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Fluctuating Electric Field Gradients at 111Cd in Ice

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Abstract

111Cd–PAC measurements have been made using the high specific activity of 111In in the methanol–water mixtures of various concentrations at the room temperature. These experiments revealed that the perturbation factors 〈A 2 G 2〉 (integrated over two mean lives τN) do not follow the dependence of the macroscopic viscosity η. The observed dynamic character of the PAC spectra in ice is explained by the mobility of orientational and ionic defects. The activation energy for the diffusion process was determined to be E a =0.35(1) eV.

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Authors and Affiliations

  1. Skobeltsyn Institute of Nuclear Physics, Moscow State University, 119899, Moscow, Russia

    Z. Z. Akselrod

  2. Joint Institute for Nuclear Research, LNP, P.O. Box 79, Moscow, Russia

    D. V. Filossofov, O. I. Kochetov, N. A. Korolev, N. A. Lebedev, A. F. Novgorodov & V. V. Timkin

  3. Institute for Nuclear Research, BAS, 1000, Sofia, Bulgaria

    M. Milanov & A. I. Velichkov

  4. Vereshchagin Institute of High Pressure Physics, RAS, 142092, Troitsk, Moscow reg., Russia

    E. N. Shirani

Authors
  1. Z. Z. Akselrod
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  2. D. V. Filossofov
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  3. O. I. Kochetov
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  4. N. A. Korolev
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  5. N. A. Lebedev
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  6. M. Milanov
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  7. A. F. Novgorodov
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  8. E. N. Shirani
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  9. V. V. Timkin
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  10. A. I. Velichkov
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Akselrod, Z.Z., Filossofov, D.V., Kochetov, O.I. et al. Fluctuating Electric Field Gradients at 111Cd in Ice. Hyperfine Interactions 136, 705–710 (2001). https://doi.org/10.1023/A:1020577428217

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