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Microscopic model of optically induced anisotropy of third-order nonlinearity in azo-dye polymer systems

  • Atoms, Spectra, Radiations
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Abstract

A large photoinduced reversible change of third-harmonic generation in azo-dye polymer thin films was recently observed. In this work, the microscopic interpretation of this phenomenon is given. The model presented is based on an angular hole burning and molecular reorientation due to trans-cis photoisomerization of azo-dye molecules.

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References

  1. L. M. Hayden, G. F. Sauter, F. R. Ore, et al., J. Appl. Phys. 68, 456 (1990).

    Article  ADS  Google Scholar 

  2. M. Dumont, S. Hosotte, G. Froc, and Z. Sekkat, Proc. SPIE 2042, 2 (1994).

    ADS  Google Scholar 

  3. Z. Sekkat and M. Dumont, Appl. Phys. B B53, 121 (1991).

    Google Scholar 

  4. P. N. Prasad and D. J. Williams, Introduction to Nonlinear Optical Effects in Molecules and Polymers (Wiley, New York, 1991).

    Google Scholar 

  5. K. Y. Wong and A. F. Garito, Phys. Rev. A 34, 5051 (1986).

    ADS  Google Scholar 

  6. Z. Sekkat and M. Dumont, Appl. Phys. B B54, 486 (1992).

    Google Scholar 

  7. V. M. Churikov and C. C. Hsu, Appl. Phys. Lett. 77, 2095 (2000).

    Article  ADS  Google Scholar 

  8. Z. Sekkat, D. Morichere, M. Dumont, et al., J. Appl. Phys. 71, 1543 (1992).

    Article  ADS  Google Scholar 

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From Pis’ma v Zhurnal Éksperimental’no\(\overset{\lower0.5em\hbox{$\smash{\scriptscriptstyle\smile}$}}{l} \) i Teoretichesko\(\overset{\lower0.5em\hbox{$\smash{\scriptscriptstyle\smile}$}}{l} \) Fiziki, Vol. 72, No. 8, 2000, pp. 595–599.

Original English Text Copyright © 2000 by Churikov.

This article was submitted by the authors in English.

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Churikov, V.M. Microscopic model of optically induced anisotropy of third-order nonlinearity in azo-dye polymer systems. Jetp Lett. 72, 415–418 (2000). https://doi.org/10.1134/1.1335119

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  • DOI: https://doi.org/10.1134/1.1335119

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