Abstract
Emission inventories are a fundamental input for atmospheric chemical transport models in order to accurately simulate air pollution and its impacts. In Australia, emission inventories are currently not available for electricity generators at high temporal and spatial resolutions. In this study, a new high spatial and temporal resolution inventory for Australian power plant emissions has been developed. The emissions from coal- and gas-fired power plants have been estimated using 5-min electricity generation time-series data and emission factors. The emissions are estimated from 2010 to 2019 for sulfur dioxide (\(\hbox {SO}_2\)), nitrogen oxide (\(\hbox {NO}_{2}\)), particulate matter (PM) and mercury (Hg). We estimate that, for 2019, the coal-fired power plants in Australia emitted significant amounts of \(\hbox {SO}_2\) (485.7 kTonne) and \(\hbox {NO}_{2}\) (452 kTonne), as there are no sulfur dioxide or nitrogen oxide controls in place. In contrast, PM emissions are mitigated by particulate matter control devices and coal-fired power plants emit an estimated 27.48 and 13.46 kTonne of \(\hbox {PM}_{10}\) and \(\hbox {PM}_{2.5}\), respectively. Coal-fired power plants were responsible for an estimated 3.13 tonnes of Hg emissions. Gas-fired plant emissions are significantly lower than coal-fired power emissions for all pollutants. Temporal analysis showed that coal- and gas-fired power plant emissions vary quite markedly during the day and over the week. There is a strong diurnal cycle in the gas-fired emissions, which, if ignored by assuming constant emissions (such as is routinely done), will lead to significant errors in modeled air pollution.
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Data availability statement
The datasets generated during the current study are available in the PANGEA repository, https://www.pangaea.de/tok/97ba6fe716625d601585573684b3fef15a83afec
References
AEC (2016) Retirement of coal fired power stations. https://www.aph.gov.au/Parliamentary_Business/Committees/Senate/Environment_and_Communications/Coal_fired_power_stations/Final_Report, Accessed on 10 Aug 2019. Published by the Australian Energy Council, Submission 44, November 2016. ISBN 978-1-76010-542-6
AEMO (2018) National Electricity Market Fact Sheet. Published by Australian Energy Market Operator, Australia. https://www.aemo.com.au/-/media/Files/Electricity/NEM/National-Electricity-Market-Fact-Sheet.pdf. Accessed on 2 Feb 2019
Beelen R, Raaschou-Nielsen O, Stafoggia M, Andersen ZJ, Weinmayr G, Hoffmann B, Wolf K, Samoli E, Fischer P, Nieuwenhuijsen M, Vineis P, Xun WW, Katsouyanni K, Dimakopoulou K, Oudin A, Forsberg B, Modig L, Havulinna AS, Lanki T, Turunen A, Oftedal B, Nystad W, Nafstad P, De Faire U, Pedersen NL, Östenson CG, Fratiglioni L, Penell J, Korek M, Pershagen G, Eriksen KT, Overvad K, Ellermann T, Eeftens M, Peeters PH, Meliefste K, Wang M, Bueno-De-Mesquita B, Sugiri D, Krämer U, Heinrich J, De Hoogh K, Key T, Peters A, Hampel R, Concin H, Nagel G, Ineichen A, Schaffner E, Probst-Hensch N, Künzli N, Schindler C, Schikowski T, Adam M, Phuleria H, Vilier A, Clavel-Chapelon F, Declercq C, Grioni S, Krogh V, Tsai MY, Ricceri F, Sacerdote C, Galassi C, Migliore E, Ranzi A, Cesaroni G, Badaloni C, Forastiere F, Tamayo I, Amiano P, Dorronsoro M, Katsoulis M, Trichopoulou A, Brunekreef B, Hoek G (2014) Effects of long-term exposure to air pollution on natural-cause mortality: an analysis of 22 European cohorts within the multicentre ESCAPE project. Lancet 383(9919):785–795. https://doi.org/10.1016/S0140-6736(13)62158-3
Broome RA, Fann N, Cristina TJ, Fulcher C, Duc H, Morgan GG (2015) The health benefits of reducing air pollution in Sydney, Australia. Environ Res 143:19–25. https://doi.org/10.1016/j.envres.2015.09.007
Cardu M, Baica M (1999) Regarding a global methodology to estimate the energy-ecologic efficiency of thermopower plants. Energy Convers Manag 40(1):71–87
Cohen DD, Crawford J, Stelcer E, Atanacio AJ (2012) Application of positive matrix factorization, multi-linear engine and back trajectory techniques to the quantification of coal-fired power station pollution in metropolitan Sydney. Atmos Environ 61:204–211. https://doi.org/10.1016/j.atmosenv.2012.07.037
Crawford J, Cohen DD, Stelcer E, Atanacio AJ (2017) Long term fine aerosols at the Cape Grim global baseline station: 1998–2016. Atmos Environ 166:34–46. https://doi.org/10.1016/J.ATMOSENV.2017.07.012
Crippa M, Guizzardi D, Muntean M, Schaaf E, Dentener F, van Aardenne JA, Monni S, Doering U, Olivier JGJ, Pagliari V, Janssens-Maenhout G (2018) Gridded emissions of air pollutants for the period 1970–2012 within EDGAR v4. 3.2. Earth Syst Sci Data Discuss. https://doi.org/10.5194/essd-2018-31
DECC (2019) Air Emissions Inventory for the Greater Metropolitan Region in New South Wales. Published by DECC (NSW Department of Environment and Climate Change), October 2019. https://www.environment.nsw.gov.au/. Accessed on 14 Mar 2019
DSEWPC (2012) NPI emission estimation technique manual for fossil fuel electric power generation, report version 3.0, National Pollutant Inventory (NPI). Published by Department of Sustainability, Environment, Water, Population and Communities (DSEWPC), Canberra, ACT, Australia. https://www.npi.gov.au/resource/emission-estimation-technique-manual-fossil-fuel-electric-power-generation. Accessed on 10 Oct 2018
Durie RA (1992) Structure. Properties and consequences for utilization. Elsevier Science and Technology, Oxford
EAAP (2019) Energy adequacy assessment projection report 2019. Published by AEMO, Australia. https://www.aph.gov.au/Parliamentary_Business/Committees/Senate/Environment_and_Communications/Coal_fired_power_stations/Final_Report0. Accessed on 2 Sept 2020
EPA NSW (2012) Air emissions inventory for the greater metropolitan region in New South Wales, 2008 calendar year. Published by ANSW Environment Protection Authority (NSW EPA) Technical Report 7, August. https://www.aph.gov.au/Parliamentary_Business/Committees/Senate/Environment_and_Communications/Coal_fired_power_stations/Final_Report1. Accessed on 2 July 2019
Ewald B (2018) The value of health damage due to sulphur dioxide emissions from coal- fired electricity generation in NSW and implications for pollution licences. Aust N Z J Public Health. https://www.aph.gov.au/Parliamentary_Business/Committees/Senate/Environment_and_Communications/Coal_fired_power_stations/Final_Report2
Forster P, Ramaswamy V, Artaxo P, Berntsen T, Betts R, Fahey DW, Haywood J, Lean J, Lowe DC, Myhre G, Nganga J, Prinn R, Raga G, Schulz M, Van Dorland R (2007) Changes in atmospheric constituents and in radiative forcing. Cambridge University Press, Cambridge (Chapter 2)
Huleatt MB (1991) Handbook of Australian black coals: geology, resources, seam properties, and product specifications
Jansohn P (2013) Modern gas turbine systems: high efficiency, low emission, fuel flexible power generation. Elsevier, Amsterdam
Janssens-Maenhout G, Crippa M, Guizzardi D, Dentener F, Muntean M, Pouliot G, Keating T, Zhang Q, Kurokawa J, Wankmüller R, Denier van der Gon H, Kuenen JJP, Klimont Z, Frost G, Darras S, Koffi B, Li M (2015) HTAP\_v2.2: a mosaic of regional and global emission grid maps for 2008 and 2010 to study hemispheric transport of air pollution. Atmos Chem Phys 15(19):11411–11432. https://www.aph.gov.au/Parliamentary_Business/Committees/Senate/Environment_and_Communications/Coal_fired_power_stations/Final_Report3
Jerrett M, Burnett RT, Pope CA, Ito K, Thurston G, Krewski D, Shi Y, Calle E, Thun M (2009) Long-term ozone exposure and mortality. N Engl J Med 360(11):1085–1095. https://www.aph.gov.au/Parliamentary_Business/Committees/Senate/Environment_and_Communications/Coal_fired_power_stations/Final_Report4
Lamarque JF, Bond TC, Eyring V, Granier C, Heil A, Klimont Z, Lee D, Liousse C, Mieville A, Owen B (2010) Historical (1850–2000) gridded anthropogenic and biomass burning emissions of reactive gases and aerosols: methodology and application. Atmos Chem Phys 10(15):7017–7039
Lelieveld J, Evans JS, Fnais M, Giannadaki D, Pozzer A (2015) The contribution of outdoor air pollution sources to premature mortality on a global scale. Nature 525(7569):367–371. https://www.aph.gov.au/Parliamentary_Business/Committees/Senate/Environment_and_Communications/Coal_fired_power_stations/Final_Report5
Liu F, Zhang Q, Tong D, Zheng B, Li M, Huo H, He K (2015) High-resolution inventory of technologies, activities, and emissions of coal-fired power plants in China from 1990 to 2010. Atmos Chem Phys 15(23):13299–13317
Matthias V, Arndt JA, Aulinger A, Bieser J, Denier van der Gon H, Kranenburg R, Kuenen J, Neumann D, Pouliot G, Quante M (2018) Modeling emissions for three-dimensional atmospheric chemistry transport models. J Air Waste Manag Assoc 68(8):763–800
Meij R (1994) Trace element behavior in coal-fired power plants. Fuel Process Technol 39(1–3):199–217
Miller JA, Bowman CT (1989) Mechanism and modeling of nitrogen chemistry in combustion. Prog Energy Combust Sci 15(4):287–338
Muzio L, Quartucy G (1997) Implementing \(no_{{\rm x}}\) control: research to application. Prog Energy Combust Sci 23(3):233–266
Myhre G, Shindell D, Bréon FM, Collins W, Fuglestvedt J, Huang J, Koch D, Lamarque JF, Lee D, Mendoza B, Nakajima T, Robock A, Stephens G, Takemura T, Zhang H (2013) Anthropogenic and natural radiative forcing. Climate change 2013: the physical science basis contribution of working group I to the Fifth assessment report of the intergovernmental panel on climate change, pp 659–740. https://doi.org/10.1017/CBO9781107415324.018
Nelson PF (2007) Atmospheric emissions of mercury from Australian point sources. Atmos Environ 41(8):1717–1724. https://www.aph.gov.au/Parliamentary_Business/Committees/Senate/Environment_and_Communications/Coal_fired_power_stations/Final_Report6
Nelson PF, Morrison AL, Malfroy HJ, Cope M, Lee S, Hibberd ML, Meyer CM, McGregor J (2012) Atmospheric mercury emissions in Australia from anthropogenic, natural and recycled sources. Atmos Environ 62:291–302
Pavlish JH, Sondreal EA, Mann MD, Olson ES, Galbreath KC, Laudal DL, Benson SA (2003) Status review of mercury control options for coal-fired power plants. Fuel Process Technol 82(2–3):89–165
Pavri R, Moore GD (2001) Gas turbine emissions and control. GE Energy Services, Atlanta
Perry G, Allardice D, Kiss L (1984) The chemical characteristics of Victorian brown coal. ACS Symp Ser Oxford Univ Press 264:3–14
Sengupta S, Datta A, Duttagupta S (2007) Exergy analysis of a coal-based 210 Victorian thermal power plant. Int J Energy Res 31(1):14–28
Srivastava RK, Hall RE, Khan S, Culligan K, Lani BW (2005) Nitrogen oxides emission control options for coal-fired electric utility boilers. J Air Waste Manag Assoc 55(9):1367–1388
Strezov V, Cho HH (2020) Environmental impact assessment from direct emissions of Australian thermal power generation technologies. J Clean Prod 270(122):515
Tang M, Mudd GM (2015) The pollution intensity of Australian power stations: a case study of the value of the national pollutant inventory (npi). Environ Sci Pollut Res 22(23):18410–18424
USEPA (1995) Compilation of air emission factors, AP-42, 5th edn, Volume 1: stationary point and area sources. https://www.epa.gov/air-emissions-factors-and-quantification/ap-42-compilation-air-emissions-factors. Accessed on 22 Aug 2020
USEPA (1998) Section 1.1, Bituminous and Subbituminous coal combustion. In: Compilation of air pollutant emission factors, Volume 1: stationary point and area sources, 5th edn, AP-42, Supplement E.https://www.epa.gov/sites/production/files/2020-09/documents/1.1_bituminous_and_subbituminous_coal_combustion.pdf Accessed on 22 Aug 2020
Vedrenne M, Borge R, Lumbreras J, Rodríguez ME, de la Paz D, Pérez J, de Andrés JM, Quaassdorff C (2016) A comprehensive approach for the evaluation and comparison of emission inventories in Madrid. Atmos Environ 145:29–44
Von Schneidemesser E, Monks PS, Allan JD, Bruhwiler L, Forster P, Fowler D, Lauer A, Morgan WT, Paasonen P, Righi M (2015) Chemistry and the linkages between air quality and climate change. Chem Rev 115(10):3856–3897
Wang X, Liang XZ, Jiang W, Tao Z, Wang JXL, Liu H, Han Z, Liu S, Zhang Y, Grell GA, Peckham SE (2010) WRF-Chem simulation of East Asian air quality: sensitivity to temporal and vertical emissions distributions. Atmos Environ 44(5):660–669. https://www.aph.gov.au/Parliamentary_Business/Committees/Senate/Environment_and_Communications/Coal_fired_power_stations/Final_Report7
Wendt J (1980) Fundamental coal combustion mechanisms and pollutant formation in furnaces. Prog Energy Combust Sci 6(2):201–222
World Bank Organisation (2020) Urban population (% of total population) - Australia. Published by World Bank Organisation. https://www.aph.gov.au/Parliamentary_Business/Committees/Senate/Environment_and_Communications/Coal_fired_power_stations/Final_Report8. Accessed on 22 Aug 2020
Xu W, Zeng Z, Xu Z, Li X, Chen X, Li X, Xiao R, Liang J, Chen G, Lin A et al (2020) Public health benefits of optimizing urban industrial land layout-the case of Changsha, china. Environ Pollut 263(114):388
Zhao Y, Wang S, Nielsen CP, Li X, Hao J (2010) Establishment of a database of emission factors for atmospheric pollutants from Chinese coal-fired power plants. Atmos Environ 44(12):1515–1523. https://www.aph.gov.au/Parliamentary_Business/Committees/Senate/Environment_and_Communications/Coal_fired_power_stations/Final_Report9
Acknowledgements
RS and MG acknowledge support from the Australian Research Council (ARC) Centre of Excellence for Climate Extremes (CE170100023) and the Australian Research Council’s Discovery Project: Tackling Atmospheric Chemistry Grand Challenges in the Southern Hemisphere (DP160101598). This research was undertaken with the assistance of resources and services from the National Computational Infrastructure (NCI) - under project q90, which is supported by the Australian Government.
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MG is supported by the Australian Government Research Training Program Scholarship.
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MG conceptualized and planned the study, performed the data analysis, and prepared the original draft of the manuscript. JS conceptualized and planned the study supervised the study, and reviewed and edited the manuscript. RS conceptualized and planned the study, supervised the study, acquired funding, and reviewed the manuscript. RR reviewed and edited the manuscript. All authors have read and approved the final manuscript.
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Garg, M., Silver, J.D., Schofield, R. et al. Hourly emission inventories for air toxic emissions for eastern Australian electricity generators derived from energy distribution data. Int. J. Environ. Sci. Technol. 19, 2973–2992 (2022). https://doi.org/10.1007/s13762-021-03429-5
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DOI: https://doi.org/10.1007/s13762-021-03429-5