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Effects of MgO ceramic filler on microwave dielectric properties of MgO/polymers (polytetrafluoroethylene, polypropylene, polystyrene) composites

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Abstract

The microwave dielectric properties of MgO/polytetrafluoroethylene (PTFE), polypropylene (PP), and polystyrene (PS) composites were investigated as a function of the MgO content and crystallinity of the polymers. MgO powders were prepared by two-step heat treatment. Ceramic polymer composites were prepared with 0.1–0.5 volume fractions (Vf) MgO filler dispersed on three types of polymer matrices using the hot-moulding technique. With the increase in the MgO content, the dielectric constants (K) of the composites increased owing to the decrease in the interparticle distance between the MgO ceramics and higher K of MgO (9.61) than those of PTFE (2.14), PP (3.05), and PS (3.40). Several theoretical models were employed to predict the effective K of the composite. The predicted values were compared to experimental data. With the increase in the MgO content, the quality factor (Q × f) of the composites decreased owing to the increase in the blocking effect. In particular, the MgO/PP composite with Vf of MgO of 0.1 exhibited a higher Q × f (48,330 GHz) than those of the MgO/PS and MgO/PTFE composites with Vf of MgO of 0.1.

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References

  1. M. Ma, K. Song, Y. Ji, F. Hussain, A. Khesro, M. Mao, L. Xue, P. Xu, B. Liu, Z. Lu, D. Zhou, D. Wang, S. Sun, Ceram. Int. 47, 19241–19246 (2021)

    Google Scholar 

  2. R. Peng, H. Su, Y. Li, Y. Lu, C. Yu, L. Shi, D. Chen, B. Liao, J. Alloys Compd. 868, 159006 (2021)

    Article  Google Scholar 

  3. D.H. Im, C.J. Jeon, E.S. Kim, Ceram. Int. 38, 191–195 (2012)

    Article  Google Scholar 

  4. A.S. Luyt, J.A. Molefi, H. Krump, Polym. Degrad. Stabil. 91, 1629–1636 (2006)

    Article  Google Scholar 

  5. W. Zhou, Thermochim. Acta. 512, 1–2 (2011)

    Article  Google Scholar 

  6. T. Hu, J. Juuti, H. Jantunen, T. Vilkman, J. Eur. Ceram. Soc. 27, 13–15 (2007)

    Article  Google Scholar 

  7. J.Y. Chen, W.H. Hsu, C.L. Huang, J. Alloys Compd. 504, 284–287 (2010)

    Article  Google Scholar 

  8. E.S. Kim, C.J. Jeon, IEEE Trans. Ultrason. Ferroelectr. Freq. Control 58, 1939–1946 (2011)

    Google Scholar 

  9. S. Rajesh, K.P. Murali, R. Ratheesh, Polym. Compos. 30, 1480–1485 (2009)

    Article  Google Scholar 

  10. Y.C. Chen, H.C. Lin, Y.D. Lee, J. Polym. Res. 10, 247–258 (2003)

    Google Scholar 

  11. G. Sui, S. Jana, W.H. Zhong, M.A. Fuqua, C.A. Ulven, Acta Mater. 56, 2381–2388 (2008)

    Article  Google Scholar 

  12. F. Lanyi, N. Wenzke, J. Kaschta, D.W. Schubert, Adv. Eng. Mater. 22, 1900796 (2019)

    Google Scholar 

  13. H.W. Starkweather, P. Zoller, G.A. Jones, A.J. Vega, J. Polym. Sci. B: Polym. Phys. 20, 751–761 (1982)

    Google Scholar 

  14. B.W. Hakki, P.D. Coleman, I.R.E. Trans, Microwave Theor. Tech. 8, 402–410 (1960)

    Article  Google Scholar 

  15. T. Nishikawa, K. Wakino, H. Tamura, H. Tanaka, Y. Ishikawa, IEEE MTT-S Int. Microw. Symp. Dig. 87, 277–280 (1987)

    Article  Google Scholar 

  16. P.S. Anjana, M.T. Sebastian, M.N. Suma, P. Mohanan, Int. J. Appl. Ceram. Technol. 5, 325–333 (2008)

    Google Scholar 

  17. H.Y. Hwang, S.K. Jeoung, J.H. Shin, J.M. Kim, K.Y. Lee, Polymer (Korea) 34, 352–356 (2010)

    Google Scholar 

  18. S. George, V.N. Deepu, P. Mohanan, M.T. Sebastian, Polym. Eng. Sci. 50, 570–576 (2010)

    Article  Google Scholar 

  19. Z. Cai, X. Wang, B. Luo, W. Hong, L. Li, Compos. Sci. Technol. 145, 105–113 (2017)

    Google Scholar 

  20. P.S. Anjana, M.T. Sebastian, M.N. Suma, P. Mohanan, Int. J. Appl. Ceram. Technol. 5, 325–333 (2008)

    Article  Google Scholar 

  21. C.J. Jeon, E.S. Kim, Jpn. J. Appl. Phys. 51, 111502 (2012)

    Article  ADS  Google Scholar 

  22. C.J. Jeon, E.S. Kim, J. Adv. Dielectr. 1, 127–134 (2011)

    Google Scholar 

  23. C.J. Jeon, E.S. Kim, Ferroelectrics 434, 27–36 (2012)

    Article  ADS  Google Scholar 

  24. S. Thomas, V.N. Deepu, P. Mohanan, M.T. Sebastian, J. Am. Ceram Soc. 91, 1971–1975 (2008)

    Article  Google Scholar 

  25. S.C. Tjong, G.D. Liang, S.P. Bao, Polym. Eng. Sci. 48, 177–183 (2008)

    Article  Google Scholar 

  26. M.T Sebastian, H. Jantunen, Int. J. Appl. Ceram. Technol. 7, 415–434 (2010)

    Google Scholar 

  27. G. Subodh, C. Pavithran, P. Mohanan, M.T. Sebastian, J. Eur. Ceram. Soc. 27, 3039–3044 (2007)

    Article  Google Scholar 

  28. K.S. Deepa, M.T. Sebastian, J. James, Appl. Phys. Lett. 91, 202904 (2007)

    Article  Google Scholar 

Download references

Acknowledgements

This work was supported by Kyonggi University Graduate Research Assistantship 2022.

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Correspondence to Eung Soo Kim.

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Jeong, J.Y., Kim, E.S. Effects of MgO ceramic filler on microwave dielectric properties of MgO/polymers (polytetrafluoroethylene, polypropylene, polystyrene) composites. J. Korean Phys. Soc. 82, 81–90 (2023). https://doi.org/10.1007/s40042-022-00683-9

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  • DOI: https://doi.org/10.1007/s40042-022-00683-9

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