Abstract
The annual CLEERS conference sponsored by the U.S. Department of Energy and organized by the Oak Ridge National Laboratory was held in Ann Arbor, MI, 18–20 September 2018. It brought together emission control scientists, engineers, and investigators from academia, national labs, and industry from across the U.S. and abroad, discussing the latest emission control technologies, trends, challenges, and regulations. Presentations, deliberations, exchanges, and panel discussions displayed a much-needed focus on the latest up-and-coming approaches to further advance NOx reduction, a major remaining challenge especially in diesel emission control, using further advances in selective catalytic reduction (SCR) of NOx, passive NOx adsorbers, lean NOx traps, and SCR on particulate filter, amongst others. Discussions were further held on diesel oxidation catalysts, gasoline particulate filters, three-way catalysts, and hydrocarbon SCR, and also on the latest catalyst washcoat technologies, materials, and catalytic processes such as diffusion and kinetics, testing, and computer simulations.
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Abbreviations
- BEA:
-
Beta polymorph A—one of various zeolite types
- CHA:
-
Chabazite—one of various zeolite types, also SSZ-13 (a synthetic type of CHA)
- DFT:
-
Density functional theory
- DOC:
-
Diesel oxidation catalyst
- E10:
-
Fuel blended with 9–10% ethanol
- FTP:
-
Federal test protocol
- GPF:
-
Gasoline particulate filter
- HC:
-
Hydrocarbon
- LNT:
-
Lean NOx trap
- LTNA:
-
Low-temperature NOx adsorber
- TWC:
-
Three-way catalyst
- NOx :
-
Nitrogen oxides: NO, NO2, etc.
- NEDC:
-
New European drive cycle
- NMR:
-
Nuclear magnetic resonance
- PEMS:
-
Portable emission measurement system
- PM:
-
Particulate matter (in diesel emission)
- QENS:
-
Quasielastic neutron scattering
- SI:
-
(SI engine) Spark-ignition
- TG:
-
Thermogravimetry
- TPR:
-
Temperature-programmed reaction
- C2, C3, Cx :
-
Refers to Cx as in CxHy components in diesel fuel and gasoline
- DRIFTS:
-
Diffuse reflectance infrared Fourier transform spectroscopy
- DPF:
-
Diesel particulate filter
- FTIR:
-
Fourier transform infrared spectroscopy
- FWC:
-
Four-way catalyst (also called GPF)
- H2O:
-
Water
- HPLC:
-
High-performance liquid chromatography
- LO:
-
Light-off
- SCR:
-
Selective catalytic reduction
- MOC:
-
Methane oxidation catalyst
- N2O:
-
Nitrous oxide, a potent greenhouse gas
- NH3 :
-
Ammonia
- OBD:
-
Onboard diagnostics
- PGM:
-
Platinum group metal
- PNA:
-
Passive NOx adsorber
- SDPF:
-
Combined SCR-DPF (also called SCRF)
- T50:
-
Temperature for 50% catalytic efficiency
- TPD:
-
Temperature-programmed desorption
References
Hammershøi, P.S., Vennestrøm, P.N.R., Falsig, H., Jensen, A.D., Janssens, T.V.W.: Importance of the Cu oxidation state for the SO2-poisoning of a Cu-SAPO-34 catalyst in the NH3-SCR reaction. Appl. Catal. B Environ. 236, 377–383 (2018). https://doi.org/10.1016/j.apcatb.2018.05.038
Hammershøi, P.S., Jensen, A.D., Janssens, T.V.W.: Impact of SO2-poisoning over the lifetime of a Cu-CHA catalyst for NH3–SCR. Appl. Catal. B Environ. 238, 104–110 (2018). https://doi.org/10.1016/j.apcatb.2018.06.039
Acknowledgments
Professor Andrea Strzelec (Mississippi State University) and Dr. Se Oh (General Motors R&D) contributed to “In the Memory of Dr. Dick Blint.” Their input is hereby appreciated.
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Most presentations of speakers could be found at https://cleers.org/event/2018-cleers-workshop.
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Masoudi, M., Hensel, J. & Tegeler, E. A Review of the 2018 U.S.-DOE CLEERS Conference: Trends and Deeper Insights in Reduction of NOx and Particulate in Diesel and Gasoline Engines and Advances in Catalyst Materials, Mechanisms, and Emission Control Technologies. Emiss. Control Sci. Technol. 6, 113–125 (2020). https://doi.org/10.1007/s40825-019-00134-1
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DOI: https://doi.org/10.1007/s40825-019-00134-1