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Aerosols Emitted from a Livestock Farm in Southern Germany

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Abstract

We studied the atmospheric aerosol of a farm directly on farm, downwind, and in the background with the aim to characterize the aerosol source of livestock farming physically and chemically. The farm hosted chicken, cattle and pig.The farm was found to be a source of primary and secondary particles. Super-μm particles of various types were emitted from the stables and adjacent facilities related to farming activities. On farm elevated concentrations of ammonia, particulate ammonium and nitrate were observed. The significant emission of condensation nuclei and large, 2 μm-sized particles (droplets) was observed under humid conditions in plumes which most likely originated from open manure pits at least in one case. It is suggested that this aerosol mode consisted of ammonium haze droplets formed by saturation of advected air with ammonia within a few minutes. In one night, a mass uptake of Δm > 5.4 μg m-3 in the super-μm mode was observed along with a loss of Δm = —1.0 μg m-3 in the sub-μm mode based on differential sampling upwind and downwind of the farm. The particulate matter mass median diameter was correspondingly shifted from 1.32 to 3.39 μm. About one third of the mass increase was due to organic carbon. Furthermore, differential sampling showed particulate calcium and nitrate/nitric acid to be emitted from the farm, too. The study encourages to systematically characterize the aerosol emitted from livestock raising in future studies of similar kind.

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References

  • BMU — Federal Ministry for the Environment, Nature Conservation and Reactor Safety: 1997, ‘Klimaschutz in Deutschland’, 2nd Report of the Federal Government, Umweltbundesamt, Berlin, Germany, 324 pp.

    Google Scholar 

  • Cercasov, V., Pantelica, A., Salagean, M. and Schreiber, H.: 1998, ‘Comparative evaluation of some pollutants in the airborne particulate matter in Eastern and Western Europe: two-city study Bucharest-Stuttgart’, Environ. Poll. 101, 331—337.

    Article  CAS  Google Scholar 

  • CORINAIR: 1998, ‘Atmospheric Emission Inventory Guidebook’, 1st ed., G. McInnes (ed.), European Environment Agency, Copenhagen, Denmark.

    Google Scholar 

  • Doorn, M. R. J., Natschke, D. F., Thorneloe, S. A. and Southerland, J.: 2002, ‘Development of an emission factor for ammonia emissions from US swine farms based on field tests and application of a mass balance method', Atmos. Environ. 36, 5619—5625.

    Article  CAS  Google Scholar 

  • Dorsey, J. R., Nemitz, E., Gallagher, M.W., Fowler, D., Williams, P. I., Bower, K. N. and Beswick, K. M.: 2002, ‘Direct measurements and parametersiation of aerosol flux, concentration and emission velocity above a city’, Atmos. Environ. 36, 791—800.

    Article  CAS  Google Scholar 

  • Dougle, P. G., Veefkind, J. P. and ten Brink, H. M.: 1998, ‘Crystallisation of mixtures of ammonium nitrate, ammonium sulphate and soot’, J. Aerosol Sci. 29, 375—386.

    CAS  Google Scholar 

  • Gallmann, E., Hartung, E. and Jungbluth, H.: 2000, ‘Assessment of two pig housing and ventilation systems regarding indoor air quality and gas emissions — diurnal and seasonal effects’, Proceedings International Conference Agricultural Engineering, 2.—7.7.2000, Warwick, UK, Contribution No. 00-FB-002, 9 pp.

  • IIASA — International Institute for Applied Systems Analyses: 2001, ‘Rains PM Modul’, IIASA, Laxenburg (Austria). Internet: http://www.iiasa.ac.at/?rains/PM/pm-home.html

  • Jaenicke, R.: 1988, ‘Aerosol physics and chemistry’, Landolt-Börnstein Neue Serie 4b, 391—457.

    Google Scholar 

  • Lammel, G., Brüggemann, E., Gnauk, T., Müller, K., Neusüss, C. and Röhrl A.: 2003, ‘A new method to study aerosol source contributions along the tracts of air parcels and its application to the near-ground level aerosol chemical composition in central Europe’, J. Aerosol Sci. 34, 36—61.

    Google Scholar 

  • Lange, I.G., Daxenberger, A., Schiffer, A., Witters, H., Ibarreta, D. and Meyer, H. D. H.: 2002, ‘Sex hormones originating from different livestock production systems: fate and potential disrupting activity in the environment’, Anal. Chim. Acta 473, 27—37.

    Article  CAS  Google Scholar 

  • Mehlmann, A. and Warneck, P.: 1995, ‘Atmospheric gaseous HNO3, particulate nitrate and aerosol size distributions of major ionic species at a rural site in Western Germany’, Atmos. Environ.. 29, 2359—2373.

    Article  CAS  Google Scholar 

  • Mozurkewich, M.: 1993, ‘The dissociation constant of ammonium nitrate and its dependence on temperature, relative humidity and particle size’, Atmos. Environ.. 27A, 261—270.

    CAS  Google Scholar 

  • Müller, K.: 1999, ‘A three-year study of the aerosol in northwest Saxony’, Atmos. Environ. 33, 1679—1685.

    Article  Google Scholar 

  • Nemitz, E., Dorsey, J. R., Flynn, M., Gallagher, M. W. and Sutton, M. A.: 2002, ‘Particle growth above grassland following NH4NO3 fertiliser application’, in P. M. Midgley and M. Reuther (eds), Transport and Chemical Transformation in the Troposphere, Proceedings of EUROTRAC Symposium 2002, Garmisch-Partenkirchen, 11—15 March 2002, Margraf, Weikersheim, Germany, 310 pp. + CDROM

  • Rogge, W. F., Mazurek, M. A., Hildemann, L. M., Cass, G. R. and Simoneit, B. R. T.: 1993, ‘Quantification of urban organic aerosols at a molecular level: Identification, abundance and sesonal variation’, Atmos. Environ. 27A, 1309—1330.

    CAS  Google Scholar 

  • Rogge, W. F., Mazurek, M. A., Hildemann, L. M., Cass G. R. and Simoneit, B. R. T., et al.: 1991—1998, ‘Sources of fine organic aerosol. Parts 1.—9.’, Environ. Sci. Technol. 25, 1112—1125 and 27, 636—651 and 27, 1892—1904 and 27, 2700—2710 and 27, 2736—2744 and 28, 1375—1388 and 31, 2726—2730 and 31, 2731—2737 and 32, 13—22.

    Article  CAS  Google Scholar 

  • Röhrl, A. and Lammel, G.: 2002, ‘Determination of malic acid and other C4 dicarboxylic acids in atmospheric aerosol samples’, Chemosphere 46, 1195—1199.

    Article  Google Scholar 

  • Schmid, H., Laskus, L., Abraham, H. J., Baltensperger, U., Lavanchy, V., Bizjak, M., Burba, P., Cachier, H., Crow, D., Chow, J., Gnauk, T., Even, A., ten Brink, H. M., Giesen, K. P., Hitzenberger, R., Hueglin, C., Maenhaut, W., Pio, C., Carvalho, A., Putaud, J. P., Toom-Sauntry, D. and Puxbaum, H.: 2001, ‘Results of the "Carbon Conference" international aerosol carbon round robin test stage I’, Atmos. Environ. 35, 2111—2121.

    CAS  Google Scholar 

  • Schneider, F., Engelhardt, T. and Wieser, P.: 2002, ‘Properties of airborne dust from pig husbandries and their effects on measurement’, in T. Hinz (ed.), Landbauforschung Völkenrode, Particulate Matter in and from Agriculture, Special Issue 235, Bundesforschungsanstalt für Landwirtschaft, Braunschweig, Germany, pp. 163—173.

    Google Scholar 

  • Seinfeld, J. H.: 1986, ‘Atmospheric Chemistry and Physics of Air Pollution’, Wiley, New York.

    Google Scholar 

  • Steinhoff, G., Haupt, O. and Dannecker, W.: 2000, ‘Fast determination of trace elements on aerosol-loaded filters by X-ray fluorescence analysis considering the inhomogeneous elemental distribution’, Freenius J. Anal. Chem. 366, 174—177.

    CAS  Google Scholar 

  • Sutton, M. A., Asman, W. A. H., Ellermann, T., van Jaarsveld, J. A., Acker, A., Aneja, V., Duyzer, J., Horvath, L., Paramonov, S., Mitrosinkova, M., Sim Tang, Y., Achermann, B., Gauger, T., Bartniki, J., Neftel, A. and Erisman, J. W.: 2003, ‘Establishing the link between ammonia emission control and measurements of reduced nitrogen concentrations and deposition’, Environ. Monit. Assess. 82, 149—185.

    Article  CAS  Google Scholar 

  • Takai, H., Pedersen, S., Johnsen, J. O., Metz, J. H. M., Groot Koerkamp, P. W. G., Uenk, G. H., Phillips, V. R., Holden, M. R., Sneath, R. W., Short, J. L., White, R. P., Hartung, J., Seedorf, J., Schröder, M., Linkert, K. H. and Wathes, C.M.: 1998, ‘Concentrations and emissions of airborne dust in livestock buildings in northern Europe’, J. Agric. Eng. Res. 70, 59—77.

    Article  Google Scholar 

  • Tang, I. N. and Munkelwitz, H. R.: 1994, ‘Aerosol phase transformation and growth in the atmosphere’, J. Applied Meteor. 33, 791—796.

    Google Scholar 

  • Turnbull, A. B. and Harrison, R. M.: 2000, ‘Major component contributions to PM10 composition in the United Kingdom’, Atmos. Environ. 34, 3129—3137.

    Article  CAS  Google Scholar 

  • Wehner, B., Birmili, W., Gnauk, T. and Wiedensohler, A.: 2002, ‘Particle number size distributions in a street canyon and their transformations into the urban-air background: measurements and a simple model study’, Atmos. Environ.. 36, 2214—2223.

    Article  Google Scholar 

  • Weingartner, E., Keller, C., Stahel, W.A., Burtscher, H. and Baltensperger, U.: 1997, ‘Aerosol emissions in a road tunnel’ Atmos. Environ. 31, 451—462.

    CAS  Google Scholar 

  • Winkler, P.: 1988, ‘The growth of atmospheric aerosol particles with relative humidity’, Physica Scripta 37, 223—230.

    CAS  Google Scholar 

  • Wurster, R.: 1997, ‘EDX measurements on nanoparticles in a high resolution scanning electron microscope’, J. Trace Microprobe Techniques 15, 467—470.

    CAS  Google Scholar 

  • Zimmerling, R., Dämmgen, U., Küsters, A., Grünhage, L. and Jäger, H. J.: 1996, ‘Response of a grassland ecosystem to air pollution. IV. The chemical climate: Concentrations of non-criteria pollutants (trace gases and aerosols)’, Environ. Poll. 91, 139—147.

    Article  CAS  Google Scholar 

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Lammel, G., Schneider, F., Brüggemann, E. et al. Aerosols Emitted from a Livestock Farm in Southern Germany. Water, Air, & Soil Pollution 154, 313–330 (2004). https://doi.org/10.1023/B:WATE.0000022962.65942.4b

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