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Electric Hyperfine Interactions of 57Fe Impurity Atoms in ACrO3 Perovskite-Type Chromites (A = Sc, In, Tl, Bi)

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Abstract

Perovskite-type chromites ACr0.9557Fe0.05O3 (A = Sc, In, Tl, Bi) have been studied by probe Mössbauer spectroscopy on 57Fe nuclei. The spectra of the ACr0.9557Fe0.05O3 samples (A = Sc, In, Bi) measured above the Néel temperature TN indicate the presence of several nonequivalent positions occupied by impurity iron atoms in all chromites. To explain significant differences in quadrupole splittings, semi-empirical calculations of the electric field gradient have been performed for all studied compounds within the ionic model taking into account monopole and dipole contributions. The performed calculations are in satisfactory agreement with experimental data.

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Funding

This work was supported by the Russian Foundation for Basic Research (project no. 19-03-00976).

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Authors and Affiliations

  1. Faculty of Chemistry, Moscow State University, 199991, Moscow, Russia

    A. V. Sobolev, A. V. Bokov, I. A. Presniakov & I. S. Glazkova

  2. Research Center for Functional Materials, National Institute for Materials Science (NIMS), 305-0044, Tsukuba, Ibaraki, Japan

    W. Yi & A. A. Belik

Authors
  1. A. V. Sobolev
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  2. A. V. Bokov
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  3. W. Yi
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  4. A. A. Belik
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  5. I. A. Presniakov
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  6. I. S. Glazkova
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Corresponding author

Correspondence to A. V. Sobolev.

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Translated by R. Tyapaev

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Sobolev, A.V., Bokov, A.V., Yi, W. et al. Electric Hyperfine Interactions of 57Fe Impurity Atoms in ACrO3 Perovskite-Type Chromites (A = Sc, In, Tl, Bi). J. Exp. Theor. Phys. 129, 896–902 (2019). https://doi.org/10.1134/S1063776119090127

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