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Aging of the field-induced asymmetry in a disordered ferroelectric

  • Solid and Condensed State Physics
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Abstract.

The isothermal aging of the asymmetry induced in the disordered dielectric crystal \(\mbox{KTa}_{1-x} \mbox{Nb}_{x} \mbox{O}_{3} \) (x=0.027) submitted to the biasing electric field E, is investigated. To this end, the response of the complex dielectric constant to infinitesimal field changes \(\delta{\bf E}\), applied to the sample after a variable aging delay, has been measured for different magnitudes of E and after different aging delays. Two different experimental procedures have been used: in both cases the response strongly depends on the time spent under field. For short aging delays, the response has a strong contribution proportional to δE and a weak quadratic contribution proportional to \(\left({\delta E}\right)^2\). As time elapses, the linear and the quadratic contributions age in opposite ways: the former decreases whereas the latter increases. This paradoxical behaviour is analyzed in the framework of a model which attributes aging and the related effects (rejuvenation, memory) to the evolution of polarization domain walls: the decrease of the linear contribution is related to the decrease of the total wall area, while the increase of the quadratic term is attributed to wall reconformations.

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Bonello, B., Doussineau, P., Dupuis, V. et al. Aging of the field-induced asymmetry in a disordered ferroelectric. Eur. Phys. J. B 52, 219–225 (2006). https://doi.org/10.1140/epjb/e2006-00279-5

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  • DOI: https://doi.org/10.1140/epjb/e2006-00279-5

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