Evaluation of specific cost of obtainment of lead-208 isotope by gas centrifuges using various raw materials

Abstract

Evaluations of the specific cost of producing by gas centrifuges highly enriched 208Pb isotope, which may be used as a coolant and a neutron reflector in promising fast neutron reactors, have been carried out. The methodology originally developed for column type separation elements was applied in the calculations. As raw materials, a mixture of natural lead isotopes and radiogenic lead were considered. In the latter case which the content of the target isotope is nearly 1.5 times greater than in a former one. The price limit for the cost of radiogenic lead was established, up to which lower specific cost of producing highly enriched 208Pb isotope were achieved compared to the natural isotopic mixture.

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References

  1. 1.

    Khorasanov, G.L. and Blokhin, A.I., A Low Neutron Absorbing Coolant for Lead Fast Reactors and Accelerator Driven Systems, in Cooling Systems: Energy, Engineering, and Applications, Shanley, A.I., Ed., New York: Nova, 2011, p. 89.

    Google Scholar 

  2. 2.

    Khorasanov, G.L., Korobeynikov, V.V., Ivanov, A.P., and Blokhin, A.I., Minimization of an Initial Fast Reactor Uranium-Plutonium Load by Using Enriched Lead-208 as a Coolant, Nucl. Eng. Des., 2009, no. 239, p. 1703.

  3. 3.

    Apse, V.A., Kulikov, G.G., Shmelev, A.N., and Sirotkin, A.M., Possibility of Improvement of Neutron-Physical and Thermal-Hydraulic Parameters of Energetic and Fast Reactors with the Use of Radiogenic Lead as the Heat Transfer Medium, Yad. Fiz. Inzh., 2010, vol. 1, no. 5, p. 387.

    Google Scholar 

  4. 4.

    Bokhan, P.A., Buchanov, V.V., Zakrevskii, D.E., et al., Current Trends in Laser Separation of Isotopes in Monoatomic Vapors, Russ. Laser Res., 2003, vol. 24, no. 2, p. 159.

    Article  CAS  Google Scholar 

  5. 5.

    Babichev, A.P., Gorshunov, N.M., Dolgolenko, D.A., et al., Electron Cyclotron Resonance: Source of Plasma for Isotope Separation by the Ion Cyclotron Resonance Method, Prikl. Fiz., 2001, no. 3, p. 41.

  6. 6.

    Borisevich, V.D., Borman, V.D., Sulaberidze, G.A., et al., Fizicheskie osnovy razdeleniya izotopov v gazovoi tsentrifuge (Physical Foundations of Isotope Separation in a Gas Centrifuge), Borman, V.D., Ed., Moscow: Mos. Energ. Inst., 2011.

    Google Scholar 

  7. 7.

    Seneda, J.A., Forbicini, C.A.L.G., Queiroz, C.A., et al., Study on Radiogenic Lead Recovery from Residues in Thorium Facilities Using Ion Exchange and Electrochemical Process, Prog. Nucl. Energy, 2010, vol. 52, no. 3, p. 304.

    Article  CAS  Google Scholar 

  8. 8.

    Song, T., Zeng, S., Sulaberidze, G.A., et al., Comparative Study of the Model and Optimum Cascades for Multicomponent Isotope Separation, Sep. Sci. Technol., 2010, vol. 45, p. 2113.

    Article  CAS  Google Scholar 

  9. 9.

    Cohen, K., The Theory of Isotope Separation as Applied to the Large Scale Production of 235 U, New York: McGraw-Hill, 1951.

    Google Scholar 

  10. 10.

    Sulaberidze, G.A., Palkin, V.A., Borisevich, V.D., et al., Teoriya kaskadov dlya razdeleniya binarnykh i mnogokomponentnykh izotopnykh smesei (Cascade Theory for Separation of Binary and Multicomponent Isotope Mixtures), Borman, V.D., Ed., Moscow: MIFI, 2011.

    Google Scholar 

  11. 11.

    Tetramethyl Lead, The Hazardous Substances Data Bank (HSDB), Bethesda, Md.: USA National Library of Medicine, 1989.

    Google Scholar 

  12. 12.

    Chuzhinov, V.A., Laguntsov, N.I., Nikolaev, B.I., and Sulaberidze, G.A., Optimizing the Operation of Mass Diffusion Cascades, At. Energ., 1975, vol. 38, no. 6, p. 363.

    Article  Google Scholar 

  13. 13.

    Kaminskii, V.A., Sulaberidze, G.A., Tubin, A.A., and Chuzhinov, V.A., Multiparameter Optimization of Isotope Separation, Inzh.-Fiz. Zh., 1982, vol. 42, no. 4, p. 608.

    CAS  Google Scholar 

  14. 14.

    Aisen, E.M., Borisevich, V.D., Levin, E.V., et al., Study of Isotope Separation of Some Chemical Elements in a Gas Centrifuge, Nucl. Instrum. Methods Phys. Res., Sect. A, 1996, vol. 374, no. 1, p. 127.

    Article  CAS  Google Scholar 

  15. 15.

    Sinev, N.M., Ekonomika yadernoi energetiki (Economics of Nuclear Power), Moscow: Energoatomizdat, 1987.

    Google Scholar 

  16. 16.

    Zippe, G., Beams, J.W., and Kuhlthau, A.R., The Development of Short Bowl Ultracentrifuges, Progress Report, no. 1, Charlottesville: Virginia Univ., 1958.

    Google Scholar 

  17. 17.

    Glazer, A., Characteristics of the Gas Centrifuge for Uranium Enrichment and Their Relevance for Nuclear Weapon Proliferation, Sci. Global Security, 2008, vol. 16, p. 1.

    Article  Google Scholar 

  18. 18.

    Bortnyanskii, A.L., Demidov, V.L., Motovilov, S.A., et al., Experimental Laser Complex for Lead Isotope Separation by Selective Photochemical Reactions, X Mezhd. konf. “Fiziko-khimicheskie protsessy pri selektsii atomov i molekul” (X Int. Conf. on Physical and Chemical Processes in the Selection of Atoms and Molecules), Moscow, 2005, p. 76.

  19. 19.

    Andrienko, O.S., Afanas’ev, V.G., Egorov, N.B., et al., Lead Metal Production from Tetramethyllead, Perspektiv. Mater., 2010, no. 8, p. 199.

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Correspondence to A. Yu. Smirnov.

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Original Russian Text © A.Yu. Smirnov, V.D. Borisevich, G.A. Sulaberidze, 2012, published in Teoreticheskie Osnovy Khimicheskoi Tekhnologii, 2012, Vol. 46, No. 4, pp. 463–469.

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Smirnov, A.Y., Borisevich, V.D. & Sulaberidze, A. Evaluation of specific cost of obtainment of lead-208 isotope by gas centrifuges using various raw materials. Theor Found Chem Eng 46, 373–378 (2012). https://doi.org/10.1134/S0040579512040161

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Keywords

  • 208Pb
  • Lead Isotope
  • Isotope Separation
  • Specific Cost
  • Natural Mixture