Unconventional spin-charge phase separation in a model 2D cuprate
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In this work, we address a challenging problem of a competition of charge and spin orders for high-Tc cuprates within a simplified 2D spin-pseudospin model which takes into account both conventional Heisenberg Cu2+−Cu2+ antiferromagnetic spin exchange coupling (J) and the on-site (U) and intersite (V) charge correlations in the CuO2 planes with the on-site Hilbert space reduced to only three effective charge states (nominally Cu1+;2+;3+). We performed classical Monte Carlo calculations for large square lattices implying the mobile doped charges and focusing on a case of a small intersite repulsion V ≪ J. The on-site attraction (U < 0) does suppress the antiferromagnetic ordering and gives rise to a checkerboard charge order with the doped charge distributed randomly over a system in the whole temperature range. However, under the on-site repulsion (U > 0) the homogeneous ground state antiferromagnetic solutions of the doped system found in a mean-field approximation are shown to be unstable with respect to a phase separation with the charge and spin subsystems behaving like immiscible quantum liquids. Puzzlingly, with lowering the temperature one can observe two sequential phase transitions: first, an antiferromagnetic ordering in the spin subsystem diluted by randomly distributed charges, then, a charge condensation in the charge droplets. The effects are illustrated by the Monte Carlo calculations of the specific heat and longitudinal magnetic susceptibility.
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