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Optical limiters and diffraction elements based on a COANP-fullerene system: Nonlinear optical properties and quantum-chemical simulation

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Abstract

The results of optical study and quantum-chemical simulation of a conjugated organic system, 2-cyclooctylamino-5-nitropyridine (COANP)-fullerene, performed to determine its potential for application as a limiter of visible and near-IR laser radiation and as a material for diffraction elements in systems for reversible recording of optical information, are presented. Complexation between a COANP molecule and fullerene is considered as one of the main mechanisms responsible for the corresponding properties of this system. For the first time, nonlinear optical characteristics of COANP-C60 and COANP-C70 systems are comparatively studied and the intermolecular interaction between a COANP molecule and fullerene is analyzed on the quantum-chemical level.

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Authors and Affiliations

  1. Vavilov State Optical Institute All-Russia Research Center, St. Petersburg, 199034, Russia

    N. V. Kamanina

  2. Russian University of Peoples’ Friendship, Moscow, 117198, Russia

    E. F. Sheka

Authors
  1. N. V. Kamanina
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  2. E. F. Sheka
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Correspondence to N. V. Kamanina.

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__________

Translated from Optika i Spektroskopiya, Vol. 96, No. 4, 2004, pp. 659–673.

Original Russian Text Copyright © 2004 by Kamanina, Sheka.

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Kamanina, N.V., Sheka, E.F. Optical limiters and diffraction elements based on a COANP-fullerene system: Nonlinear optical properties and quantum-chemical simulation. Opt. Spectrosc. 96, 599–612 (2004). https://doi.org/10.1134/1.1719152

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