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Nonlinear Optical Diagnostics of Thin Polycrystalline Lead Zirconate Titanate Films

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Abstract

Nonlinear optical microscopy techniques have been used to study thin films of single-phase (perovskite) and two-phase (perovskite–pyrochlore) lead zirconate titanate (PZT) deposited on Pt/TiO2/SiO2/Si by means of radio-frequency magnetron sputtering at various target–substrate distances (D = 30–70 mm). Results revealed inhomogeneous distribution of second-harmonic generation in spherulitic perovskite islands, including increased signal intensity at perovskite/pyrochlore interface, which may be related to a nonuniform distribution of mechanical stresses. Factors responsible for the observed strong variation in second-harmonic signal are discussed, including the mutual relationship between changes in the character of spherulitic structure and conditions of PZT film deposition depending on the target–substrate distance.

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Funding

This work was supported in part in the framework of a state order (project no. FSFZ-2020-0022) for E.D. Mishina and by the Program of Grants for Young MIREA–RTU Scientists (project no. NICh-43) for A.S. Elshin.

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Authors and Affiliations

  1. MIREA–Russian Technological University, 119454, Moscow, Russia

    A. S. Elshin & E. D. Mishina

  2. Ioffe Institute, Russian Academy of Sciences, 194021, St. Petersburg, Russia

    I. P. Pronin & S. V. Senkevich

Authors
  1. A. S. Elshin
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  2. I. P. Pronin
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  3. S. V. Senkevich
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  4. E. D. Mishina
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Correspondence to A. S. Elshin.

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The authors declare that they have no conflict of interest.

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Translated by P. Pozdeev

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Elshin, A.S., Pronin, I.P., Senkevich, S.V. et al. Nonlinear Optical Diagnostics of Thin Polycrystalline Lead Zirconate Titanate Films. Tech. Phys. Lett. 46, 385–388 (2020). https://doi.org/10.1134/S1063785020040215

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  • DOI: https://doi.org/10.1134/S1063785020040215

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