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Proton induced reactions on 114Sn and 120Sn targets at energies up to 18 MeV

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Abstract

We measure cross sections of proton-induced reactions on tin up to energies of 18 MeV using the stacked-foil activation technique, and report first experimental values for 114Sn(p,α)111In, 120Sn(p,α)117gIn, and 114Sn(p,x)113Sn reactions. Measured cross sections have been compared to existing experimental values and numerical calculations based on Talys1.95. Our data are in good agreement with all previous experiments, and also with Talys1.95 results except for 120Sn(p,α)117m,gIn reactions where the numerical calculations are shifted to higher energies. We also measure isomeric cross section ratios for 117m,gIn and 120m,gSb pairs as functions of the incident proton energy.

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Data Availability Statement

This manuscript has no associated data or the data will not be deposited. [Authors’ comment: The data obtained in this study are contained in the publication].

References

  1. S.M. Qaim, Radiochemical determination of nuclear data for theory and applications. J. Radioanal. Nucl. Chem. 284, 489–505 (2010). https://doi.org/10.1007/s10967-010-0460-5

    Article  Google Scholar 

  2. E. Gadioli, P.E. Hodgson, Nucleon-alpha reactions in nuclei. Rep. Prog. Phys. 52, 247–299 (1989). https://doi.org/10.1088/0034-4885/52/3/001

    Article  ADS  Google Scholar 

  3. S.M. Qaim, M. Uhl, F. Rosch, F. Szelecseny, Excitation functions of (p, α) reactions on 64 Ni, 78Kr, and 86Sr. Phys. Rev. C 52(2), 733–739 (1995). https://doi.org/10.1103/physrevc.52.733

    Article  ADS  Google Scholar 

  4. A. Hermanne, F. Tarkanyi, F. Ditroi, S. Takacs, R.A. Rebeles, M.S. Uddin, M. Hagiwara, M. Baba, Y. Shubin, S.F. Kovalev, Experimental study of the excitation functions of proton induced reactions on natSn up to 65 MeV. Nucl. Instrum. Methods Phys. Res. Sect. B 247, 180–191 (2006). https://doi.org/10.1016/j.nimb.2006.02.005

    Article  ADS  Google Scholar 

  5. M.U. Khandaker, K. Kim, K.-S. Kim, M. Lee, Y.S. Lee, G. Kim, Y.-S. Cho, Y.-O. Lee, Excitation functions of the proton-induced nuclear reactions on natSn up to 40 MeV. Nucl. Instrum. Methods Phys. Res. Sect. B 267, 23–31 (2009). https://doi.org/10.1016/j.nimb.2008.11.017

    Article  ADS  Google Scholar 

  6. S.M. Kormali, D.L. Swindle, E.A. Schweikert, Charged particle activation of medium Z elements. J. Radioanal. Chem. 31, 437–450 (1976). https://doi.org/10.1007/BF02518508

    Article  Google Scholar 

  7. E.A. Skakun, V.G. Batiy, Yu.N. Raklvnenko, O.A. Rastrepin, Cross sections of (p, gamma) reactions on isotopes 54Fe,112Sn and 114Cd at proton energies up to 9 MeV. Sov. J. Nucl. Phys. 45, 384 (1987)

    Google Scholar 

  8. V.G. Batij, E.A. Skakun, (p,n) reaction cross sections on 115,116,120-Sn isotopes. In 9 International Symposium Nuclei in the Cosmos, CERN, vol. 204 (2006)

  9. E.A. Skakun, V.G. Batij, Level density parameters from excitation cross sections of isomeric state. Zeitschrift fuer Physik A Hadrons Nuclei 344, 13 (1992). https://doi.org/10.1007/BF01291012

    Article  ADS  Google Scholar 

  10. V.G. Batij, E.A. Skakun, Cross sections of (p,n) reaction on 117-, 118-, 122-, 124-Sn. In Conference on Nuclear Data for Science and Technology, vol. 2 (2007), p. 1325

  11. G.N. Lovchikova, O.A. Salnikov, S.P. Simakov, A.M. Trufanov, G.V. Kotelnikova, V. Pilz, T. Streil, Study of mechanism of the reactions 94-Zr(p, n)94-Nb, 119-Sn(p, n)119-Sb and 122-Sn(p, n)122-Sb in the proton energy region 6–9 MeV. Sov. J. Nucl. Phys. 31, 1 (1980)

    Google Scholar 

  12. C.H. Johnson, J.K. Bair, C.M. Jones, S.K. Penny, D.W. Smith, p-Wave size resonances observed by the (p, n) reaction for 2.6- to 7-MeV protons incident on isotopes of Sn. Phys. Rev. C 15, 196 (1977). https://doi.org/10.1103/PhysRevC.15.196

    Article  ADS  Google Scholar 

  13. A.P. Klyucharev, E.A. Skakun, Y.N. Rakivnenko, I.A. Romanii, Excitation functions of (p, n) reactions on some Sn isotopes and the isomeric cross section ratios. Sov. J. Nucl. Phys. 11, 530 (1970)

    Google Scholar 

  14. Bull. Russ. Acad. Sci. Phys. 75, 1274 (2011)https://doi.org/10.3103/S1062873811070380

  15. E.A. Skakun, A. Iordakesku, V.A. Lutsik, Ju.N. Rakivnenko, I.A. Romanij, Excitation functions and isomeric ratios for 122-Sn(p,n)122m,g-Sb and 124-Sn(p,n)124m2,m1-Sb reactions. In Conference: 29. Conference on Nuclear Spectroscopy and Nuclear Structure, Riga 1979 (1979). p. 291

  16. V.G. Batij, E.A. Skakun, Yu.N. Rakivnenko, O.A. Rastrepin, Study of the spin dependence of the level density for nuclei near the closed proton shell with Z=50. Yad. Fiz. 47, 978 (1988)

    Google Scholar 

  17. J.-P. Blaser, F. Boehm, P. Marmier, D.C. Peaslee, Fonctions d’excitation de la reaction (p, n). J. Helvetica Physica Acta 24, 3 (1951)

    Google Scholar 

  18. J.L. Need, B. Linder, Cross sections for formation of the isomeric pair In117 and In117m in the Sn120(p, alpha) reaction. Phys. Rev. 129, 1298 (1963). https://doi.org/10.1103/PhysRev.129.1298

    Article  ADS  Google Scholar 

  19. F.R. Chloupek, ASt.J. Murphy, R.N. Boyd, A.L. Cole, J. Goerres, R.T. Guray, G. Raimann, J.J. Zach, T. Rauscher, J.V. Schwarzenberg, P. Tischhauser, M.C. Wiescher, Measurements of proton radiative capture cross sections relevant to the astrophysical rp- and gamma-processes. Nucl. Phys. Sect. A 652, 391 (1999). https://doi.org/10.1016/S0375-9474(99)00167-0

    Article  ADS  Google Scholar 

  20. C.H. Johnson, R.L. Kernell, (p, n) cross sections and the strength functions for 3- to 5.5-MeV protons on In and on Sn isotopes. J. Phys. Rev. Part C Nucl. Phys. 2, 639 (1970). https://doi.org/10.1103/PhysRevC.2.639

    Article  ADS  Google Scholar 

  21. N. Ozkan, ASt.J. Murphy, R.N. Boyd, A.L. Cole, M. Famiano, R.T. Guray, M. Howard, L. Sahin, J.J. Zach, R. de Haan, J. Goerres, M. Wiescher, M.S. Islam, T. Raucher, Cross section measurements of the 102Pd(p, gamma)103Ag, 116Sn(p, gamma)117Sn, and 112Sn(alpha, gamma)116Te reactions relevant to the astrophysical rp- and gamma-processes. Nucl. Phys. Sect. A 710, 469 (2002). https://doi.org/10.1016/S0375-9474(01)00755-2

    Article  ADS  Google Scholar 

  22. M.A. Famiano, R.S. Kodikara, B.M. Giacherio, V.G. Subramanian, A. Kayani, Measurement of the (p, alpha) cross sections of 46Ti, 64Zn, 114Sn, and 116Sn at astrophysically relevant energies. Nuclear Physics, Section A 802, 26 (2008). https://doi.org/10.1016/j.nuclphysa.2008.01.013

    Article  ADS  Google Scholar 

  23. R.L. Bramblett, T.W. Bonner, Neutron evaporation spectra from (p, n) reactions. Nucl. Phys. 20, 395 (1960). https://doi.org/10.1016/0029-5582(60)90182-6

    Article  Google Scholar 

  24. E.K. Elmaghraby, S.A. Said, F.I. Asfour, Investigation of the proton induced reactions on tin at low energies. Appl. Rad. Isotopes 67, 147–151 (2009). https://doi.org/10.1016/j.apradiso.2008.07.017

    Article  Google Scholar 

  25. N. Miyazawa, M. Uesugi, A. Yokoyama, Preparation of a carrier free 124Sb tracer produced in the Sn (p, n) reaction. Radiochim. Acta 109, 453–458 (2021). https://doi.org/10.1515/ract-2020-0105

    Article  Google Scholar 

  26. E. Betak, E. Rurarz, S. Mikolajewski, J. Wojtkowska, A new method of pure 111In production by proton-induced nuclear reactions with enriched 112Sn. Nicleonika 52(1), 17–27 (2007)

    Google Scholar 

  27. H. Thisgaard, M. Jensen, Production of the Auger emitter Sb-119 for targeted radionuclide therapy using a small PET-cyclotron. Appl. Radiat. Isotopes 67, 34 (2009)

    Article  Google Scholar 

  28. http://www.nndc.bnl.gov/qcalc/

  29. J. Blachot, Nuclear data sheets for A=111. Nucl. Data Sheets 110, 1239 (2009). https://doi.org/10.1016/j.nds.2009.04.002

    Article  ADS  Google Scholar 

  30. J. Blachot, Nuclear data sheets for A=113. Nucl. Data Sheets 111, 1471 (2010). https://doi.org/10.1016/j.nds.2010.05.001

    Article  ADS  Google Scholar 

  31. K. Kitao, Y. Tendow, A. Hashizume, Nuclear data sheets for A=120. Nucl. Data Sheets 96, 241 (2002). https://doi.org/10.1006/ndsh.2002.0012

    Article  ADS  Google Scholar 

  32. G.H. Hovhannisyan, T.M. Bakhshiyan, R.K. Dallakyan, Photonuclear production of the medical isotope 67Cu. Nucl. Inst. Methods Phys. Res. B 498, 48–51 (2021). https://doi.org/10.1016/j.nimb.2021.04.016

    Article  ADS  Google Scholar 

  33. G.H. Hovhannisyan, T.M. Bakhshiyan, A.R. Balabekyan, I.A. Kerobyan, Production of 47Sc in photonuclear reactions on natTi targets at the bremsstrahlung endpoint energy of 30 and 40 MeV. Appl. Radiat. Isot. 182, 110138 (2021). https://doi.org/10.1016/j.apradiso.2022.110138

    Article  Google Scholar 

  34. A.S. Danagulyan, G.H. Hovhannisyan, T.M. Bakhshiyan, R.H. Avagyan, A.E. Avetisyan, I.A. Kerobyan, R.K. Dallakyan, Photonuclear Reactions on 112,118,124Sn, natTe, and natHf Targets. Phys. At. Nucl. 77(11), 1313–1320 (2014). https://doi.org/10.1134/S1063778814100056

    Article  Google Scholar 

  35. K.P.Nesteruk, L. Ramseyer, T.S. Carzaniga, S. Braccini, Measurement of the beam energy distribution of a medical cyclotron with a multi-leaf Faraday cup instruments 3, 4 (2019). https://doi.org/10.3390/instruments3010004

  36. H. Piel, S.M. Qaim, G. Stöcklin, Excitation functions of (p, xn) reactions on natNi and highly enriched 62Ni-possibility of production of medically important radioisotope 62Cu at a small cyclotron. Radiochem. Acta (1992). https://doi.org/10.1524/ract.1992.57.1.1

    Article  Google Scholar 

  37. A. Hermanne et al., Monitor reactions. Nucl. Data Sheets 148, 338–382 (2018)

    Article  ADS  Google Scholar 

  38. J.F. Ziegler, SRIM-2003. Nucl. Instrum. Methods B 219–220, 1027–1036 (2004). https://doi.org/10.1016/j.nimb.2004.01.208

    Article  ADS  Google Scholar 

  39. A. Koning, S. Hilaire, S. Goriely, TALYS 1.95. A nuclear reaction program (2019). https://www-nds.iaea.org/talys/tutorials/talys_v1.96.pdf

  40. A.S. Danagulyan, G.H. Hovhannisyan, T.M. Bakhshiyan, I.A. Kerobyan, Analysis of isomeric ratios for medium-mass nuclei. Phys. At. Nucl. 79(5), 679–685 (2016). https://doi.org/10.1134/S1063778816050070

    Article  Google Scholar 

  41. A.S. Danagulyan, G.H. Hovhannisyan, T.M. Bakhshiyan, G.V. Martirosyan, Special features of isomeric ratios in nuclear reactions induced by various projectile particles. Phys. At. Nucl. 79(3), 326–334 (2016). https://doi.org/10.1134/S1063778816020058

    Article  Google Scholar 

  42. G.S. Karapetyan, Fission and spallation data evaluation using induced-activity method. Eur. Phys. J. Plus 130, 180 (2015). https://doi.org/10.1140/epjp/i2015-15180-7

    Article  Google Scholar 

  43. D. Kolev, J. Ernst, The role of angular-momentum removal in photonuclear reactions as deduced from the isomeric ratios for 120m, gSb and 117m, gIn. J. Phys. G Nucl. Part. Phys. 24, 589–599 (1998). https://doi.org/10.1088/0954-3899/24/3/010

    Article  ADS  Google Scholar 

  44. S. Sudár, S.M. Qaim, Isomeric cross-section ratio for the formation of 58Com, g in neutron, proton, deuteron, and alpha-particle induced reactions in the energy region up to 25 MeV. Phys. Rev. C. 53, 2885–2892 (1996). https://doi.org/10.1103/physrevc.53.2885

    Article  ADS  Google Scholar 

  45. M.S. Uddin, M.S. Basunia, S. Sudár et al., Excitation functions of proton-induced nuclear reactions on 86Sr, with particular emphasis on the formation of isomeric states in 86Y and 85Y. Eur. Phys. J. A 58, 67 (2022). https://doi.org/10.1140/epja/s10050-022-00714-w

    Article  ADS  Google Scholar 

  46. S. Sudár, S.M. Qaim, Mass number and excitation energy dependence of the Θeff/Θrig parameter of the spin cut-off factor in the formation of an isomeric pair. Nucl. Phys. A 979, 113–142 (2018). https://doi.org/10.1016/j.nuclphysa.2018.09.039

    Article  ADS  Google Scholar 

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Acknowledgements

The authors are thankful to the staff of Cyclotron18/18 of the Radioisotope Production Center, Yerevan, for the operation of the accelerator, and assistance in transporting the irradiated targets.

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Correspondence to G. H. Hovhannisyan.

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Communicated by Alessia Di Pietro.

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Hovhannisyan, G.H., Bakhshiyan, T.M., Martirosyan, G.V. et al. Proton induced reactions on 114Sn and 120Sn targets at energies up to 18 MeV. Eur. Phys. J. A 59, 161 (2023). https://doi.org/10.1140/epja/s10050-023-01071-y

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