Abstract
75As NMR measurements were performed as a function of temperature and doping in Eu1−x K x Fe2As2 (x = 0.5,0.7) samples. The large Eu2+ moments and their fluctuations are found to dominate the 75As NMR properties. The 75As nuclei close to the Eu2+ moments likely have a very short spin-spin relaxation time (T 2) and are wiped out of our measurement window. The 75As nuclei relatively far from Eu2+ moments are probed in this study. Increasing the Eu content progressively decreases the signal intensity with no signal found for the full-Eu sample (x = 0). The large 75As NMR linewidth arises from an inhomogeneous magnetic environment around them. The spin lattice relaxation rate (1/T 1) for x = 0.5 and 0.7 samples is nearly independent of temperature above 100 K and results from a dipolar coupling to paramagnetic fluctuations of the Eu2+ moments. The behavior of 1/T 1 at lower temperatures has contributions from the antiferromagnetic fluctuations of the Eu2+ moments as also the fluctuations intrinsic to the FeAs planes and from superconductivity.
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Dey, T., Khuntia, P., Mahajan, A.V. et al. 75As NMR local probe study of magnetism in (Eu1−xKx)Fe2As2 . Eur. Phys. J. B 86, 458 (2013). https://doi.org/10.1140/epjb/e2013-40483-6
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DOI: https://doi.org/10.1140/epjb/e2013-40483-6