Abstract
We study the modification of the exciton absorption in cuprous oxide by the presence of free carriers excited through above band gap excitation. Without this pumping, the absorption spectrum below the band gap consists of the yellow exciton series with principal quantum numbers up to more than n = 20, depending on the temperature, changing over to an about constant, only slowly varying absorption above the gap. Careful injection of free carriers, starting from densities well below 1 μm–3, leads to a reduction of the band gap through correlation effects. The excitons in the Rydberg regime above n = 10 remain unaffected until the band gap approaches them. Then they lose oscillator strength and ultimately vanish upon crossing with the band gap.
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References
C. F. Klingshirn, Semiconductor Optics (Springer, Berlin, 2012).
N. F. Mott, Rev. Mod. Phys. 40, 677 (1968); G. B. Norris and K. K. Bajaj, Phys. Rev. B 26, 6706 (1982).
M. Capizzi, S. Modesti, A. Frova, J. L. Staehli, M. Guzzi, and R. A. Logan, Phys. Rev. B 29, 2028 (1984); J. Collet, J. Phys. Chem. Solids 46, 417 (1985).
D. Semkat, F. Richter, D. Kremp, G. Manzke, W.-D. Kraeft, and K. Henneberger, Phys. Rev. B 80, 155201 (2009).
J. Brandt, D. Fröhlich, C. Sandfort, M. Bayer, H. Stolz, and N. Naka, Phys. Rev. Lett. 99, 217403 (2007).
E. F. Gross and N. A. Karrjew, Dokl. Akad. Nauk SSSR 84, 471 (1952).
E. F. Gross, Nuovo Cimento 4, 672 (1956).
F. Schöne, S.-O. Krüger, P. Grünwald, H. Stolz, S. Scheel, M. Aßmann, J. Heckötter, J. Thewes, D. Fröhlich, and M. Bayer, Phys. Rev. B 93, 075203 (2016).
M. Aßmann, J. Thewes, D. Fröhlich, and M. Bayer, Nat. Mater. 15, 741 (2016).
Ch. Uihlein, D. Fröhlich, and R. Kenklies, Phys. Rev. B 23, 2731 (1981).
R. J. Elliott, Phys. Rev. 108, 1384 (1957).
T. Itoh and S. Narita, J. Phys. Soc. Jpn. 39, 140 (1975).
S. John, C. Soukoulis, M. H. Cohen, and E. N. Economou, Phys. Rev. Lett. 57, 1777 (1986).
J. Heckötter, M. Freitag, D. Fröhlich, M. Aßmann, M. Bayer, P. Grünwald, F. Schöne, D. Semkat, H. Stolz, and S. Scheel, arXiv:1709.00891 [condmat. mtrl-sci].
H. Haug and S. Koch, Quantum Theory of the Optical and Electronic Properties of Semiconductors (Word Scientific, Singapore, 1993).
R. Zimmermann, Phys. Status Solidi B 146, 371 (1988); G. Manzke, D. Semkat, F. Richter, D. Kremp, and K. Henneberger, J. Phys.: Conf. Ser. 210, 012020 (2010); R. Zimmermann, K. Kilimann, W. D. Kraeft, D. Kremp, and G. Röpke, Phys. Status Solidi B 90, 175 (1978); G. Manzke, D. Semkat, and H. Stolz, New J. Phys. 14, 095002 (2012).
H. Stolz, R. Schwartz, F. Kieseling, S. Som, M. Kaupsch, S. Sobkowiak, D. Semkat, N. Naka, Th. Koch, and H. Fehske, New J. Phys. 14, 105007 (2012); R. Schwartz, N. Naka, F. Kieseling, and H. Stolz, New J. Phys. 14, 023054 (2012).
D. Kremp, M. Schlanges, and W.-D. Kraeft, Quantum Statistics of Nonideal Plasmas (Springer, Berlin, 2005).
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Heckötter, J., Freitag, M., Aßmann, M. et al. Critical Dependence of the Excitonic Absorption in Cuprous Oxide on Experimental Parameters. Phys. Solid State 60, 1618–1624 (2018). https://doi.org/10.1134/S1063783418080097
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DOI: https://doi.org/10.1134/S1063783418080097