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A comparative Raman study of 0.65(PbMg1/3Nb2/3O3) -0.35(PbTiO3) single crystal and thin film

  • H. Bouyanfif
  • M. El Marssi
  • N. Lemée
  • F. Le Marrec
  • M. G. Karkut
  • B. Dkhil
  • Yu. I. Yuzyuk
Regular Article

Abstract

We report a comparative Raman study of 0.65(PbMg1/3Nb2/3O3)-0.35(PbTiO3) (PMN-0.35PT) single crystal and thin film. Raman spectra investigation indicates a change in bulk from the high temperature cubic to the tetragonal phase and then to the low temperature Mc monoclinic phase. The transition temperatures are in good agreement with the ones previously observed by dielectric measurements on the same sample. In contrast, we observe no phase transition to the monoclinic phase in the PMN-0.35PT 4000 Å thick film and only a cubic to tetragonal diffuse transition has been determined at high temperature. The enhanced stability of the tetragonal phase and the absence of low temperature monoclinic phase have been attributed to the in plane strain.

Keywords

Solid State and Materials 

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Copyright information

© EDP Sciences, SIF, Springer-Verlag Berlin Heidelberg 2012

Authors and Affiliations

  • H. Bouyanfif
    • 1
  • M. El Marssi
    • 1
  • N. Lemée
    • 1
  • F. Le Marrec
    • 1
  • M. G. Karkut
    • 1
  • B. Dkhil
    • 2
  • Yu. I. Yuzyuk
    • 3
  1. 1.Laboratoire de Physique de la Matière CondenséeUniversité de Picardie Jules VerneAmiensFrance
  2. 2.Laboratoire SPMSEcole Centrale ParisChatenay Malabry CedexFrance
  3. 3.Faculty of PhysicsSouthern Federal UniversityRostov-on-DonRussia

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