Excitation functions and thick target yields of the \(^{\mathrm {nat}}\hbox {Zr}(\hbox {p},\hbox {x})^{{95}}\hbox {Zr}\), \(^{95\mathrm {m}}\hbox {Nb}\), \(^{95\mathrm {g}}\hbox {Nb}\) reactions

Abstract

We measured the excitation functions for the production of the radionuclides \(^{{95}}\hbox {Zr}\), \(^{95\mathrm {m}}\hbox {Nb}\) and \(^{95\mathrm {g}}\hbox {Nb}\) from the \(^{\mathrm {nat}}\hbox {Zr}(\hbox {p},\hbox {x})\) reactions in the proton energy range of 10.6–43.6 MeV. The experiment was performed by irradiation of zirconium and copper foils simultaneously using 45 MeV proton beam from the MC-50 Cyclotron at the Korea Institute of Radiological and Medical Sciences, Korea, and the induced activity was measured with an HPGe \(\upgamma \)-ray detector. Proton energies along the foil stack were calculated using the computer code SRIM-2013. The proton beam flux entered each foil was determined via the \(^{\mathrm {nat}}\hbox {Cu}(\hbox {p},\hbox {x})^{{62}}\hbox {Zn}\) and \(^{\mathrm {nat}}\hbox {Cu}(\hbox {p},\hbox {x})^{{65}}\hbox {Zn}\) monitoring reactions. The cumulative cross sections of the \(^{\mathrm {nat}}\hbox {Zr}(\hbox {p},\hbox {x})^{{95}}\hbox {Zr}\) reaction were measured because it was unable to separate the activity from the decay of \(^{{95}}\hbox {Y}\) to \(^{{95}}\hbox {Zr}\). However, independent cross sections of the \(^{\mathrm {nat}}\hbox {Zr}(\hbox {p},\hbox {x})^{95\mathrm {m}}\hbox {Nb}\) and \(^{\mathrm {nat}}\hbox {Zr}(\hbox {p},\hbox {x})^{95\mathrm {g}}\hbox {Nb}\) reactions were determined, since the independent activities of \(^{95\mathrm {m}}\hbox {Nb}\) and \(^{95\mathrm {g}}\hbox {Nb}\) can also be measured. In addition, the thick target yields of the \(^{{95}}\hbox {Zr}\), \(^{95\mathrm {m}}\hbox {Nb}\) and \(^{95\mathrm {g}}\hbox {Nb}\) isotopes were also determined. The current results are compared with the previously measured data as well as with the theoretical values from the TALYS-1.9 code and the TENDL-2019 data library.

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Data Availability Statement

This manuscript has associated data in a data repository. [Authors’ comment: All data used in this paper are deposited in the EXFOR data library and TENDL-2019 data library, and the data produced during this study will be deposited in the EXFOR data library.]

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Acknowledgements

The authors express their sincere thanks to the staff of the MC-50 Cyclotron Laboratory in the Korea Institute of Radiological and Medical Sciences (KIRAMS), Korea for the excellent operation and their support during the experiment. This research was partly supported by the National Research Foundation of Korea through a Grant provided by the Ministry of Science and ICT (NRF-2017R1D1A1B03030484, NRF2013M7A1A1075764, and NRF-2018R1A6A1A06024970) and by the Vietnam National Foundation for Science and Technology Development (NAFOSTED) under Grant No. 103.04-2018.314.

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Nguyen, V.D., Nguyen, T.L., Nguyen, T.H. et al. Excitation functions and thick target yields of the \(^{\mathrm {nat}}\hbox {Zr}(\hbox {p},\hbox {x})^{{95}}\hbox {Zr}\), \(^{95\mathrm {m}}\hbox {Nb}\), \(^{95\mathrm {g}}\hbox {Nb}\) reactions. Eur. Phys. J. A 56, 194 (2020). https://doi.org/10.1140/epja/s10050-020-00199-5

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