Abstract
Lithium fluoride nanocrystals were irradiated by gamma rays at a temperature below the temperature corresponding to the mobility of anion vacancies. The kinetics of the aggregation of radiation-induced defects in subsurface layers of nanocrystals during annealing after irradiation was elucidated. The processes that could be used to determine the activation energy of the diffusion of anion vacancies were revealed. The value of this energy in subsurface layers was obtained. For subsurface layers, the concentrations ratio of vacancies and defects consisting of one vacancy and two electrons was found. The factors responsible for the differences in the values of the activation energies and concentration ratios in subsurface layers and in the bulk of the crystals were discussed.
Similar content being viewed by others
References
N. Salah, P. D. Sahare, and A. A. Rupasov, J. Lumin. 124, 357 (2007).
N. Salah, Rad. Phys. Chem. 80, 1 (2011).
A. Kovacs, M. Baranyai, W. L. McLaughlin, S. D. Miller, A. Miller, P. G. Fuochi, M. Lavalle, and I. Slezsak, Radiat. Phys. Chem. 57, 691 (2000).
S. Almaviva, M. Marinelli, E. Milani, G. Prestopino, A. Tucciarone, C. Verona-Rinati, M. Angelone, D. Lattanzi, M. Pillon, R. M. Montereali, and M. A. Vincenti, J. Appl. Phys. 103, 054501 (2008).
R. M. Montereali, in Handbook of Thin Film Materials, Ed. by H. S. Nalwa (Academic, New York, 2002), p. 399.
R. Larciprete, I. Gregoratti, M. Danailov, R. M. Montereali, F. Bonfigli, M. Kiskinova, Appl. Phys. Lett. 80, 3862 (2002).
V. Zielasek, T. Hildebrandt, and M. Henzler, Phys. Rev. B: Condens. Matter 62, 2912 (2000).
S. V. Moharil and B. T. Deshmukh, Radiat. Eff. Defects Solids 34, 189 (1977).
A. P. Voitovich, V. S. Kalinov, M. V. Korzhik, E. F. Martynovich, L. P. Runets, and A. P. Stupak, Radiat. Eff. Defects Solids 168, 130 (2013).
A. P. Voitovich, V. S. Kalinov, A. P. Stupak, A. N. Novikov, and L. P. Runets, J. Lumin. 157, 28 (2015).
L. A. Lisitsyna, Sov. Phys. Solid State 34 (9), 1441 (1992).
A. P. Voitovich, V. S. Kalinov, L. P. Runets, A. P. Stupak, E. F. Martynovich, R. M. Montereali, and G. Baldacchini, J. Lumin. 143, 207 (2013).
A. P. Voitovich, V. S. Kalinov, E. F. Martynovich, A. N. Novikov, and A. P. Stupak, Phys. Solid State 54 (9), 1768 (2012).
J. Frenkel, Kinetic Theory of Liquids (Dover, New York, 1955; Nauka, Leningrad, 1975).
B. P. Chandra, N. L. Patel, S. S. Rahangdale, R. P. Patel, and V. K. Patle, Pramana—J. Phys. 60, 109 (2003).
Author information
Authors and Affiliations
Corresponding author
Additional information
Original Russian Text © A.P. Voitovich, V.S. Kalinov, E.F. Martynovich, A.P. Stupak, L.P. Runets, 2015, published in Fizika Tverdogo Tela, 2015, Vol. 57, No. 9, pp. 1709–1714.
Rights and permissions
About this article
Cite this article
Voitovich, A.P., Kalinov, V.S., Martynovich, E.F. et al. Diffusion and aggregation of subsurface radiation defects in lithium fluoride nanocrystals. Phys. Solid State 57, 1752–1758 (2015). https://doi.org/10.1134/S1063783415090334
Received:
Published:
Issue Date:
DOI: https://doi.org/10.1134/S1063783415090334