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Degradation of the Optical Properties of Two-Layer Hollow ZnO/SiO2 Particles after Irradiation with Protons

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Abstract

A comparative analysis of the diffuse reflectance spectra in the range of 200–2500 nm and their changes after the irradiation of bilayer hollow ZnO/SiO2 particles and bulk ZnO microparticles with 100 keV protons is carried out. Simulation of the effect of protons on an ensemble of hollow bilayer particles in the GEANT4 environment is presented. Analysis of the experimental and theoretical calculations shows that the radiation resistance of hollow ZnO/SiO2 particles is less than that of bulk ZnO microparticles. This effect of increasing the radiation resistance of hollow ZnO/SiO2 particles can be due to: their high specific surface, which is a sink of radiation-induced defects; the presence of a protective amorphous SiO2 layer on the surface of ZnO microspheres, which lead to a decrease in the concentration of absorption centers in ZnO, causing absorption in the visible range of the spectrum.

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Authors and Affiliations

  1. Аmur State University, 675027, Blagoveshchensk, Russia

    A. N. Dudin & V. V. Neshchimenko

  2. Harbin Institute of Technology, 150001, Harbin, Heilongjiang, People’s Republic of China

    Chundong Li

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  1. A. N. Dudin
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  2. V. V. Neshchimenko
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  3. Chundong Li
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Correspondence to A. N. Dudin.

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Translated by N. Petrov

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Dudin, A.N., Neshchimenko, V.V. & Li, C. Degradation of the Optical Properties of Two-Layer Hollow ZnO/SiO2 Particles after Irradiation with Protons. J. Surf. Investig. 15 (Suppl 1), S173–S178 (2021). https://doi.org/10.1134/S1027451022020288

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