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Study of PM2.5 in Beijing suburban site by neutron activation analysis and source apportionment

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Abstract

Airborne particulate matter (APM) was collected in coarse fraction and in PM2.5 during spring of 2002 in Beijing suburban sampling site by Gent SFU sampler. More attention has been paid to the special “events” such as dust, storm and haze. Taking advantage of the combination of thermal or epithermal neutron irradiation with Compton suppression spectrometer system, twenty elemental (Al, Si, Ca, K, Dy, Cu, I, In, Ba, W, Sn, Sb, As, Ti, Br, V, Mn, Cl, Na, Zn) concentration were determined. Among them, several key trace elements that cannot be accomplished by the traditional neutron activation analysis (NAA) were determined. The analysis of trace elemental concentration in PM2.5 shows that the anthropogenic elements such as As, In, Sn, Sb have different trends than crustal elements. The back-trajectories of the high concentration anthropogenic pollution elements revealed their source region. Six potential sources were resolved by positive matrix factorization (PMF), two area type and four source type, as soil, limestone quarry, crop burning and mixture of residue motor and coal burning sampling sites. Taking into account of everyday air particle back trajectories, source compositions together with source regions were also identified.

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References

  1. D. W. Dockery et al., Amer. Rev. Diseases, 139 (1989) 587.

    CAS  Google Scholar 

  2. M. Lippmann, Inhal. Toxicol., 7 (1995) 753.

    CAS  Google Scholar 

  3. D. W. Dockery, C. A. Pope, X. Xu, J. D. Spengler, J. H. Ware, M. E. Fay, B. G. Ferris Jr., F. E. Speizer, New Engl. J. Med., 329 (1993) 1753.

    Article  CAS  Google Scholar 

  4. D. W. Dockey, C. A. Pope, Rev. Public Health, 15 (1994) 107.

    Article  Google Scholar 

  5. Kebin He, Fumo Yang, Yongliang Ma, Qiang Zhang, Xiaohong Yao, Chak K. Chan, Steven Cadle, Tai Chan, P. Mulawa, Atmos. Environ., 35 (2001) 4959.

    Article  CAS  Google Scholar 

  6. Y. Zhang, X. Tang, M. Bi, D. Tang, D. Zhao, Acta Sci., 7 (1987) 269.

    CAS  Google Scholar 

  7. J. Zhang, Z. Chen, W. Wang, Acta Sci., 18 (1998) 62.

    CAS  Google Scholar 

  8. Lei Cao, Weizhi Tian, Bangfa Ni, Yangmei Zhang, Pingsheng Wang, Atmos. Environ., 36 (2002) 1951.

    Article  CAS  Google Scholar 

  9. M. P. Zelenka, W. E. Wilson, J. C. Chow, P. J. Lioy, Atmos. Environ., 28 (1994) 1425.

    Article  CAS  Google Scholar 

  10. J. G. Watson, Tan Zhou, J. C. Chow, J. Engelbrecht, E. M. Fujita, W. E. Wilson, Chemosphere, 49 (2002) 1093.

    Article  CAS  Google Scholar 

  11. Ph. K. Hopke, Chem. Listy, 10 (1991) 21.

    CAS  Google Scholar 

  12. Liu Xiande, Ph. K. Hopke, D. Cohen, G. Bailey, Sci. Total Environ., 175 (1995) 65.

    Article  Google Scholar 

  13. X. Querol, A. Alastuey, S. Rodriguez, F. Plana, C. R. Ruiz, N. Cots, G. MassaguÉ, O. Puig, Atmos. Environ., 35 (2001) 6407.

    Article  CAS  Google Scholar 

  14. J. W. Winchester, W. Lu, L. Ren, M. Wang, W. Maenhaut, Atmos. Environ., 15 (1981) 933; 1399.

    Article  CAS  Google Scholar 

  15. J. W. Winchester, M. Bi, Atmos. Environ., 18 (1984) 1399.

    Article  CAS  Google Scholar 

  16. M. Bi, J. Chen, R. Yao, F. Ding, M. Wang, X. Tang, M. Zhong, P. Liu, X. Feng, J. W. Winchester, H. C. Kaufmann, Biol. Trace Elem. Res., 6 (1984) 19.

    Article  CAS  Google Scholar 

  17. J. W. Winchester, Wang Ming Xing, Lu Wei Xiu, Ren Li Xin, Hong Zhong Shang, Nucl. Instrum. Meth. Phys. Res., B231 (1984) 503.

    Google Scholar 

  18. S. Yang, Y. Yang, Q. Qian, B. Chen, M. Zhong, C. Hu, Y. Sha, P. Liu, M. Yuan, J. Acta Sci., 7 (1987) 411.

    CAS  Google Scholar 

  19. F. Wei, E. Teng, G. Wu, W. Hu, Sci. Technol., 33 (1999) 4188.

    Article  CAS  Google Scholar 

  20. L. B. Davis, Guo Jixiang, Atmos. Environ., 34 (2000) 2703.

    Article  CAS  Google Scholar 

  21. Zhang Ren-jian, Wang Ming-xing, Xia Xiang-ao, J. Environ. Sci., 14 (2002) 7.

    CAS  Google Scholar 

  22. P. Paatero, U. Tapper, Chem. listy, 18 (1993) 183.

    CAS  Google Scholar 

  23. P. Paatero, U. Tapper, Environmetrics, 5 (1994) 111.

    Google Scholar 

  24. S. Juntto, P. Paatero, Environmetrics, 5 (1994) 127.

    Google Scholar 

  25. Y. L. Xie, P. K. Hopke, P. Paatero, L. A. Barrie, S. M. Li, J. Atmos. Sci., 56 (1999) 249.

    Article  Google Scholar 

  26. K. G. Paterson, J. L. Sagady, D. L. Hooper, Environ. Sci. Technol., 33 (1999) 635.

    Article  CAS  Google Scholar 

  27. M. Zhou, K. Okada, F. Qian, P.-M. Wu, L. Su, B. E. Casareto, T. Shimohara, Atmos. Res., 40 (1996) 19.

    Article  CAS  Google Scholar 

  28. Chang-Jin Ma, M. Kasahara, R. HÖller, T. Kamiya, Atmos. Environ., 35 (2001) 2707.

    Article  CAS  Google Scholar 

  29. R. A. Duce, C. K. Unni, B. J. Ray, J. M. Prospero, J. T. Merrill, Science, 209 (1980) 1522.

    CAS  Google Scholar 

  30. M. Uematsu, R. A. Duce, J. M. Prospero, L. Q. Chen, J. T. Merrill, R. L. McDonald, J. Geophys. Res., 88 (1983) 5343.

    Article  CAS  Google Scholar 

  31. Y. S. Chuang, Atmos. Environ., 26A (1992) 743.

    Google Scholar 

  32. M. Leinen, J. M. Prospero, E. Arnold, M. Blank, J. Geophys. Res., 99 (1994) 21017.

    Article  Google Scholar 

  33. S. Landsberger, J. Radioanal. Nucl. Chem., 179 (1994) 67.

    Article  CAS  Google Scholar 

  34. S. R. Biegalski, S. Landsberger, J. Radioanal. Nucl. Chem., 192 (1995) 195.

    Article  CAS  Google Scholar 

  35. S. Landsberger, S. Peshev, J. Radioanal. Nucl. Chem., 202 (1996) 201.

    Article  CAS  Google Scholar 

  36. B. Mason, Principles of Geochemistry, 3rd ed., New York, 1966, 45.

  37. M. S. Germanl, L. Gokmen, A. C. Sigleo, G. S. Kowalczyk, L. Olmez, A. M. Small, D. L. Anderson, M. P. Falley, M. C. Gulovall, C. E. Choquette, E. A. Lepel, G. E. Gordom, W. H. Zoller, Anal. Chem., 52 (1980) 2240.

    Article  Google Scholar 

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Lei, C., Landsberger, S., Basunia, S. et al. Study of PM2.5 in Beijing suburban site by neutron activation analysis and source apportionment. Journal of Radioanalytical and Nuclear Chemistry 261, 87–94 (2004). https://doi.org/10.1023/B:JRNC.0000030939.64724.9d

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  • DOI: https://doi.org/10.1023/B:JRNC.0000030939.64724.9d

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