Abstract
Air pollution is one of the main environmental problems in the metropolitan area of São Paulo (MASP) in Brazil, with frequent exceedances of air quality standards. Occasionally, the exceedance events last many days, resulting in continuous exposure to concentrations above the standards, with impacts to human health. In this air pollution long-term study, a method was developed to identify persistent exceedance events (PEE) of particulate matter (PM10) and ozone (O3) and associated surface weather patterns. Between 2005 and 2017, 119 PEE were identified, with exceedances occurring simultaneously in at least 50% of monitoring stations along 3 to 14 consecutive days. Median PM10 and O3 concentrations increased by 60% during the events. Mean fields of sea level pressure from global reanalysis data revealed the influence of high-pressure systems and pre-frontal conditions. PM10 events were frequent in austral winter and mostly driven by anomalous atmospheric circulation with a wind change to northwest. On the other hand, O3 events were common in the spring, associated with higher positive anomalies of temperature and solar radiation. Overall, results show that PEE span a regional scale, differing from ordinary exceedance events that can be driven by local conditions. Policy makers should be aware of the frequency of PEE in the development of mitigation measures against the exposure to harmful levels of air pollutants. The concept of PEE can be applied to other metropolitan areas and may support the development of data-driven air quality predictive models based on current or forecasted weather conditions.
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The research was based on air quality public data provided by CETESB (https://qualar.cetesb.sp.gov.br/), meteorological data provided by IAG/USP meteorological station (https://www.iag.usp.br/) and ERA-Interim reanalysis data (https://www.ecmwf.int/). The dataset about persistent exceedance events developed in this research is provided in a worksheet as a supplementary material.
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References
Abe K, Miraglia S (2016) Health impact assessment of air pollution in São Paulo, Brazil. Int J Environ Res Public Health 13(7):694. https://doi.org/10.3390/ijerph13070694
Alvares CA et al (2013) Köppen’s climate classification map for Brazil. Meteorol Z 22(6):711–728. https://doi.org/10.1127/0941-2948/2013/0507
Brito J et al (2018) Disentangling vehicular emission impact on urban air pollution using ethanol as a tracer. Sci Rep 8(1):10679. https://doi.org/10.1038/s41598-018-29138-7
Carvalho VSB et al (2015) Air quality status and trends over the metropolitan area of São Paulo, Brazil as a result of emission control policies. Environ Sci Policy 47:68–79. https://doi.org/10.1016/j.envsci.2014.11.001
CETESB (2019) Qualidade do ar no Estado de São Paulo em 2018. São Paulo. Available at: https://cetesb.sp.gov.br/ar/publicacoes-relatorios/.
Chen ZH et al (2008) Relationship between atmospheric pollution processes and synoptic pressure patterns in northern China. Atmos Environ 42:6078–6087. https://doi.org/10.1016/j.atmosenv.2008.03.043
Chiquetto JB et al (2019) Air quality standards and extreme ozone events in the São Paulo megacity. Sustainability (switzerland) 11(13):1–14. https://doi.org/10.3390/su11133725
Coelho CAS, Cardoso DHF, Firpo MAF (2016) Precipitation diagnostics of an exceptionally dry event in São Paulo, Brazil. Theoret Appl Climatol 125(3–4):769–784. https://doi.org/10.1007/s00704-015-1540-9
Cohen AJ et al (2017) Estimates and 25-year trends of the global burden of disease attributable to ambient air pollution: an analysis of data from the Global Burden of Diseases Study 2015. The Lancet 6736(17):1–12. https://doi.org/10.1016/S0140-6736(17)30505-6
de Araujo JM, do Rosário NMÉ (2020) Poluição atmosférica associada ao material particulado no Estado de São Paulo: análise baseada em dados de satélite. Revista Brasileira De Ciências Ambientais (online) 55(1):32–47. https://doi.org/10.5327/z2176-947820200552
de Andrade MF et al (2017) Air quality in the megacity of São Paulo: evolution over the last 30 years and future perspectives. Atmos Environ 159:66–82. https://doi.org/10.1016/j.atmosenv.2017.03.051
Foss M, Chou SC, Seluchi ME (2017) Interaction of cold fronts with the Brazilian plateau: a climatological analysis. Int J Climatol 37(9):3644–3659. https://doi.org/10.1002/joc.4945
Gozzo LF et al (2021) Padrões climatológicos associados a eventos de seca no Leste do Estado de São Paulo. Revista Brasileira De Climatologia 28:321–341. https://doi.org/10.5380/abclima.v28i0.76268
Hersbach H et al (2020) The ERA5 global reanalysis. Q J R Meteorol Soc 146(730):1999–2049. https://doi.org/10.1002/qj.3803
IAG-USP (2017) Boletim Climatológico anual da Estação Meteorológica do IAG/USP. São Paulo. Available at: http://www.estacao.iag.usp.br/Boletins/2017.pdf.
Kukkonen J et al (2005) ‘Analysis and evaluation of selected local-scale PM10 air pollution episodes in four European Cities: Helsinki, London Milan and Oslo analysis and evaluation of selected local-scale PM 10 air pollution episodes in four European cities: Helsinki, London. Atmos Environ. https://doi.org/10.1016/j.atmosenv.2004.09.090
Kumar P et al (2016) New directions: from biofuels to wood stoves: the modern and ancient air quality challenges in the megacity of São Paulo. Atmos Environ 140:364–369. https://doi.org/10.1016/j.atmosenv.2016.05.059
Lencioni S (2015) Região Metropolitana de São Paulo como centro da inovação do Brasil. Cadernos Metrópole 17(34):317–328. https://doi.org/10.1590/2236-9996.2015-3401
Liu C et al (2019) Ambient particulate air pollution and daily mortality in 652 cities. N Engl J Med 381(8):705–715. https://doi.org/10.1056/NEJMoa1817364
Molina MJ, Molina LT (2004) Megacities and atmospheric pollution. J Air Waste Manag Assoc 54(6):644–680. https://doi.org/10.1080/10473289.2004.10470936
Oliveira MCQD, Rizzo LV, Drumond A (2020) Characterization of air-quality degradation episodes of PM10 in the metropolitan area of São Paulo and their relationship with meteorological conditions. Environ Sci Proceed 4(1):8. https://doi.org/10.3390/ecas2020-08143
Pampuch LA et al (2016) Anomalous patterns of SST and moisture sources in the South Atlantic Ocean associated with dry events in southeastern Brazil. Int J Climatol 36(15):4913–4928. https://doi.org/10.1002/joc.4679
Reboita MS et al (2019) The south atlantic subtropical anticyclone: present and future climate. Front Earth Sci 7:1–15. https://doi.org/10.3389/feart.2019.00008
Ribeiro FND et al (2018) Effect of sea breeze propagation on the urban boundary layer of the metropolitan region of Sao Paulo, Brazil. Atmos Res 214(July):174–188. https://doi.org/10.1016/j.atmosres.2018.07.015
Salvo A, Geiger FM (2014) Reduction in local ozone levels in urban São Paulo due to a shift from ethanol to gasoline use. Nat Geosci 7(6):450–458. https://doi.org/10.1038/NGEO2144
Salvo A et al (2017) Reduced ultrafine particle levels in São Paulo’s atmosphere during shifts from gasoline to ethanol use. Nat Commun 8(1):77. https://doi.org/10.1038/s41467-017-00041-5
Sánchez MP et al (2020) Rawinsonde-based analysis of the urban boundary layer in the metropolitan region of São Paulo, Brazil. Earth Space Sci. https://doi.org/10.1029/2019EA000781
Sánchez-Ccoyllo OR, Andrade MF (2002) The influence of meteorological conditions on the behavior of pollutants concentrations in São Paulo, Brazil. Environ Pollut 116(2):257–263
Santos TC, Reboita MS, Carvalho VSB (2018) Investigation of the relationship between atmospheric variables and the concentration of MP 10 and O 3 in the state of São Paulo. Revista Brasileira De Meteorologia 33(4):631–645. https://doi.org/10.1590/0102-7786334006
Schuch D et al (2019) A two decades study on ozone variability and trend over the main urban areas of the São Paulo state, Brazil. Environ Sci Pollut Res 26(31):31699–31716. https://doi.org/10.1007/s11356-019-06200-z
Silva Dias MAF et al (2013) Changes in extreme daily rainfall for São Paulo, Brazil. Clim Change 116(3–4):705–722. https://doi.org/10.1007/s10584-012-0504-7
Sugahara S et al (2012) Homogeneity assessment of a station climate series (1933–2005) in the Metropolitan Area of São Paulo: instruments change and urbanization effects. Theoret Appl Climatol 107(3–4):361–374. https://doi.org/10.1007/s00704-011-0485-x
Takano APC et al (2019) Pleural anthracosis as an indicator of lifetime exposure to urban air pollution: an autopsy-based study in Sao Paulo. Environ Res 173(March):23–32. https://doi.org/10.1016/j.envres.2019.03.006
Targino AC et al (2019) Surface ozone climatology of South Eastern Brazil and the impact of biomass burning events. J Environ Manage 252(May):1–12. https://doi.org/10.1016/j.jenvman.2019.109645
Whiteman CD et al (2014) Relationship between particulate air pollution and meteorological variables in Utah ’s Salt Lake Valley. Atmos Environ 94:742–753
WHO (2005) Air quality guidelines for particulate matter, ozone, nitrogen dioxide and sulfur dioxide, Global update 2005, Summary of risk assessment.
Zhao SX et al (2017) Megacities, the world’s largest cities unleashed: major trends and dynamics in contemporary global urban development. World Dev 98:257–289. https://doi.org/10.1016/j.worlddev.2017.04.038
Acknowledgements
We thank Companhia Ambiental do Estado de São Paulo (CETESB) and the University of Sao Paulo (IAG/USP) meteorological station for providing data on pollutant concentrations and surface weather variables.
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All authors contributed to the study conception and design. Material preparation, data collection and analysis were performed by Oliveira. The first draft of the manuscript was written by Oliveira and all authors commented on previous versions of the manuscript. Supervision and project administration were in charge of Rizzo and Drumond. All authors read and approved the final manuscript.
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Editorial responsibility: Samareh Mirkia.
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Oliveira, M.C.Q.D., Drumond, A. & Rizzo, L.V. Air pollution persistent exceedance events in the Brazilian metropolis of Sao Paulo and associated surface weather patterns. Int. J. Environ. Sci. Technol. 19, 9495–9506 (2022). https://doi.org/10.1007/s13762-021-03778-1
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DOI: https://doi.org/10.1007/s13762-021-03778-1