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Insights of Corrosion Inhibitor Based in Pyridinium Ionic Liquids

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Abstract

Steel surfaces treated with synthesized ionic liquid (ILs) namedly 4-methyl-1-(3-phenoxypropyl) pyridinium bromide (Pyr1), 4-(dimethylamino)-1-(2-phenoxyethyl) pyridinium bromide (Pyr2) and4-(dimethylamino)-1-(3-phenoxypropyl) pyridinium bromide (Pyr3) were investigated in HCl acid media (1 M) using several techniques. Surfaces were analyzed by SEM and FESEM microscopy and by XPS spectroscopy, while the inhibition process was studied by electrochemical impedance (EIS) measurements. The results obtained by EIS demonstrated a higher charge transfer resistance that led to a high inhibition performance. According to Langmuir isotherm model and the activation parameters, these ILs can be adsorbed onto the mild steel surface through physical and chemical bonds. This study was supported by DFT and Monte Carlo calculations approach which confirms the adsorption behavior of the studied ILs.

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Acknowledgements

We also thank Engineering Laboratory of Organometallic, Molecular Materials, and Environment, Faculty of Sciences Dhar El Mahraz, Sidi Mohamed Ben Abdellah University for supporting this project. Thanks also to any structure that contributed to the realization of this work thanks to their feedback and testimonies. The present work has been supported by the Spanish Ministerio de Economía, Industria y Competividad (RTI2018-099668-BC22).

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Authors and Affiliations

  1. Engineering Laboratory of Electrochemistry, Modeling and Environment, Faculty of Sciences, University Sidi Mohamed Ben Abdellah, Fez, Morocco

    Fadoua El-Hajjaji & Mustapha Taleb

  2. King Abdulaziz City for Science and Technology, P.O. Box 6086, 11442, Riyadh, Saudi Arabia

    Rajae Salim & Saud M. Almutairi

  3. Chemistry Department, Faculty of Science, Taibah University, 30002, Al-Madinah Al-Mounawwara, Saudi Arabia

    Mouslim Messali

  4. X-Ray Photoelectron Spectroscopy Lab. Central Service to Support Research Building (SCAI), University of Málaga, 29071, Málaga, Spain

    M. Valle Martínez de Yuso

  5. Department of Inorganic Chemistry, Faculty of Science, University of Málaga, 29071, Málaga, Spain

    Enrique Rodríguez-Castellón

  6. Department of Chemistry, An-Najah National University, P. O. Box 7, Nablus, Palestine

    Shehdeh Jodeh

  7. Department of Sciences, INAMAT2-Institute for Advanced Materials and Mathematics, Public University of Navarre, Campus de Arrosadia, 31006, Pamplona, Spain

    Manuel Algarra

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  1. Fadoua El-Hajjaji
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El-Hajjaji, F., Salim, R., Messali, M. et al. Insights of Corrosion Inhibitor Based in Pyridinium Ionic Liquids. Arab J Sci Eng 48, 7755–7770 (2023). https://doi.org/10.1007/s13369-022-07502-0

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