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Current levels and distribution of 137Cs and Pu isotopes in soil on the Kazakhstan territory of the Kazakhstan-Chinese border: Semipalatinsk and Lob Nor nuclear test sites detonation

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Abstract

More than 100 soil samples were collected from 46 sites along roads and some settlements connecting Alma-Ata to Semipalatinsk City of the Kazakhstan-Chinese border and analyzed for 137Cs and Pu isotopes (238Pu, 239Pu and 240Pu). The mean 137Cs inventory at each site was within the range of 1,000-3,000 Bq/m2 for most of the sites. The 239,240Pu concentration and its inventories were observed in the wide range of 0.18-2.6 Bq/kg and 28-677 Bq/m2, respectively. At the most northern sites in the areas studied, higher239,240Pu inventories were found corresponding to the increase of 239,240Pu fraction which was not leached by hot digestion with conc. HNO3+H2O2. The 239,240Pu/137Cs activity ratios for the soil samples from the southern areas lie in the narrow range of 0.016–0.039 (most of data being 0.02–0.03), probably indicative of global fallout origin. On the other hand, a little or several higher ratios (0.05 to 0.22) were found for soil samples from the northern areas. These higher ratios demonstrate strongly that there was additional Pu input of local fallout due to the atomic explosions. From 240Pu/239Pu atomic ratios measured, contribution of local fallout 239,240Pu, probably from the SNTS, was found to be higher (60–86%) in the sites around the northern areas than the southern ones. The present data might serve not only as a current baseline information on distribution and contamination levels of the long-lived fallout radionuclides in the Kazakhstan areas of the Kazakhstan-Chinese border, but also as a aid of selection of control area for epidemiological projects.

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References

  1. U. V. Dubasov, S. A. Zelentsoz, G. A. Krasilov, V. A. Logachyov, A. M. Matsushchenko, S. G. Smagulov, B. S. Tsaturov, G. A. Tsirkov, A. K. Chernyshov, Chronological list of the atmospheric nuclear tests at the Semipalatinsk test site and their radiological characteristics, in: Scientific Research Institute for Regional Medical and Ecological Problem, Herald of the Research Program “Semipalatinsk Test Site-Altai” N4, 1994, J. H. Shoikhet (Ed.), Scientific and Practical Journal, Digest of the International Panel Meet “NATO/SCOPE-RADTEST”., Barnaul, September 5-10, 1994.

  2. V. S. Boharov, S. A. Zelentsoz, V. N. Mikhailov, At. Energ., 67 (1989) 210.

    Google Scholar 

  3. B. I. Gusev, R. I. Rosenson, Z. N. Abylkassimova, Radiat. Environ. Biophys., 36 (1997) 201.

    Article  CAS  Google Scholar 

  4. C. Lindoholm, S. L. Shimon, B. Makar, K. Baverstock (Eds), Workshop on Dosimetry of the Population Living in the Proximity of the Semipalatinsk Atomic Weapons Test Site, STUK-A187, Feburary 2002.

  5. K. Gordeev, I. Vasilenko, A. Lebedev, A. Bouville, U. Luckyanov, S. L. Simon, Y. Stepanov, S. Shinlarev, L. Anspaugh, Radiat. Environ. Biophys., 41 (2002) 61.

    CAS  Google Scholar 

  6. B. Grosche, C. Land, S. Bauer, L. M. Pivina, Z. N. Abylkassimova, B. I. Gusev, Radiat. Environ. Biophys., 41 (2002) 75.

    CAS  Google Scholar 

  7. J. Takada, M. Hoshi, S. Endo, M. Yamamoto, T. Nagatomo, B. I. Gusev, R. I. Rosenson, K. N. Apsalikov, N. J. Tchaijunusova, 2nd Intern. Symp. of Effect of Low-level Radiation for Residents near Semipalatinsk Nuclear Test Site, Hiroshima, July 23.25, 1996, M. Hoshi et al. (Eds), 1997, p. 195.

  8. J. Takada, M. Hoshi, T. Nagatomo, M. Yamamoto, S. Endo, T. Takatsuji, I. Oshikawa, B. I. Gusev, A. Kh. Sekerbaev, N. J. Tchaijunusova, J. Radiat. Res., 40 (1999) 337.

    Article  CAS  Google Scholar 

  9. M. Yamamoto, A. Tsumura, Y. Katayama, T. Tsukatani, Radiochim. Acta, 72 (1996) 209.

    CAS  Google Scholar 

  10. M. Yamamoto, T. Tsukatani, Y. Katayama, Health Phys., 71 (1996) 142.

    Article  CAS  Google Scholar 

  11. M. Yamamoto, A. Tsumura, T. Tsukatani, Radiochim. Acta, 81 (1998).

  12. M. Yamamoto, M. Hoshi, J. Takada, A. Kh. Sekerbaev, B. I. Gusev, J. Radioanal. Nucl. Chem., 242 (1999) 63.

    Article  CAS  Google Scholar 

  13. M. Yamamoto, M. Hoshi, J. Takada, S. Oikawa, I. Yoshikawa, T. Takatsuji, A. Kh. Sekerbaev, B. I. Gusev, Plutonium in the Environment, A. Kudo (Ed.), 2001, Elsevier Sciences Ltd., 2001, p. 375.

  14. M. Yamamoto, M. Hoshi, J. Takada, S. Oikawa, I. Yoshikawa, T. Takatsuji, A. Kh. Sekerbaev, B. I. Gusev, J. Radioanal. Nucl. Chem., 252 (2002) 373.

    Article  CAS  Google Scholar 

  15. B. I. Gusev et al., Estimation of external exposure doses in the population on the territories of Makanchi and Urdzhar districts of the Semipalatinsk Region formed due to Chines nuclear tests, A Transitional Report (Archives of Kazakh Scientific Research Institute for Radiation Medicine and Ecology), Semipalatinsk, 1990.

  16. V. Hodge, C. Smith, J. Whiting, Chemosphere, 32 (1996) 2067.

    Article  CAS  Google Scholar 

  17. M. Yamamoto, K. Komura, M. Sakanoue, J. Radiat. Res., 24 (1983) 237.

    Article  CAS  Google Scholar 

  18. M. Yamamoto, M. Hoshi, J. Takada, A. Sakaguchi, K. N. Apsalikov, B. I. Busev, J. Radioanal. Nucl. Chem., 261 (2004) 19.

    Article  CAS  Google Scholar 

  19. P. W. Krey, E. P. Hardy, USAES Report HASL-235, New York, 1970.

  20. P. W. Krey, D. C. Bogen, J. Radioanal. Nucl. Chem., 115 (1987) 335.

    Article  CAS  Google Scholar 

  21. E. P. Hardy, USAES Report HASL-306, New York, 1976, p. I–51.

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Authors and Affiliations

  1. Low Level Radioactivity Laboratory, K-INET, Kanazawa University Tatsunokuchi, Ishikawa, 923-1224, Japan

    M. Yamamoto & A. Sakaguchi

  2. International Radiation Information Center, Research Institute for Radiation Biology and Medicine, Hiroshima University Hiroshima, 734-5883, Japan

    M. Hoshi & J. Takada

  3. Kazakh Scientific Research Institute for Radiation Medicine and Ecology, Semipalatinsk, The Kazakhstan Republic

    K. N. Apsalikov & B. I. Gusev

Authors
  1. M. Yamamoto
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  2. M. Hoshi
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  3. J. Takada
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  4. A. Sakaguchi
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  5. K. N. Apsalikov
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  6. B. I. Gusev
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Yamamoto, M., Hoshi, M., Takada, J. et al. Current levels and distribution of 137Cs and Pu isotopes in soil on the Kazakhstan territory of the Kazakhstan-Chinese border: Semipalatinsk and Lob Nor nuclear test sites detonation. Journal of Radioanalytical and Nuclear Chemistry 261, 533–545 (2004). https://doi.org/10.1023/B:JRNC.0000037093.74415.7e

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  • DOI: https://doi.org/10.1023/B:JRNC.0000037093.74415.7e

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