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Coherent Acoustic Phonon Activation by Fast Electron Transfer in the Exciton Redox-Quenching Reaction with Methyl Viologen in Cadmium Selenide

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Abstract

Fast exciton quenching by methyl viologen (MV2+), an electron acceptor, on the CdSe quantum dot surface impulsively induces acoustic vibration via the mechanism of inverse piezoelectric effect, thereby causing an increase in the amplitude of the coherent acoustic phonon in the CdSe/MV2+ system compared to pure CdSe.

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ACKNOWLEDGMENTS

This work was supported by the Russian Science Foundation, grant no. 17-13-01506.

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Authors and Affiliations

  1. Semenov Institute of Chemical Physics, Russian Academy of Sciences, 119991, Moscow, Russia

    F. E. Gostev, I. V. Shelaev, A. V. Aibush, A. N. Kostrov, A. A. Titov & V. A. Nadtochenko

  2. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, 119991, Moscow, Russia

    S. Yu. Kochev & Yu. A. Kabachii

  3. Institute of Problems of Chemical Physics, Russian Academy of Sciences, 142432, Chernogolovka, Moscow oblast, Russia

    N. N. Denisov & V. A. Nadtochenko

  4. Faculty of Chemistry, Moscow State University, 119991, Moscow, Russia

    V. A. Nadtochenko

Authors
  1. F. E. Gostev
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  2. I. V. Shelaev
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  3. A. V. Aibush
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  4. A. N. Kostrov
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  5. A. A. Titov
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  6. S. Yu. Kochev
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  7. Yu. A. Kabachii
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  8. N. N. Denisov
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  9. V. A. Nadtochenko
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Corresponding author

Correspondence to V. A. Nadtochenko.

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Translated by S. Zatonsky

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Gostev, F.E., Shelaev, I.V., Aibush, A.V. et al. Coherent Acoustic Phonon Activation by Fast Electron Transfer in the Exciton Redox-Quenching Reaction with Methyl Viologen in Cadmium Selenide. High Energy Chem 52, 508–509 (2018). https://doi.org/10.1134/S001814391806005X

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  • DOI: https://doi.org/10.1134/S001814391806005X

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