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Energy Dissipation Pathway Control in Polymer Derived Ceramic (PDC) Composites

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Abstract

Ceramics are brittle due in large part to the limited availability of energy dissipation pathways when they are subjected to an impact load. The primary avenue for improving the material reliability and energy-absorption capability is to create new energy dissipation mechanisms that can be used to replace or minimize the kinetic energy associated with the debris shattering. In this paper, a computational framework is developed to investigate the relationship between phase composition and energy dissipation pathways in polymer derived ceramic (PDC) composites by accounting for the key processing parameters and deformation/failure mechanisms. It is found that the phase composition that promotes both the Mullins effect and the ligament bridging mechanism can significantly improve the structural integrity of the composite material. A fundamental understanding of how to redistribute the impact energy dissipation in a controllable path would hold great promise for fabricating PDC composites with tailored properties.

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References

  1. Colombo P, Mera G, Riedel R, Sorarù GD (2010) Polymer-derived ceramics: 40 years of research and innovation in advanced ceramics. J Am Ceram Soc 93(7):1805–1837

    CAS  Google Scholar 

  2. Mitchell T, Lagerlöf KP (1985) Dislocations in ceramics. Mater Sci Technol 1:944–949

    Article  CAS  Google Scholar 

  3. Osnes K, Holmen JK, Hopperstad OS, Børvik T (2019) Fracture and fragmentation of blast-loaded laminated glass: an experimental and numerical study. Int J Impact Eng 132:103334

    Article  Google Scholar 

  4. Yadav S, Ravichandran G (2003) Penetration resistance of laminated ceramic/polymer structures. Int J Impact Eng 28(5):557–574

    Article  Google Scholar 

  5. Tan G, Yu Q, Liu Z, Wang X, Zhang M, Liu Y, Zhang Z, Ritchie RO (2021) Compression fatigue properties and damage mechanisms of a bioinspired nacre-like ceramic-polymer composite. Scr Mater 203:114089

    Article  CAS  Google Scholar 

  6. Grujicic M, Ramaswami S, Snipes J (2016) Nacre-like ceramic/polymer laminated composite for use in body-armor applications. AIMS Mater Sci 3:83–113

    Article  CAS  Google Scholar 

  7. Eckel ZC, Zhou C, Martin JH, Jacobsen AJ, Carter WB, Schaedler TA (2016) Additive manufacturing of polymer-derived ceramics. Science 351(6268):58–62

    Article  CAS  Google Scholar 

  8. Kulkarni A, Sorarù GD, Pearce JM (2020) Polymer-derived SiOC replica of material extrusion-based 3-D printed plastics. Addit Manuf 32:100988

    CAS  Google Scholar 

  9. Konstantinou G, Kakkava E, Hagelüken L, Sasikumar PVW, Wang J, Makowska MG, Blugan G, Nianias N, Marone F, Van Swygenhoven H (2020) Additive micro-manufacturing of crack-free PDCs by two-photon polymerization of a single, low-shrinkage preceramic resin. Addit Manuf 35:101343

    CAS  Google Scholar 

  10. Jambe B, Marchand-Brynaert J, Devaux J (1995) Thermal degradation of poly(methyl-n-hexylsilylene). J Polym Sci A 33(8):1283–1292

    Article  CAS  Google Scholar 

  11. Francis A (2018) Progress in polymer-derived functional silicon-based ceramic composites for biomedical and engineering applications. Mater Res Express 5(6):062003

    Article  Google Scholar 

  12. Bernard S, Fiaty K, Cornu D, Miele P, Laurent P (2006) Kinetic modeling of the polymer-derived ceramics route: investigation of the thermal decomposition kinetics of poly [B-(methylamino) borazine] precursors into boron nitride. J Phys Chem B 110(18):9048–9060

    Article  CAS  Google Scholar 

  13. Ma C, Li Y (2022) Modeling of phase transition in fabrication of polymer-derived ceramics (PDCs). Int J Comput Mater Sci Eng 11(02):2150032

    CAS  Google Scholar 

  14. Stabler C, Reitz A, Stein P, Albert B, Riedel R, Ionescu E (2018) Thermal properties of SiOC glasses and glass ceramics at elevated temperatures. Materials 11(2):279

    Article  Google Scholar 

  15. Contact constraint enforcement methods in Abaqus/Explicit, https://abaqus-docs.mit.edu/2017/English/SIMACAEITNRefMap/simaitn-c-expcontactconstraints.htm.

  16. Diani J, Fayolle B, Gilormini P (2009) A review on the Mullins effect. Eur Polymer J 45(3):601–612

    Article  CAS  Google Scholar 

  17. Ma C, Ji T, Robertson CG, Rajeshbabu R, Zhu J, Dong Y (2017) Molecular insight into the Mullins effect: irreversible disentanglement of polymer chains revealed by molecular dynamics simulations. Phys Chem Chem Phys 19(29):19468–19477

    Article  CAS  Google Scholar 

  18. Hohenberger TW, Windslow RJ, Pugno NM, Busfield JJC (2019) A constitutive model for both low and high strain nonlinearities in highly filled elastomers and implementation with user-defined material subroutines in ABAQUS. Rubber Chem Technol 92(4):653–686

    Article  CAS  Google Scholar 

  19. Hanson DE, Hawley M, Houlton R, Chitanvis K, Rae P, Orler EB, Wrobleski DA (2005) Stress softening experiments in silica-filled polydimethylsiloxane provide insight into a mechanism for the Mullins effect. Polymer 46(24):10989–10995

    Article  CAS  Google Scholar 

  20. Volokh KY (2007) Hyperelasticity with softening for modeling materials failure. J Mech Phys Solids 55(10):2237–2264

    Article  CAS  Google Scholar 

  21. Kim TK, Kim JK, Jeong OC (2011) Measurement of nonlinear mechanical properties of PDMS elastomer. Microelectron Eng 88(8):1982–1985

    Article  CAS  Google Scholar 

  22. Shahriari M, Saeidi Googarchin H (2020) Numerical investigation of the impact fracture performance of a composite laminated windshield considering the Park-Paulinho-Roesler cohesive zone model. Compos Struct 249:112568

    Article  Google Scholar 

  23. Moysan C, Riedel R, Harshe R, Rouxel T, Augereau F (2007) Mechanical characterization of a polysiloxane-derived SiOC glass. J Eur Ceram Soc 27(1):397–403

    Article  CAS  Google Scholar 

  24. Vashisth A, Khatri S, Hahn SH, Zhang W, Van Duin ACT, Naraghi M (2019) Mechanical size effects of amorphous polymer-derived ceramics at the nanoscale: experiments and ReaxFF simulations. Nanoscale 11(15):7447–7456

    Article  CAS  Google Scholar 

  25. To T, Stabler C, Ionescu E, Riedel R, Célarié F, Rouxel T (2020) Elastic properties and fracture toughness of SiOC-based glass-ceramic nanocomposites. J Am Ceram Soc 103(1):491–499

    Article  CAS  Google Scholar 

  26. Shahriari M, Googarchin HS (2020) Numerical investigation of the impact fracture performance of a composite laminated windshield considering the Park-Paulinho-Roesler cohesive zone model. Compos Struct 249:112568

    Article  Google Scholar 

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Acknowledgements

The authors acknowledge the support from NH BioMade Project that is provided by the National Science Foundation's Research Infrastructure Improvement Award # 1757371, as well as the start-up funds from Thayer School of Engineering at Dartmouth College.

Funding

Funding was provided by National Science Foundation (Grant Number 1757371) and Thayer School of Engineering at Dartmouth College (Start-up funding).

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Correspondence to Y. Li.

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Li, Y., Ma, C. & Larkin, K. Energy Dissipation Pathway Control in Polymer Derived Ceramic (PDC) Composites. J. dynamic behavior mater. 8, 405–417 (2022). https://doi.org/10.1007/s40870-022-00344-9

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  • DOI: https://doi.org/10.1007/s40870-022-00344-9

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