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Anomalous Change in the Size of a Spin Polaron in the Paramagnetic Temperature Range in La1.2Sr1.8Mn2O7

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Abstract

This study continues investigation of the magnetic and electrical properties of double perovskite La1.2Sr1.8Mn2O7, which has a colossal magnetoresistance (above 1200) near the Curie temperature. It is shown that the colossal magnetoresistance observed in La1.2Sr1.8Mn2O7 is adequately described based on the “orientational” and “spin-polaron” conduction mechanisms. It is found that, in the absence of a magnetic field, the linear size of a spin polaron decreases with an increase in temperature in the ferromagnetic region, whereas during the transition of manganite to the paramagnetic state the linear size begins to increase, with a maximum at 180 K. At temperatures above 180 K, the anomalous temperature change in the size of a spin polaron disappears. In the absence of a magnetic field, the detected peak in the temperature dependence of the spin-polaron size is maximum; the peak height decreases after applying a magnetic field. Mechanisms are proposed to explain this anomalous temperature behavior of the spin-polaron size.

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ACKNOWLEDGMENTS

I am grateful to K.I. Kugel’ and N.I. Solin for helpful discussions of the results and valuable remarks.

Funding

This study was performed within the state contract “Kvant” with the Ministry of Science and Higher Education of the Russian Federation (no. AAAA-A18-118020190095) and supported in part by the Russian Foundation for Basic Research (project no. 19-02-01000).

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Correspondence to S. A. Gudin.

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Translated by A. Sin’kov

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Gudin, S.A. Anomalous Change in the Size of a Spin Polaron in the Paramagnetic Temperature Range in La1.2Sr1.8Mn2O7. Phys. Solid State 64, 6–10 (2022). https://doi.org/10.1134/S1063783422010085

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  • DOI: https://doi.org/10.1134/S1063783422010085

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