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Deoxygenation of CO2 Absorbent Based on Monoethanolamine in Gas–Liquid Membrane Contactors Using Composite Membranes

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Abstract

This work is devoted to the removal of dissolved oxygen from a model absorbent based on monoethanolamine (MEA) to prevent its oxidative degradation during the absorption purification of flue gases from carbon dioxide. Composite membranes based on porous ceramic and polymeric supports with a thin selective layer of poly[1-(trimethylsilyl)-1-propyne] or its blend with polyvinyltrimethylsilane are developed, and gas-liquid membrane contactors are created on their basis. It is shown that the use of these contractors in the vacuum mode allows the removal of up to 60% of dissolved oxygen from the model sorbent.

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ACKNOWLEDGMENTS

We are grateful to P.A. Safronov for his help in manufacturing membrane contractors and D.S. Bakhtin for recording SEM images.

This work was carried out using the equipment of the Shared Research Center Analytical Center of Deep Oil Processing and Petrochemistry, Topchiev Institute of Petrochemical Synthesis, Russian Academy of Sciences.

Funding

This work was performed at the Topchiev Institute of Petrochemical Synthesis, Russian Academy of Sciences and supported by the Russian Science Foundation within the framework of project no. 21-79-10400. D.K., S.Sh., T.A., and S.B. are grateful to the Foundation for financial support.

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Authors and Affiliations

  1. Topchiev Institute of Petrochemical Synthesis, Russian Academy of Sciences, 119991, Moscow, Russia

    D. O. Kalmykov, S. A. Shirokikh, D. N. Matveev, T. S. Anokhina & S. D. Bazhenov

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  1. D. O. Kalmykov
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  2. S. A. Shirokikh
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  3. D. N. Matveev
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  4. T. S. Anokhina
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  5. S. D. Bazhenov
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Correspondence to D. O. Kalmykov.

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Translated by T. Soboleva

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Kalmykov, D.O., Shirokikh, S.A., Matveev, D.N. et al. Deoxygenation of CO2 Absorbent Based on Monoethanolamine in Gas–Liquid Membrane Contactors Using Composite Membranes. Membr. Membr. Technol. 5, 333–343 (2023). https://doi.org/10.1134/S2517751623050049

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  • DOI: https://doi.org/10.1134/S2517751623050049

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