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Solving the activity–stability trade-off riddle

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Atomically dispersed and nitrogen-coordinated single iron site catalysts hold great promise to replace platinum for proton-exchange membrane fuel cells, but they suffer from significant performance loss. Now, solving the conundrum to distinguish durable and non-durable FeN4 active sites can guide high-performance catalyst design.

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Fig. 1: In situ identification of active sites in Fe–N–C catalysts.

References

  1. Wang, X. X., Swihart, M. T. & Wu, G. Nat. Catal. 2, 578–589 (2019).

    Article  CAS  Google Scholar 

  2. Wu, G., More, K. L., Johnston, C. M. & Zelenay, P. Science 332, 443–447 (2011).

    Article  CAS  Google Scholar 

  3. Zhang, H. et al. Energy Environ. Sci. 12, 2548–2558 (2019).

    Article  CAS  Google Scholar 

  4. Zhang, H. et al. J. Am. Chem. Soc. 139, 14143–14149 (2017).

    Article  CAS  Google Scholar 

  5. He, Y., Liu, S., Priest, C., Shi, Q. & Wu, G. Chem. Soc. Rev. 49, 3484–3524 (2020).

    Article  CAS  Google Scholar 

  6. Shao, Y., Dodelet, J.-P., Wu, G. & Zelenayet, P. Adv. Mater. 31, 1807615 (2019).

    Article  Google Scholar 

  7. Jia, Q., Liu, E., Jiao, L., Pann, S. & Mukerjee, S. Adv. Mater. 31, 1805157 (2018).

    Article  Google Scholar 

  8. Li, J. et al. Nat. Catal. https://doi.org/10.1038/s41929-020-00545-2 (2020).

  9. Wang, X. X., Prabhakaran, V., He, Y., Shao, Y. & Wu, G. Adv. Mater. 31, 1805126 (2019).

    Article  Google Scholar 

  10. He, Y. et al. Adv. Mater. 32, 2003577 (2020).

    Article  CAS  Google Scholar 

  11. Shi, Q. et al. Mater. Today 37, 93–111 (2020).

    Article  CAS  Google Scholar 

  12. Zhu, Y. et al. Adv. Energy Mater. 10, 1902844 (2020).

    Article  CAS  Google Scholar 

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Correspondence to Gang Wu.

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Liu, S., Shi, Q. & Wu, G. Solving the activity–stability trade-off riddle. Nat Catal 4, 6–7 (2021). https://doi.org/10.1038/s41929-020-00567-w

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