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A study of reaction rates of (n, f ) , (n,\( \gamma\)) and (n, 2n) reactions in natU and 232Th by the neutron fluence produced in the graphite set-up (GAMMA-3) irradiated by 2.33 GeV deuteron beam

  • J. Adam
  • Chitra Bhatia
  • K. Katovsky
  • V. KumarEmail author
  • M. Majerle
  • V. S. Pronskikh
  • A. M. Khilmanovich
  • B. A. Martsynkevich
  • I. V. Zhuk
  • V. M. Golovatiouk
  • W. Westmeier
  • A. A. Solnyshkin
  • V. M. Tsoupko-Sitnikov
  • A. S. Potapenko
Regular Article - Experimental Physics

Abstract

Spallation neutrons produced in the collision of a 2.33GeV deuteron beam with a large lead target are moderated by a thick graphite block surrounding the target and used to activate the radioactive samples of natU and Th put at three different positions, identified as holes “a”, “b” and “c” in the graphite block. Rates of the (n, f), (n, \( \gamma\) and (n, 2n) reactions in the two samples are determined using the gamma spectrometry. The ratios of the experimental reaction rates, R (n, 2n)/R (n, f), for 232Th and natU are estimated in order to understand the role of the (n, x n) kind of reactions in Accelerator-Driven Sub-critical Systems. For the Th-sample, the ratio is ∼ 54 (10)% in the case of hole “a” and ∼ 95 (57)% in the case of hole “b” compared to 1.73(20)% for hole “a” and 0.710(9)% for hole “b” in the case of the natU sample. Also the ratio of fission rates in uranium to thorium, natU (n, f)/ 232Th (n, f), is ∼ 11.2 (17) in the case of hole “a” and 26.8(85) in hole “b”. Similarly, the ratio 238U (n, 2n)/ 232Th (n, 2n) is 0.36(4) for hole “a” and 0.20(10) for hole “b” showing that 232Th is more prone to the (n, x n) reaction than 238U . All the experimental reaction rates are compared with the simulated ones by generating neutron fluxes at the three holes from MCNPX 2.6c and making use of the LA150 library of cross-sections. The experimental and calculated reaction rates of all the three reactions are in reasonably good agreement. The transmutation power, P norm as well as P norm/P beam of the set-up is estimated using the reaction rates of the (n, \( \gamma\) and (n, 2n) reactions for both the samples in the three holes and compared with some of the results of the “Energy plus Transmutation” set-up and TARC experiment.

Keywords

Neutron Energy 133Xe Cumulative Yield Lead Target 232Th Sample 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

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Copyright information

© SIF, Springer-Verlag Berlin Heidelberg 2011

Authors and Affiliations

  • J. Adam
    • 1
    • 2
  • Chitra Bhatia
    • 3
  • K. Katovsky
    • 1
  • V. Kumar
    • 3
    • 7
    Email author
  • M. Majerle
    • 2
  • V. S. Pronskikh
    • 1
  • A. M. Khilmanovich
    • 4
  • B. A. Martsynkevich
    • 4
  • I. V. Zhuk
    • 5
  • V. M. Golovatiouk
    • 1
  • W. Westmeier
    • 5
  • A. A. Solnyshkin
    • 1
  • V. M. Tsoupko-Sitnikov
    • 1
  • A. S. Potapenko
    • 6
  1. 1.Joint Institute for Nuclear ResearchDubna (Moscow Region)Russian Federation
  2. 2.Czech Academy of ScienceNuclear Physics InstituteŘežCzech Republic
  3. 3.HENP Laboratory (ADS Program), Physics DepartmentUniversity of RajasthanJaipurIndia
  4. 4.Institute of Physics of National Academy of SciencesMinskBelarus
  5. 5.Kernchemie InstitutePhilips-UniversitätMarburgGermany
  6. 6.Joint Institute of Power and Nuclear ResearchSosny, MinskBelarus
  7. 7.University School of Basic and Applied SciencesGGS IPUniversityNew DelhiIndia

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