Skip to main content
Log in

Tritium Distribution in Soil in the Area of “Atomic” Lake near the Semipalatinsk Test Site

  • SOIL PHYSICS
  • Published:
Eurasian Soil Science Aims and scope Submit manuscript

Abstract

Data on concentrations and distribution of tritium in soils of the “Atomic” Lake excavation explosion area of Semipalatinsk Nuclear Test Site (Kazakhstan, East Kazakhstan oblast) are discussed. The concentrations of tritium in surface soil horizons and in soil profiles have been determined in the bulk soil samples and in different particle-size fractions. Tritium concentration in soils reaches 240 000 Bq/kg. A correlation has been found between tritium and europium concentrations in soils. Presumably, tritium formation is controlled by two mechanisms. One of them is the neutron activation process, i.e., nuclear reactions with lithium, boron, and nitrogen isotopes present in the soil; the other mechanism is related to the capture of tritium that was initially in the charge of mineral particles formed upon condensation from the red-hot explosion zone.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1.
Fig. 2.
Fig. 3.
Fig. 4.

Similar content being viewed by others

REFERENCES

  1. MI 2143-91. State System for Ensuring Uniformity of Measurements. Activity of Radionuclides in Large Samples. Measurement on Gamma-Spectrometer: Recommendations (Almaty, 1998) [in Russian].

  2. V. A. Baturin, Tritium is Dangerous: Popular about Complicate Things (Chelyabinsk, 2001), p. 22.

  3. T. Yu. Bogatyreva and A. K. Aidarkhanova, “Leaching of human-made radionuclides from soil at the Semipalaltinsk test site as one of the main contamination mechanisms of natural water,” Vestn. Nats. Yad. Tsentra, Resp. Kazakh., No. 4, 160–164 (2018).

  4. A. F. Vadyunina and Z. A. Korchagina, Practical Manual for Analysis of Physical Properties of Soils (Agropromizdat, Moscow, 1986) [in Russian].

    Google Scholar 

  5. A. E. Kunduzbaeva, A. M. Kabdyrakova, N. V. Larionova, et al., “Speciation of artificial radionuclides in soils of “Atomic” Lake of the Semipalatinsk Test Site,” Aktual. Vopr. Radioekol. Kazakh. 1 (6), 288 (2017.

    Google Scholar 

  6. I. I. Linge and I. I. Kryshev, Radioecological Situation in the Regions of Rosatom Enterprises (SAM Poligrafist, Moscow, 2015), p. 13.

    Google Scholar 

  7. V. A. Logachev, Nuclear Tests in the USSR: Current Radioecological Status of Landfills (AT, Moscow, 2002), pp. 93–94.

  8. O. N. Lyakhova, S. N. Lukashenko, N. V. Larionova, et al., “Tritium as an indicator of nuclear tests,” Aktual. Vopr. Radioekol. Kazakh. 2 (3), 123 (2011).

    Google Scholar 

  9. V. A. Naumov and S. G. Klimin, “Tritium in radioecological safety of the Kola region,” Vestn. Mosk. Gos. Tekh. Univ. 1 (3), 145 (1998).

    Google Scholar 

  10. Organization of Monitoring of Underground Waters of Former Semipalatinsk Test Site: A Final Report on the MNTTS K-893 Project (Institute of Radiation Safety and Ecology, Kurchatov, 2005) [in Russian].

  11. A Report on Scientific Research by the Institute of Radiation Safety and Ecology, National Nuclear Center of Kazakhstan Performed within the Project “Analysis of Modern Status and Impact of the Nuclear Power Objects at the Semipalatinsk Test Site on the Environment” (Institute of Radiation Safety and Ecology, Kurchatov, 2009) [in Russian].

  12. A. V. Pushkarev, V. V. Dolin, V. M. Priimachenko, V. N. Bobkov, and R. A. Pushkareva, Kinetics of Isotope-Hydrogen Exchange in Bentonite-Sand Mixture (Institute of Environment Geochemistry, Kyiv, 2007), No. 15, pp. 27–36.

  13. Radiation Situation in Russia and Adjacent Countries in 2011: Yearbook, Ed. by S. M. Vakulovskii (Obninsk, 2012) [in Russian].

    Google Scholar 

  14. L. V. Timonova, O. N. Lyakhova, S. N. Lukashenko, and A. O. Aidarkhanov, “The content of tritium in soil in the nuclear testing areas of Semipalatinsk Test Site,” Radiats. Biol., Radioekol. 55, 667–672 (2015). https://doi.org/10.7868/S0869803115050136

    Article  Google Scholar 

  15. Chelovek. Energiya. Atom., No. 4 (6), 67 (2009).

  16. N. Baglan, S. B. Kim, C. Cossonnet, I. V. Croudace, M. Fournier, D. Galeriu, P. E. Warwick, N. Momoshima, and E. Ansoborlo, “Organically bound tritium (OBT) behavior and analysis: outcomes of the seminar held in Balaruc-les-Bains in May 2012,” Radioprot. EDP Sci. 48, 127–144 (2013).

    Article  Google Scholar 

  17. Environmental Fate of Tritium in Soil and Vegetation. Part of the Tritium Studies Project (Canadian Nuclear Safety Commission, 2013).

  18. ISO 9698:2019: Water Quality—Tritium—Test Method Using Liquid Scintillation Counting (International Organization for Standardization, Geneva, 2019).

  19. IUSS Working Group WRB, World Reference Base for Soil Resources, International Soil Classification System for Naming Soils and Creating Legends for Soil Maps, World Soil Resources Report No. 106 (UN Food and Agriculture Organization, Rome, 2014).

  20. D. J. Kim, PhD Thesis (University of Southampton, Southampton, 2009).

  21. A. Lopez-Galindo, P. Fenoll Hach-Alip, and A. V. Pushkarev, “Tritium redistribution between water and clay minerals,” Appl. Clay Sci. 39, 151–159 (2008).

    Article  Google Scholar 

  22. Z. B. Serzhanova, A. K. Aidarkhanova, S. N. Lukashenko, O. N. Lyakhova, L. V. Timonova, and A. M. Raimkanova, “Researching of tritium speciation in soils of “Balapan” site,” J. Environ. Radioact. 192, 621–627 (2018). https://doi.org/10.1016/j.jenvrad.2018.02.016

    Article  Google Scholar 

Download references

Funding

This study was partially supported by the Russian Foundation for Basic Research, project no. 19-0016-00146/9.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to L. V. Timonova.

Ethics declarations

The authors declare that they have no conflict of interest.

Additional information

Translated by O. Eremina

Supplementary material

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Timonova, L.V., Lyakhova, O.N., Lukashenko, S.N. et al. Tritium Distribution in Soil in the Area of “Atomic” Lake near the Semipalatinsk Test Site. Eurasian Soil Sc. 53, 355–361 (2020). https://doi.org/10.1134/S1064229320030096

Download citation

  • Received:

  • Revised:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1134/S1064229320030096

Keywords:

Navigation