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Thermodynamics of the frustrated J1-J2 Heisenberg ferromagnet on the body-centered cubic lattice with arbitrary spin

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Abstract

We use the spin-rotation-invariant Green’s function method as well as the high-temperature expansion to discuss the thermodynamic properties of the frustrated spin-S J 1-J 2 Heisenberg magnet on the body-centered cubic lattice. We consider ferromagnetic nearest-neighbor bonds J 1< 0 and antiferromagnetic next-nearest-neighbor bonds J 2 ≥ 0 and arbitrary spin S. We find that the transition point \hbox{$J_2^c$} J 2 c between the ferromagnetic ground state and the antiferromagnetic one is nearly independent of the spin S, i.e., it is very close to the classical transition point \hbox{$J_2^{c,{\rm clas}}= \frac{2}{3}|J_1|$} J 2 c, clas = 2 3 | J 1 | . At finite temperatures we focus on the parameter regime \hbox{$J_2<J_2^c$} J 2 < J 2 c with a ferromagnetic ground-state. We calculate the Curie temperature T C (S, J 2) and derive an empirical formula describing the influence of the frustration parameter J 2 and spin S on T C . We find that the Curie temperature monotonically decreases with increasing frustration J 2, where very close to \hbox{$J_2^{c,{\rm clas}}$} J 2 c, clas the T C (J 2)-curve exhibits a fast decay which is well described by a logarithmic term \hbox{$1/\textrm{log}(\frac{2}{3}|J_1|-J_{2})$} 1 / log ( 2 3 | J 1 | − J 2 ) . To characterize the magnetic ordering below and above T C , we calculate the spin-spin correlation functions ⟨ S 0 S R ⟩, the spontaneous magnetization, the uniform static susceptibility χ 0 as well as the correlation length ξ. Moreover, we discuss the specific heat C V and the temperature dependence of the excitation spectrum. As approaching the transition point \hbox{$J_2^c$} J 2 c some unusual features were found, such as negative spin-spin correlations at temperatures above T C even though the ground state is ferromagnetic or an increase of the spin stiffness with growing temperature.

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Müller, P., Richter, J., Hauser, A. et al. Thermodynamics of the frustrated J1-J2 Heisenberg ferromagnet on the body-centered cubic lattice with arbitrary spin. Eur. Phys. J. B 88, 159 (2015). https://doi.org/10.1140/epjb/e2015-60113-7

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