 17, 18]).

The exploration of the inverted neutrino mass hierarchy (\(\langle m_{\nu }\rangle \sim 0.02\)–0.05 eV) is a challenge of the experiments in preparation or R&D stage. Such a sensitivity can be reached in searches able to detect an extremely low activity with half-life in the range \(T_{1/2} \sim 10^{26}\)–\(10^{27}\) yr for the most promising candidates. However, taking into account the possible quenching of the axial vector coupling constant \(g_A\) [19, 20, 21, 22], the experimental program should foresee the possibility to go towards an-order-of-magnitude higher half-life sensitivities, of the order of \(T_{1/2} \sim 10^{27}\)–\(10^{28}\) yr. The accomplishment of such an ambitious plan requires the construction of detectors containing a large number of \(2\beta \) active nuclei (\(10^{27}\)–\(10^{28}\) nuclei, \(\sim 10^3\)–\(10^4\) moles of isotope of interest), with an as-high-as-possible detection efficiency and an extremely low (ideally zero) radioactive background, and able to distinguish the effect searched for. The last requirement implies, in particular, an as-high-as-possible energy resolution – to identify the effect unambiguously and to avoid the presence of a tail from the SM-allowed two-neutrino double beta (\(2\nu 2\beta \)) decay in the region of the \(0\nu 2\beta \) peak (region of interest, ROI) – and time resolution – to avoid random coincidences of events from \(2\nu 2\beta \) decays and other components of the background [23].

The technique of scintillating and Cherenkov-radiation low-temperature bolometers [24, 25, 26, 27, 28, 29] is one of the most suitable detection method for the next generation \(2\beta \) experiments, thanks to the high detection efficiency (70–90%, depending on the crystal composition and volume) and the excellent energy resolution (a few keV). In addition, this technique suppresses the background caused by \(\alpha \) radioactive contamination to a very low level thanks to the excellent particle discrimination. Following this approach, the CUPID group of interest [30] proposes to perform a tonne-scale bolometric \(0\nu 2\beta \) decay search with a sensitivity high enough to probe the inverted hierarchy of the neutrino mass and even go towards the normal hierarchy region. This experiment would be a follow-up to the CUORE experiment with particle identification for background rejection.

There are both theoretical and experimental arguments to develop \(0\nu 2\beta \) decay experiments with several nuclei. First of all, the ambiguity of the theoretical calculations of nuclear matrix elements (NME) of the \(0\nu 2\beta \) decay remains significant, not to say that there are no experimental tests of the calculations so far. Therefore, no one can safely suggest the nucleus with the highest decay probability. Furthermore, data on \(0\nu 2\beta \) decay rate in a few nuclei will be definitely useful to adjust theoretical calculations of the NME since the ratio of the calculated lifetimes is very sensitive to different models [31]. From the experimental point of view, taking into account the extremely low decay probability and the possibility that spurious effects mimick the signal searched for, an observation of \(0\nu 2\beta \) decay in different nuclei will be requested in case of positive evidence in one of the candidates. Indeed, there have already been many false claims of double beta decay in the history of the experimental search for this process [32].

Therefore, there is a strong call for experiments with several nuclei candidates. At the same time one can extract competitive estimations of the Majorana neutrino mass by combining data of experiments with several different isotopes. In this paper we demonstrate that the sensitivity to the Majorana neutrino mass that can be achieved in a cryogenic experiment with several nuclei is similar to the sensitivity of an experiment utilizing only one of the candidates and exploiting the same experimental volume. Of course, the same argument can be applied to other physics parameters related to different mechanisms inducing \(0\nu 2\beta \) decay, although deepening this aspect goes beyond the scope of this paper.

## 2 Experimental concepts

On the basis of the above considerations, we propose a next generation \(0\nu 2\beta \) decay bolometric experiment studying several isotopes simultaneously. To complete the general discussion of the previous section, we stress that there are also practical, but not less important, reasons to implement such cryogenic \(0\nu 2\beta \) experiment: the production of a large amount of a given isotope (at the hundreds of kg scale) looks rather questionable, while the production, e.g., of one quarter of the same quantity for four isotopes looks more realistic, given the existing enrichment techniques and capabilities. We remark that different sets of centrifugues are used for different nuclei in the centrifugation enrichment technique (presently the only one that provides a high enough throughput). Enrichment in different isotopes can therefore be performed in parallel. A similar argument applies to crystal production, which is mandatory for the bolometric approach. Crystals containing different candidates can be grown in parallel, since each type of crystal requires specific technologies and is typically produced in a specialized laboratory or company. A multi-isotope experiment can therefore provide a remarkable reduction of the time required to build the detector, especially in the case, discussed below, in which the single module structure is the same for each type of crystal.

We will consider the candidates \(^{82}\)Se, \(^{100}\)Mo, \(^{116}\)Cd and \(^{130}\)Te, which can be studied with the scintillating (the first three ones) and Cherenkov-radiation (the last one) bolometric technique with excellent prospects. Although our considerations apply to a generic next-generation cryogenic experiment, the most natural implementation of this multi-isotope approach is in the framework of the CUPID proposal. Therefore, in the following we will refer to the four-isotope option as CUPID-4, while we will designate CUPID-1 the conventional one-isotope version preliminarily discussed in Ref. [30].

As for the detector technology, we will stick to the basic configuration of the single module of CUORE [14, 15], consisting of a large crystal (125 cm\(^3\) in case of CUORE) coupled to a neutron transmutation doped (NTD) Ge thermistor, working as a temperature sensor, and to a Si-doped heater for detector response stabilization. Each crystal is hold by small PTFE elements inside a copper frame. The read-out electronics operates at room temperature and is based on the well-known Si-JFET technology. CUORE is taking data successfully [15] and there is no reason to change substantially this experimental configuration.

The bolometric light detector, which is not present in CUORE but will be necessary to reject the \(\alpha \) background in future bolometric searches, will consist of a thin Ge disk (50 mm diameter, 0.15 mm thickness) with an NTD Ge thermistor as well. It will be operated in the Neganov–Luke mode in order to achieve a high enough sensitivity to reject \(\alpha \) background in the TeO\(_2\) crystals – used in the \(^{130}\)Te section – by exploiting Cherenkov radiation [28, 33, 34] and the two-neutrino double beta decay random coincidences in the \(^{100}\)Mo section [35]. The same Si-JFET-based read-out electronics adopted for the main crystal, and used now in CUORE, can be employed. The same type of light detectors can be coupled to all the four crystal types, but the Neganov–Luke option is not strictly necessary in the \(^{82}\)Se and \(^{116}\)Cd cases. Of course, other technologies for the light detector may be viable: a vibrant R&D activity is ongoing on this subject [29, 30].

We will assume an array of 1300 scintillating and Cherenkov-radiation bolometers (compatible with the experimental volume of the current CUORE cryostat or of a similar dedicated infrastructure) based on cylindrical ultra-radiopure crystals – 5 cm diameter and 5 cm height – enriched to 100% in the isotope of interest. In case of the CUPID-1 option, the crystals will consist of only one of the following compounds: zinc selenide (Zn\(^{82}\)Se), lithium molybdate (Li\(_{2}^{100}\)MoO\(_4\)), cadmium tungstate (\(^{116}\)CdWO\(_4\)), or tellurium oxide (\(^{130}\)TeO\(_2\)). As for the CUPID-4 option, we will assume that the 1300 elements will be shared among crystals of each type. We stress that a remarkable advantage of the bolometric technique for a multi-isotope experiment is that detectors are based exactly on the same technology, are operated in the same set-up and are exposed to the same background sources.

All the four aforementioned compounds have been successfully tested as scintillating or Cherenkov-radiation bolometers, using crystals grown from enriched materials. It was shown as well that the Neganov–Luke light detectors have the requested performance [34]. The energy resolution of the detectors at the energies \(Q_{2\beta }\) were estimated from existing experimental data concerning ZnSe [36], Li\(_2\)MoO\(_4\) [37], CdWO\(_4\) [38], and TeO\(_2\) [39]. The detection efficiencies for the \(0\nu 2\beta \) decay effect were taken from Ref. [27] (ZnSe and TeO\(_2\)), while for Li\(_2\)MoO\(_4\) and CdWO\(_4\) detectors the efficiencies were estimated by using the GEANT4 simulation package.

## 3 Approaches to estimate neutrino mass from several \(0\nu 2\beta \) experiments

A value (limit) on the effective Majorana neutrino mass can be derived from the experimental data collected by an experiment following the CUPID-4 scheme. Attempts to estimate a limit on the effective Majorana neutrino mass combining data of the most sensitive experiments are already reported in the literature [40, 41]. We propose here other approaches driven also by the quite similar performance of the cryogenic detectors foreseen in CUPID.

### 3.1 Sum of counts in the region of interest

*i*-th \(0\nu 2\beta \) experiment with \(N_i\) nuclei, with a detection efficiency \(\varepsilon _i\), over a live time \(t_i\) is inversely proportional to the nucleus half-life:

*S*(\(\lim S\)) can be obtained from the analysis of the experimental data accumulated with several detectors as following (assuming a large enough number of counts):

Nevertheless, as it will be shown in Sects. 4.3 and 4.4, the method is quite effective in case of experiments with similar mass of the isotope of interest, background, efficiency and energy resolution, which is expected to be the case of CUPID-4.

In Sect. 4.4 we will consider “zero background” CUPID-like experiments. Approximation of data with mainly bins with zero counts is not robust enough. Thus, one can calculate the sum of counts in selected energy intervals to estimate experimental sensitivities to the Majorana neutrino mass by using only the given background and no true signal.

### 3.2 Weighted averages and errors of neutrino mass square

This method reduces the impact of experiments with high background on the combined neutrino mass limit. This approach can be applied to extract a combined limit even from experiments with rather different characteristics (e.g., bolometers, HPGe detectors, Xe-filled scintillators, etc).

Below we will show how the discussed methods can be applied to the case of CUPID-like experiments.

## 4 Results and discussion

### 4.1 Input data

The various contributions to the background in a large scintillating and Cherenkov-radiation bolometric experiment and in the CUORE experiment are discussed respectively in Ref. [27] and Ref. [43]. According to the discussions in these works, we will assume that the external contributions to the background (external \(\gamma \) radiation, muons, neutrons) can be reduced to below 10\(^{-4}\) counts/yr/keV/kg by proper material selection and shielding. A similarly low contribution will be provided by the bulk crystal radioactivity. The dominant source of background will be then related to contamination of close structures, typically the surface of the crystals and of the holders. Presently, \(\alpha \) particles generated at the surface of the crystal holders are indeed the dominant background source in CUORE, at the level of 10\(^{-2}\) counts/yr/keV/kg [15, 43]. Switching on particle identification capability by the detection of light emitted by the crystals, the residual level of background is estimated by the simulations based on the CUORE background model and reported in Ref. [44]. The remaining background events are determined by \(\beta \)’s and \(\gamma \)’s emitted by close contamination of the crystals and details of the set-up. The most challenging contaminant nuclei are the \(\beta \) active \(^{208}\)Tl (\(Q_{\beta }=4999\) keV, descendant of \(^{228}\)Th in the \(^{232}\)Th family) and \(^{214}\)Bi (\(Q_{\beta }=3269\) keV, descendant of \(^{226}\)Ra in the \(^{238}\)U family). Both \(Q_{\beta }\) values exceed the \(Q_{2\beta }\) of the CUPID-4 isotopes of interest.

Characteristics of a possible CUPID set-up with \(^{82}\)Se, \(^{100}\)Mo, \(^{116}\)Cd and \(^{130}\)Te in the CUPID-1 option assuming 1300 detector modules with \(\oslash 5\times 5\) cm crystals enriched to 100% in the isotope of interest. The considered parameters are the FWHM energy resolution at \(Q_{2\beta }\) (FWHM), the detection efficiency (\(\varepsilon \)), the detector mass (*M*) and the number of nuclei of interest (*N*)

Candidate | \(Q_{2\beta }\) (keV) | Crystal | FWHM | \(\varepsilon \) | | |
---|---|---|---|---|---|---|

[48] | compound | (keV) | (kg) | |||

\(^{82}\)Se | 2997.9(5) | Zn\(^{82}\)Se | 13.8 | 0.76 | 672 | \(2.75\times 10^{27}\) |

\(^{100}\)Mo | 3034.36(17) | Li\(_{2}^{100}\)MoO\(_4\) | 5.4 | 0.80 | 389 | \(1.32\times 10^{27}\) |

\(^{116}\)Cd | 2813.49(13) | \(^{116}\)CdWO\(_4\) | 5.5 | 0.90 | 1008 | \(1.67\times 10^{27}\) |

\(^{130}\)Te | 2527.51(1) | \(^{130}\)TeO\(_2\) | 5.0 | 0.87 | 771 | \(2.87\times 10^{27}\) |

### 4.2 Sensitivity of CUPID-1 experiments

^{1}Ten thousands of randomly generated energy spectra were fitted by the maximum-likelihood method

^{2}to estimate the average errors of the peak area \(\sigma (S_i)\) for each nucleus. Examples of the fits are presented in Fig. 1 (energy spectra with \(S_i\approx 0\) and \(\sigma (S_i)\) equal to the average values for each detector were chosen for the presentation). The values of \(\lim S_i\) were estimated by using the Feldman-Cousins procedure [45] from the \(\sigma (S_i)\) values assuming \(S_i=0\) counts. A slightly higher sensitivity was achieved by using energy spectra with bins in units of energy resolution as it is shown in Fig. 2.

^{3}This improvement can be explained by an increase of statistics thanks to the binning in units of energy resolution. The results are presented in Table 2.

^{4}The neutrino mass limits here and below have been calculated by using the matrix elements from Ref. [46], the phase space factors from Ref. [47] and the value of the axial vector coupling constant \(g_A=1.27\). We would like to stress that the choice of the matrix elements from Ref. [46] does not mean that we give preference to these calculations, but it is used only to illustrate our approach. In Sect. 4.5 we will give a picture of the CUPID-1 and CUPID-4 sensitivity to neutrino mass using other calculations too. In the right columns of Figs. 1 and 2 positive signals for the effective neutrino mass \(\langle m_{\nu } \rangle =0.05\) eV are shown (we have used the same NME calculations to estimate the numbers of counts as for the limit estimations above).

Sensitivity of CUPID-1 experiments with Zn\(^{82}\)Se, Li\(_{2}^{100}\)MoO\(_4\), \(^{116}\)CdWO\(_4\) and \(^{130}\)TeO\(_2\) detectors assuming the background in the ROI simulated in Ref. [44] (denoted as \(I_{BG}\), counts/yr/keV/kg). The limits on the number of events, the half-lives and the neutrino mass are given at 90% C.L. The neutrino mass limits are calculated by using the matrix elements from Ref. [46], the phase space factors from Ref. [47] and the value of the axial vector coupling constant \(g_A=1.27\)

Isotope | \(I_{BG}\) | \(\sigma _S\) | \(\lim S\) | \(\lim T_{1/2}\) | \(\lim \langle m_{\nu } \rangle \) |
---|---|---|---|---|---|

(counts) | (counts) | (yr) | (eV) | ||

\(^{82}\)Se | \(3.8\times 10^{-4}\) | 7.58 | 12.4 | \(1.2\times 10^{27}\) | 0.025 |

\(^{100}\)Mo | \(3.0\times 10^{-4}\) | 2.77 | 4.54 | \(1.6\times 10^{27}\) | 0.015 |

\(^{116}\)Cd | \(4.3\times 10^{-4}\) | 6.11 | 10.0 | \(1.0\times 10^{27}\) | 0.025 |

\(^{130}\)Te | \(6.0\times 10^{-4}\) | 6.36 | 10.4 | \(1.7\times 10^{27}\) | 0.018 |

### 4.3 Sensitivity of CUPID-4 and combined limits on the neutrino mass

The sensitivity of CUPID-4 was estimated by using both the sum of counts in the ROI and the weighted averages methods.

Values of *S* and \(\sigma (S)\) can be estimated by using formula (5) and by a fit of the sum spectrum of several detectors. It should be noted that one can sum spectra measured with different nuclei (and therefore with different \(Q_{2\beta }\) values). For this purpose the spectra can be binned equally (e.g., 1 keV per channel, as in Fig. 1) or in units of energy resolution (as in Fig. 2). They can then be shifted in energy so that the decay energies of all the nuclei are in the same channel. Binning in units of energy resolution improves statistics and looks a preferable approach in case of different energy resolutions. Below we will use energy spectra binned in units of energy resolution.

The generated energy spectra of the four sets of detectors and the sum spectrum are shown in Fig. 3. The results of the fits are presented in Fig. 3 and Table 3. An estimation by using formula (5) gives \(\lim \langle m_{\nu } \rangle =0.020\) eV. Then the sum spectrum was fitted by the sum of four Gaussian functions with energy resolution FWHM=5 channels. This approach gives almost the same result: \(\lim \langle m_{\nu } \rangle =0.021\) eV. The excluded peaks for the four detectors and for the sum spectrum are shown in Fig. 3.

The best limit \(\lim \langle m_{\nu } \rangle =0.018\) eV was obtained with the second method by using the values of weighted errors of squares of neutrino mass \(\sigma \langle m_{\nu } \rangle ^2\) listed in Table 3.

Sensitivity of the CUPID-4 experiment with Zn\(^{82}\)Se, Li\(_{2}^{100}\)MoO\(_4\), \(^{116}\)CdWO\(_4\) and \(^{130}\)TeO\(_2\) detectors assuming the level of background simulated in Ref. [44] (denoted as \(I_{BG}\), counts/yr/keV/kg). The errors \(\sigma \langle m_{\nu } \rangle ^2\) and the neutrino mass limits were calculated by using the matrix elements from Ref. [46], the phase space factors from Ref. [47] and the value of the axial vector coupling constant \(g_A=1.27\)

Isotope | Approach to estimate | \(I_{BG}\) | \(\sigma _S\) | \(\lim S\) | \(\lim T_{1/2}\) | \(\lim \langle m_{\nu } \rangle \) | \(\sigma \langle m_{\nu } \rangle ^2\) |
---|---|---|---|---|---|---|---|

\(\langle m_{\nu } \rangle \) combined limit | (counts) | (counts) | (yr) | (eV) | (eV\(^2\)) | ||

\(^{82}\)Se | \(3.8\times 10^{-4}\) | 3.39 | 5.56 | \(6.5\times 10^{26}\) | 0.033 | 0.00067 | |

\(^{100}\)Mo | \(3.0\times 10^{-4}\) | 1.49 | 2.44 | \(7.5\times 10^{26}\) | 0.022 | 0.00029 | |

\(^{116}\)Cd | \(4.3\times 10^{-4}\) | 2.62 | 4.30 | \(6.1\times 10^{26}\) | 0.032 | 0.00063 | |

\(^{130}\)Te | \(6.0\times 10^{-4}\) | 3.09 | 5.07 | \(8.5\times 10^{26}\) | 0.025 | 0.00037 | |

Estimation of peak | 5.49 | 9.00 | 0.020 | ||||

Estimation of peak | 5.88 | 9.64 | 0.021 | ||||

area by fit (Sect. 3.1) | |||||||

Method described | 0.018 \(\Longleftarrow \) | 0.00020 | |||||

in Sect. 3.2 |

### 4.4 Sensitivity of “zero-background” experiments

Sensitivity of CUPID-1 experiments with Zn\(^{82}\)Se, Li\(_{2}^{100}\)MoO\(_4\), \(^{116}\)CdWO\(_4\) and \(^{130}\)TeO\(_2\) detectors assuming a level of background of \(4\times 10^{-6}\) counts/year/kg/keV. The expected background in the energy intervals \(\approx \pm 2\sigma \) are denoted as \(N_{BG}\). The neutrino mass limits \(\lim \langle m_{\nu } \rangle \) were calculated by using the matrix elements from Ref. [46], the phase space factors from Ref. [47] and the value of the axial vector coupling constant \(g_A=1.27\)

Isotope | \(N_{BG}\) | \(\lim S\) | \(\lim T_{1/2}\) | \(\lim \langle m_{\nu } \rangle \) |
---|---|---|---|---|

(counts) | (counts) | (yr) | (eV) | |

\(^{82}\)Se | 0.63 | 2.98 | \(4.6\times 10^{27}\) | 0.012 |

\(^{100}\)Mo | 0.14 | 2.56 | \(2.7\times 10^{27}\) | 0.011 |

\(^{116}\)Cd | 0.38 | 2.76 | \(3.6\times 10^{27}\) | 0.013 |

\(^{130}\)Te | 0.26 | 2.66 | \(6.2\times 10^{27}\) | 0.009 |

The energy spectra for the Majorana neutrino mass \(\langle m_{\nu } \rangle =0.02\) eV are presented in the right columns of Figs. 4 and 5. The effect can be detected in both CUPID configurations.

### 4.5 Dependence on nuclear matrix elements calculations

Sensitivity of the CUPID-4 experiment with Zn\(^{82}\)Se, Li\(_{2}^{100}\)MoO\(_4\), \(^{116}\)CdWO\(_4\) and \(^{130}\)TeO\(_2\) detectors assuming a level of background of \(4\times 10^{-6}\) counts/year/kg/keV. The numbers of background events in the energy intervals \(\approx \pm 2\sigma \) for each detector and for the sum spectrum (last line) are denoted as \(N_{BG}\). The neutrino mass limits \(\lim \langle m_{\nu } \rangle \) were calculated by assuming no true signal (see discussion in Sect. 4.4) and assuming the matrix elements from Ref. [46], the phase space factors from Ref. [47] and the value of the axial vector coupling constant \(g_A=1.27\)

Isotope | \(N_{BG}\) | \(\lim S\) | \(\lim T_{1/2}\) | \(\lim \langle m_{\nu } \rangle \) |
---|---|---|---|---|

(counts) | (counts) | (yr) | (eV) | |

\(^{82}\)Se | 0.16 | 2.57 | \(1.3\times 10^{27}\) | 0.023 |

\(^{100}\)Mo | 0.04 | 2.47 | \(7.1\times 10^{26}\) | 0.022 |

\(^{116}\)Cd | 0.09 | 2.52 | \(9.9\times 10^{26}\) | 0.025 |

\(^{130}\)Te | 0.07 | 2.50 | \(1.6\times 10^{27}\) | 0.018 |

Combined | 0.36 | 2.74 | 0.011 | |

\( \langle m_{\nu } \rangle \) limit |

## 5 Conclusions

Two approaches to estimate the Majorana neutrino mass from \(0\nu 2\beta \) decay experiments with several nuclei are proposed. The former method uses a sum of counts in the region of interest, while the latter one estimates the Majorana neutrino mass from weighted averages and errors of neutrino mass squares. The former approach is especially effective in case of similar detector performance and can be used even in the “zero background” conditions with a very poor statistics, while the latter approach allows one to estimate the neutrino mass also from experiments with completely different detectors.

By applying these methods, we have shown that the sensitivity to the neutrino mass that can be achieved in a single bolometric experiment with several nuclei (e.g., with \(^{82}\)Se, \(^{100}\)Mo, \(^{116}\)Cd, and \(^{130}\)Te) is similar to the sensitivity of a technically equivalent experiment based on only one of these nuclei and contained in the same cryostat volume. Actually, Tables 2 and 4, as well as Fig. 6, show that the pure \(^{130}\)Te option gives better results. We have to consider however that predictions of background are less safe for this nucleus, since this is the only one for which the signal is below the end point of the bulk of the natural \(\gamma \) radioactivity (2615 keV). A possible way to mitigate the effects of a residual background component from external \(\gamma \)s is to place the TeO\(_2\) crystals in the central part of the array so that the other crystals act as an active shield for the \(^{130}\)Te section.

It should be stressed that a similar data analysis can be applied not only to the Majorana neutrino mass assessment in the framework of the mass mechanism involving light neutrino exchange, but also to the estimation of physics parameters related to other possible extensions of the SM that predict \(0\nu 2\beta \) decay.

Since a multi-isotope bolometric experiment is not less sensitive than a single-isotope one to the physics parameters that rule \(0\nu 2\beta \) decay (once that background and NME uncertainties are taken into account), we believe that it represents by far a better option, for a number of fundamental and practical reasons we have extensively discussed in the previous sections. This multi-isotope approach can be naturally implemented in the framework of CUPID, which can be based in principle on very similar detectors containing different candidates and exploiting well-established technologies. We emphasize that a competitive single experiment combining results from several candidates with similar sensitivities represents a new original idea in the \(0\nu 2\beta \) decay search strategy, which currently can be effectively implemented only in the bolometric approach.

Finally, it should be noted that a multi-isotope experiment could allow for precise measurements of the \(2\nu 2\beta \) decay half-lives, which are important nuclear data also for the development of a model aiming at accurate calculations of the neutrinoless mode of the transition.

## Footnotes

- 1.
Strictly speaking, the background counting rate in Ref. [44] was estimated for TeO\(_2\) crystals. We use the simulation results also for the other compounds (taking into account of course the different \(Q_{2\beta }\)’s) assuming that the background level does not depend significantly on the detector material, as expected if the contamination is mainly located in the holders.

- 2.
We have applied the likelihood fit taking into account that approximation by the least squares method is not robust enough in the case of low statistics data, since it ignores zero entry bins.

- 3.
In this Figure and in all the following ones where spectra are shown the binning is FWHM(keV)/5.

- 4.
Similar estimations of \(S_{\sigma }\) values can be obtained by the simple equation \(S_{\sigma }\approx \sqrt{I_{BG}\times t \times M \times 1.75\times FWHM}\). However, this simple estimate becomes less relevant in case of lower statistics (even in the CUPID-1 option in case of shorter data-taking time).

## Notes

### Acknowledgements

The authors thank Dr. V.V. Kobychev for the Monte-Carlo simulations of \(0\nu 2\beta \) decay detection efficiencies of Li\(_2\)MoO\(_4\) and CdWO\(_4\) detectors. The researches were supported in part by the joint scientific project “Development of Cd-based scintillating bolometers to search for neutrinoless double-beta decay of \(^{116}\)Cd” in the framework of the PICS (Program of International Cooperation in Science) of CNRS in years 2016–2018. F.A.D. gratefully acknowledges support from the Scientific High-Level Scholarship Commission of the French Embassy in Kyiv (Ukraine) and the “Jean d’Alembert” Grants program of the University of Paris-Saclay. F.A.D. and V.I.T. were supported in part by the IDEATE International Associated Laboratory (LIA) and by the project “Investigation of neutrino and weak interaction in double beta decay of \(^{100}\)Mo” in the framework of the Programme “Dnipro” based on Ukraine-France Agreement on Cultural, Scientific and Technological Cooperation.

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