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The Effects of Nano-silica Addition on the Physical Properties of Polyethylene-Modified Asphalt Binder and the Mechanical Properties and Durability of Asphalt Mixtures

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Abstract

The effects of different dosages of nano-silica on the properties of high-density polyethylene (HDPE)- and low-density polyethylene (LDPE)-modified asphalt binders and mixtures were investigated. Penetration grade, softening point, ductility, and elastic recovery of the modified binders, as well as Marshall properties, indirect tensile strength (ITS), moisture damage, and raveling resistance of the mixtures were evaluated. Polymer modification decreased ductility and penetration grade and increased softening point, with a greater effect of HDPE than LDPE. Softening point increased and penetration grade decreased with raising the nano-silica content, with a greater effect of nano-silica on the HDPE-modified binder. The elastic recovery of asphalt binder was improved with polymer modification and the increase of nano-silica content with more elastic recovery for LDPE-modified asphalt. The Marshall properties and ITS of the asphalt mixtures were improved by polymer modification and raising the nano-silica content, with a higher ITS for HDPE-modified mixtures. Furthermore, polymer-modified mixtures have higher moisture damage and raveling resistance than the control mixture, and nano-silica addition improved the moisture damage resistance and negatively impacted the raveling resistance of the mixtures.

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References

  • Airey GD (2003) Rheological properties of styrene butadiene styrene polymer modified road bitumens. Fuel 82(14):1709–1719

    Google Scholar 

  • Alas M, Ali SIA, Abdulhadi Y, Abba SI (2020) Experimental evaluation and modeling of polymer nanocomposite modified asphalt binder using ANN and ANFIS. J Mater Civ Eng 32(10):04020305

    Google Scholar 

  • Alataş T, Yilmaz M (2013) Effects of different polymers on mechanical properties of bituminous binders and hot mixtures. Contr Build Mater 42:161–167

    Google Scholar 

  • Alghrafy YM, Abd Alla ESM, El-Badawy SM (2021) Rheological properties and aging performance of sulfur extended asphalt modified with recycled polyethylene waste. Constr Build Mater 273:121771

    Google Scholar 

  • Al-Hadidy AI, Yi-qiu T (2009) Effect of polyethylene on life of flexible pavements. Constr Build Mater 23(3):1456–1464

    Google Scholar 

  • Alhamali DI, Wu J, Liu Q, Hassan NA, Yusoff NIM, Ali SIA (2016) Physical and rheological characteristics of polymer modified bitumen with nanosilica particles. Arab J Sci Eng 41(4):1521–1530

    Google Scholar 

  • Ameri M, Hesami S, Goli H (2013) Laboratory evaluation of warm mix asphalt mixtures containing electric arc furnace (EAF) steel slag. Constr Build Mater 49:611–617

    Google Scholar 

  • Ameri M, Vamegh M, Rooholamini H, Haddadi F (2018) Investigating effects of nano/SBR polymer on rutting performance of binder and asphalt mixture. Adv Mater Sci Eng 28(8):155–173

    Google Scholar 

  • Attaelmanan M, Feng CP, Al-Hadidy AI (2011) Laboratory evaluation of HMA with high density polyethylene as a modifier. Constr and Build Mater 25(5):2764–2770

    Google Scholar 

  • Bala N, Napiah M, Kamaruddin I, Danlami N (2017) Rheological properties investigation of bitumen modified with nano-silica and polyethylene polymer. Int J Adv Appl Sci 4(10):165–174

    Google Scholar 

  • Bala N, Napiah M, Kamaruddin I (2018) Influence of nanosilica on moisture resistance of polymer modified bitumens. Pet Sci Technol 36(3):244–250

    Google Scholar 

  • Bala N, Napiah M, Kamaruddin I (2020) Nano-silica composite asphalt mixtures performance-based design and optimisation using response surface methodology. Int J Pavement Eng 21(1):29–40

    Google Scholar 

  • Becker Y, Mendez MP, Rodriguez Y (2001) Polymer modified asphalt. Vis Tecnol 9(1):39–50

    Google Scholar 

  • Behnood A, Gharehveran MM (2019) Morphology, rheology, and physical properties of polymer-modified asphalt binders. Eur Polym J 112:766–791

    Google Scholar 

  • Bhasin A, Little DN (2009) Application of microcalorimeter to characterize adhesion between asphalt binders and aggregates. J Mater Civ Eng 21(6):235–243

    Google Scholar 

  • Bhat FS, Mir MS (2021) A study investigating the influence of nano Al2O3 on the performance of SBS modified asphalt binder. Constr Build Mater 271:121499

    Google Scholar 

  • Brsileiro L, Moreno-Navarro F, Tauste-Martínez R, Matos J, Rubio-Gámez MDC (2019) Reclaimed polymers as asphalt binder modifiers for more sustainable roads: a review. Sustainability 11(3):646

    Google Scholar 

  • Cheng Y, Han H, Fang C, Li H, Huang Z, Su J (2020) Preparation and properties of nano-CaCO3/waste polyethylene/styrene-butadiene-styrene block polymer-modified asphalt. Polym Compos 41(2):614–623

    Google Scholar 

  • Chrissafis KKM, Paraskevopoulos GZ, Papageorgiou DN, Bikiaris DN (2008) Thermal and dynamic mechanical behavior nanoparticles dispersed in poly-vinyl-alcohol). J Appl Polym Sci 110:1739–1749

    Google Scholar 

  • Costa LM, Silva HM, Peralta J, Oliveira JR (2019) Using waste polymers as a reliable alternative for asphalt binder modification–Performance and morphological assessment. Constr Build Mater 198:237–244

    Google Scholar 

  • Cox BC, Smith BT, Howard IL, James RS (2017) State of knowledge for Cantabro testing of dense graded asphalt. J Mater Civ Eng 29(10):04017174

    Google Scholar 

  • Di Benedetto H et al (2004) Fatigue of bituminous mixtures. Mater Struct 37(3):202–216

    Google Scholar 

  • Doyle JD, Howard IL (2016) Characterization of dense-graded asphalt with the Cantabro Test. J Test Eval 44(1):77–88

    Google Scholar 

  • Du Z, Jiang C, Yuan J, Xiao F, Wang J (2020) Low temperature performance characteristics of polyethylene modified asphalts–a review. ConstrBuild Mater 264:120704

    Google Scholar 

  • Durrieu F, Fabienne F, Mouillet VM (2007) The influence of UV aging of a styrene/butadiene/styrene modified bitumen: comparison between laboratory and on site aging. Fuel 86(10):1446–1451

    Google Scholar 

  • EniebDiab MDA (2017) Characteristics of asphalt binder and mixture containing nanosilica. Int J Pavement Res Technol 10:148–157

    Google Scholar 

  • Fang C, Wu C, Hu J, Yu R, Zhang Z, Nie L, Zhou S, Mi X (2014) Pavement properties of asphalt modified with packaging-waste polyethylene. J Vinyl Addit Technol 20(1):31–35

    Google Scholar 

  • Galooyak SS, Dabir B, Nazarbeygi AE, Moeini A (2010) Rheological properties and storage stability of bitumen/SBS/montmorillonite composites. Constr Build Mater 24(3):300–307

    Google Scholar 

  • Gama DA, Yan Y, Rodrigues JKG, Roque R (2018) Optimizing the use of reactive terpolymer, polyphosphoric acid and high-density polyethylene to achieve asphalt binders with superior performance. Constr Build Mater 169:522–529

    Google Scholar 

  • Ghanoon SA, Tanzadeh J, Mirsepahi M (2020) Laboratory evaluation of the composition of nano-clay, nano-lime and SBS modifiers on rutting resistance of asphalt binder. Constr Build Mater 238:117592

    Google Scholar 

  • Giustozzi F, Crispino M, Toraldo E, Mariani E (2015) Mix design of polymer-modified and fiber-reinforced warm-mix asphalts with high amount of reclaimed asphalt pavement: achieving sustainable and high-performing pavements. Transp Res Rec 2523(1):3–10

    Google Scholar 

  • Gorkem C, Sengoz B (2009) Predicting stripping and moisture induced damage of asphalt concrete prepared with polymer modified bitumen and hydrated lime. Constr Build Mater 23(6):2227–2236

    Google Scholar 

  • Hamedi GH, Nejad FM, Oveisi K (2016) Estimating the moisture damage of asphalt mixture modified with nano zinc oxide. Mater Struct 49:1165–1174

    Google Scholar 

  • Hınıslıoğlu S, Ağar E (2004) Use of waste high density polyethylene as bitumen modifier in asphalt concrete mix. Mater Lett 58(3–4):267–271

    Google Scholar 

  • Iran highway asphalt paving code (2012) Vice Presidency for Strategic Planning and Supervision. The Ministry of Road and Urban Development, Publication Number 234, Iran

  • Kakar MR, Mikhailenko P, Piao Z, Bueno M, Poulikakos L (2021) Analysis of waste polyethylene (PE) and its by-products in asphalt binder. Constr Build Mater 280:122492

    Google Scholar 

  • Kumar A, Choudhary R, Kandhal PS, Julaganti A, Behera OP, Singh A, Kumar R (2020) Fatigue characterisation of modified asphalt binders containing warm mix asphalt additives. Road Mater Pavement Des 21(2):519–541

    Google Scholar 

  • Lazzara G, Milioto S (2010) Dispersions of nanosilica in biocompatible copolymers. Polym Degrad Stab 95(4):610–617

    Google Scholar 

  • Lewandowski LH (1994) Polymer modification of paving asphalt binders. Rubber Chem Technol 67(3):447–480

    Google Scholar 

  • Li R et al (2017) Developments of nano-materials and technologies on asphalt materials – a review. Constr Build Mater 143:633–648

    Google Scholar 

  • Li S, Xu W, Zhang F, Wu H, Zhao P (2022) Effect of graphene oxide on the low-temperature crack resistance of polyurethane–SBS-modified asphalt and asphalt mixtures. Polymers 14(3):453

    Google Scholar 

  • Lin P, Huang W, Li Y, Tang N, Xiao F (2017) Investigation of influence factors on low temperature properties of SBS modified asphalt. Constr Build Mater 154:609–622

    Google Scholar 

  • Mahali I, Sahoo UC (2019) Rheological characterization of nanocomposite modified asphalt binder. Int J Pavement Res Technol 12(6):589–594

    Google Scholar 

  • Mamun AA, Arifuzzaman M (2018) Nano-scale moisture damage evaluation of carbon nanotube-modified asphalt. Constr Build Mater 193:268–275

    Google Scholar 

  • Mamuye Y, Do ND, Liao MC (2017) Nano-Al2o3 composite on intermediate and high temperature properties of neat and modified asphalt binders and their effect on hot mix asphalt mixtures. Constr Build Mater 331:127304

    Google Scholar 

  • Masad E, Roja KL, Rehman A, Abdala A (2020) A review of asphalt modification using plastics: a focus on polyethylene. Texas A&M University, Qatar, Doha

    Google Scholar 

  • Moussa GS, Abdel-Raheem A, Abdel-Wahed T (2021) Effect of nanoclay particles on the performance of high-density polyethylene-modified asphalt concrete mixture. Polymers 13(3):434

    Google Scholar 

  • Napierska D, Thomassen LC, Lison D, Martens JA, Hoet PH (2010) The nanosilica hazard: another variable entity. Part Fibre Toxicol 7(1):1–32

    Google Scholar 

  • Nizamuddin S, Jamal M, Gravina R, Giustozzi F (2020) Recycled plastic as bitumen modifier: the role of recycled linear low-density polyethylene in the modification of physical, chemical and rheological properties of bitumen. J Clean Prod 266:121988

    Google Scholar 

  • Nuñez JYM, Domingos MDI, Faxina AL (2014) Susceptibility of low-density polyethylene and polyphosphoric acid-modified asphalt binders to rutting and fatigue cracking. Constr Build Mater 73:509–514

    Google Scholar 

  • Obaid HA (2021) Characteristics of warm mixed asphalt modified by waste polymer and NS. Int J Pavement Res Technol 14(3):397–401

    Google Scholar 

  • Othman AM (2010) Effect of low-density polyethylene on fracture toughness of asphalt concrete mixtures. J Mater Civ Eng 22(10):1019–1024

    Google Scholar 

  • Padhan RK, Sreeram A (2018) Enhancement of storage stability and rheological properties of polyethylene (PE) modified asphalt using cross linking and reactive polymer based additives. Constr Build Mater 188:772–780

    Google Scholar 

  • Pérez-Jiménez FE, Calzada-Pérez MA (1990) Analysis and evaluation of the performance of porous asphalt: the spanish experience surface characteristics of roadways. Int J Eng Res. https://doi.org/10.1520/STP23386S

    Article  Google Scholar 

  • Pérez-Lepe A, Martínez-Boza FJ, Attané P, Gallegos C (2006) Destabilization mechanism of polyethylene-modified bitumen. J Appl Polym Sci 100(1):260–267

    Google Scholar 

  • Punith VS, Veeraragavan AJJ (2007) Behavior of asphalt concrete mixtures with reclaimed polyethylene as additive. J Mater Civ Eng 19(6):500–507

    Google Scholar 

  • Punith VS, Veeraragavan A (2011) Behavior of reclaimed polyethylene modified asphalt cement for paving purposes. J Mater Civ Eng 23(6):833–845

    Google Scholar 

  • Quercia G, Brouwers HJH (2010) Application of nano-silica (nS) in concrete mixtures. In: 8th fib PhD symposium in Kgs, Lyngby, Denmark (pp 431–436)

  • Singh B, Kumar L, Gupta M, Chauhan GS (2013) Polymer-modified bitumen of recycled LDPE and maleated bitumen. J Appl Polym Sci 127(1):67–78

    Google Scholar 

  • Tabatabaee HA, Clopotel C, Arshadi A, Bahia H (2013) Critical problems with using the asphalt ductility test as a performance index for modified binders. Transp Res Rec 2370(1):84–91

    Google Scholar 

  • Wang Y, Kalinina A, Sun T, Nowack B (2016) Probabilistic modeling of the flows and environmental risks of nano-silica. Sci Total Environ 545:67–76

    Google Scholar 

  • Xiao F, Amirkhanian S, Wang H, Hao P (2014) Rheological property investigations for polymer and polyphosphoric acid modified asphalt binders at high temperatures. Constr Build Mater 64:316–323

    Google Scholar 

  • Yan C, Yuan L, Yu X, Ji S, Zhou Z (2022) Characterizing the fatigue resistance of multiple modified asphalts using time sweep test, LAS test and elastic recovery test. Constr Build Mater 322:125806

    Google Scholar 

  • Yang J, Tighe S (2013) Procedia – Social and Behavioral Sciences. In: Paper presented at the Intelligent and Integrated Sustainable Multimodal Transportation Systems Proceedings from the 13th COTA International Conference of Transportation Professionals (CICTP2013). Shenzhen, China. Volume 96, 6 November, 1269–1276.

  • Yao H, You ZH, Li L, Shi X, Goh S, Mills-beale J, Wingard D (2012a) Performance of asphalt binder blended with non-modified and polymer-modified nanoclay. Constr Build Mater 35:159–170

    Google Scholar 

  • Yao H, You Z, Li L, Lee CH, Wingard D, Yap YK et al (2012b) Rheological properties and chemical bonding of asphalt modified with nanosilica. J Mater Civ Eng 25(2012):1619–1630

    Google Scholar 

  • You Z et al (2011) Nanoclay-modified asphalt materials: preparation and characterization. Constr Build Mater 25(2):1072–1078

    Google Scholar 

  • Yu JY, Zhang HL, Sun P, Zhao SF (2020) Laboratory performances of nano-particles/polymer modified asphalt mixtures developed for the region with hot summer and cold winter and field evaluation. Road Mater 21(6):1529–1544

    Google Scholar 

  • Zhang F, Hu C (2016) The research for crumb rubber/waste plastic compound modified asphalt. J Therm Anal Calorim 124(2):729–741

    Google Scholar 

  • Zhang Y, Luo R, Lytton RL (2011) Characterizing permanent deformation and fracture of asphalt mixtures by using compressive dynamic modulus tests. J Mater Civ Eng 24(7):898–906

    Google Scholar 

  • Zhang Q, Khan MU, Lin X, Yi W, Lei H (2020) Green-composites produced from waste residue in pulp and paper industry: A sustainable way to manage industrial wastes. J Clean Prod 262:121251

    Google Scholar 

  • Zoorob SE, Suprama LB (2000) Laboratory design and investigation of the properties of continuously graded asphaltic concrete containing recycled plastics aggregate replacement (Plastiphalt). Cement Concr Compos 22(2000):233–242

    Google Scholar 

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Correspondence to Hasan taherkhani.

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Arshadi, M., taherkhani, H. The Effects of Nano-silica Addition on the Physical Properties of Polyethylene-Modified Asphalt Binder and the Mechanical Properties and Durability of Asphalt Mixtures. Iran J Sci Technol Trans Civ Eng 47, 4103–4116 (2023). https://doi.org/10.1007/s40996-023-01196-6

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