Abstract
Absolute calibration of the UNIT-10m setup on the basis of the results obtained by destructive analysis is examined. The calibration procedure consists in performing measurements using the SKAT laboratory test stand at the Radium Institute with a model unirradiated assembly and neutron sources with known intensity, simulating neutron emission, comparing experimental data and calculations for certain reference points. The data obtained from destructive analysis can be used to establish a relation between the neutron flux of an irradiated assembly and the parameters being determined (fuel burnup, content of the main fissioning isotopes).
A relation is presented between burnup and accumulation of the main neutron-emitting isotopes in spent RBMK fuel. The data were obtained by radiochemical and α- and mass-spectrometric methods. The total neutron emission is determined taking account of the neutron yield from spontaneous-fission reactions of even isotopes of plutonium and curium and from (α, n) reactions.
Similar content being viewed by others
REFERENCES
A. G. Korenkov, A. A. Voronkov, N. M. Kazarinov, et al., “Nondestructive control of spent fuel assembly of RBMK-1000 reactors,” in: Proceedings of the Russian International Conference on Nuclear Material Protection. Control and Accounting. March 9–14, 1997, Obninsk, pp. 729–735.
V. V. Malinovskii, V. G. Vorob'ev, and B. D. Kuz'minov, “Review of measurements of the average number of prompt fission neutrons,” Voprosy At. Nauk. Tekh., Ser. Yad. Konst., No. 5(54), 19–21 (1983).
Decay Data of the Transactinium Nuclides, Technical Reports Ser. No. 61, IAEA, Vienna (1986).
A. V. Stepanov, T. P. Makarova, and S. G. Gritchenko, “Application of the electromigration method to radiochemical studies,” J. Radioanal. Chem., 21, 411–417 (1974).
B. N. Belyaev, V. D. Domkin, T. P. Makarov, et al., “Determination of ultrasmall quantities of americium, curium, and rare-earth elements in spent nuclear fuel by mass spectrometry with isotopic dilution,” Radiokhim., 39, No. 1, 61–65 (1997).
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Korenkov, A.G., Makarova, T.P., Stepanov, A.V. et al. Destructive Analysis Determination of Neutron Emission from Spent RBMK Fuel. Atomic Energy 93, 815–822 (2002). https://doi.org/10.1023/A:1022033528105
Issue Date:
DOI: https://doi.org/10.1023/A:1022033528105