Abstract
A simplified experimental device was used to reveal the dispersed phase droplet formation process in the circumferential shear flow of a liquid–liquid cyclone reactor. Fluorescent oil and deionized water were selected as the dispersed phase and continuous phase, respectively. And the highlight of fluorescent oil under ultra-violet was applied to capture the droplet dynamic behavior. It was found that three droplet formation regimes were observed, including dripping regime, dripping-to-jetting transition regime and jetting regime. Besides, the results indicate that the order of droplet formation speed in three regimes is jetting regime, dripping-jetting transition regime and dripping regime. Moreover, two critical inlet flow rate of dispersed phase were used to characterize the transitions between regimes, which both decreased with the increase in inlet flow rate of continuous phase. But the different reduction rates of them indicate that the transition from dripping regime to jetting regime is faster at greater inlet flow rate of continuous phase. In addition, the typical droplet size distributions in three regimes indicate the size uniformity of droplets formed in dripping regime is better than that in jetting regime and dripping-to-jetting transition regime. However, with the comprehensive consideration of size, uniformity and formation speed, jetting regime is preferred.
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig1_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig2_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig3_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig4_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig5_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig6_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig7_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig8_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig9_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig10_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig11_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig12_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs40430-022-03960-7/MediaObjects/40430_2022_3960_Fig13_HTML.png)
Similar content being viewed by others
References
Zhang K, Liu JW, Liu WC, Yang JK (2011) Preparation of glass-ceramics from molten steel slag using liquid-liquid mixing method. Chemosphere 85(4):689–692
Cheng D, Feng X, Cheng JC, Yang C (2013) Numerical simulation of macro-mixing in liquid-liquid stirred tanks. Chem Eng Sci 101:272–282
Shen YY, Qin B, Li X, Zhu ZY, Cui PZ, Gao J, Wang YL (2020) Investigation of the flow characteristics of liquid-liquid two-phase mixing in an agitator equipped with a V-shaped horizontal baffle. Environ Dev Sustain 23:2298–2313
Maluta F, Montante G, Paglianti A (2020) Analysis of immiscible liquid-liquid mixing in stirred tanks by electrical resistance tomography. Chem Eng Sci 227:115898
Siddiqui SW, Norton IT (2012) Oil-in-water emulsification using confined impinging jets. J Colloid Interface Sci 377(1):213–221
Gholami A, Pourfayaz F, Hajinezhad A, Mohadesi M (2019) Biodiesel production from Norouzak (Salvia leriifolia) oil using choline hydroxide catalyst in a microchannel reactor. Renew Energy 136:993–1001
Noriega MA, Narváez PC (2020) Scale-up and cost analysis of biodiesel production using liquid-liquid film reactors: Reduction in the methanol consumption and investment cost. Energy 211:118724
Liu ZC, Meng XH, Zhang R, Xu CM, Dong H, Hu YF (2014) Reaction performance of isobutane alkylation catalyzed by a composite ionic liquid at a short contact time. AIChE J 60(6):2244–2253
Zhang MY, Zhang TY, Wang ZB, Zhu LY, Jin YH (2017) Mixing and separation of liquid-liquid two-phase in a novel cyclone reactor of isobutane alkylation catalyzed by ionic liquid. Powder Technol 316:289–295
Fuster D, Bagué A, Boeck T, Moyne LL, Leboissetier A, Popinet S, Ray P, Scardovelli R, Zaleski S (2009) Simulation of primary atomization with an octree adaptive mesh refinement and VOF method. Int J Multiph Flow 35(6):550–565
Shinjo J, Umemura A (2010) Simulation of liquid jet primary breakup: dynamics of ligament and droplet formation. Int J Multiph Flow 36(7):513–532
Duarte BADF, Barbi F, Villar MM, Serfaty R, Neto ADS (2020) Primary atomization of a turbulent liquid jet in crossflow: a comparison between VOF and FGVT methods. J Braz Soc Mech Sci Eng 42(6):277
Soni SK, Kolhe PS (2020) Liquid jet breakup and spray formation with annular swirl air. Int J Multiph Flow 134:103474
Xiao F, Wang ZG, Sun MB, Liang JH, Liu N (2016) Large eddy simulation of liquid jet primary breakup in supersonic air crossflow. Int J Multiph Flow 87:229–240
Wu LY, Chen YP (2014) Visualization study of emulsion droplet formation in a coflowing microchannel. Chem Eng Process 85:77–85
Kovalchuk NM, Roumpea E, Nowak E, Chinaud M, Angeli P, Simmons MJH (2018) Effect of surfactant on emulsification in microchannels. Chem Eng Sci 176:139–152
Liu Y, Zhang T, Lv L, Chen Y, Tang S (2020) Mass transfer and droplet formation regime in a countercurrent mini-channel extractor. Chem Eng J 402:125383
Kékesi T, Amberg G, Wittberg LP (2016) Drop deformation and breakup in flows with shear. Chem Eng Sci 140:319–329
Komrakova AE, Shardt O, Eskin D, Derksen JJ (2014) Lattice Boltzmann simulations of drop deformation and breakupin shear flow. Int J Multiph Flow 59:24–43
Zhao GY, Pan DY, Zeng LF, Shao XM (2021) Numerical study on droplet deformation in periodic pulsatile shear flow and effects of inertia. J Nonnewton Fluid Mech 289:104494
Li J, Renardy YY, Renardy M (2000) Numerical simulation of breakup of a viscous drop in simple shear flow through a volume-of-fluid method. Phys Fluids 12:269–282
Liang WJ, Wang DF, Cai ZQ, Li ZP, Huang XB, Gao ZM, Derksen JJ, Komrakova AE (2020) Deformation and breakup of single drop in laminar and transitional jet flows. Chem Eng J 386:121812
Zhang MY, Liu XZ, Zhang CC, Li XY, Zhang H, Tan ZW, Zhang LH, Wang ZB (2021) Numerical investigation of shear flow structure induced by guided vane in a liquid-liquid cyclone reactor. Chem Eng Process Process Intensif 167:108521
Zhang MY, Zhu LY, Wang ZB, Liu ZC, Liu ZZ, Xu CM, Jin YH (2017) Flow field in a liquid-liquid cyclone reactor for isobutane alkylation catalyzed by ionic liquid. Chem Eng Res Des 125:282–290
Zhang MY, Wang L, Zhu LY, Wang ZB, Liu ZC, Jin YH (2017) Phase holdup distribution and dispersion performance in a novel liquid-liquid cyclone reactor of isobutane alkylation catalyzed by ionic liquid. Chem Eng Res Des 125:257–264
Pereira NE, Ni X (2001) Droplet size distribution in a continuous oscillatory baffled reactor. Chem Eng Sci 56(3):735–739
Zhang MY, Li AJ, Zhu LY, Wang ZB, Liu ZC, Jin YH (2019) A novel liquid-liquid cyclone reactor for ionic liquid catalyzed isobutene alkylation: cold model investigation of the dispersed phase droplet size distribution. Sep Purif Technol 209:375–382
Acknowledgements
The authors gratefully acknowledge the support from the National Natural Science Foundation of China (No. 22208194), the Natural Science Foundation of Shandong Province (No. ZR2020QE204) and the Doctoral Research Fund of Shandong Jianzhu University (No. X18068Z).
Author information
Authors and Affiliations
Corresponding authors
Additional information
Technical Editor: Erick Franklin.
Publisher's Note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Rights and permissions
Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.
About this article
Cite this article
Zhang, M., Chen, J., Tang, M. et al. Visualization investigation of dispersed phase droplet formation regimes in a circumferential shear flow composed of immiscible liquid. J Braz. Soc. Mech. Sci. Eng. 45, 62 (2023). https://doi.org/10.1007/s40430-022-03960-7
Received:
Accepted:
Published:
DOI: https://doi.org/10.1007/s40430-022-03960-7