Abstract
A two-step method is employed in this study to retrieve vertical ozone profiles using scattered measurements from the limb of the atmosphere. The combination of the Differential Optical Absorption Spectroscopy (DOAS) and the Multiplicative Algebraic Reconstruction Technique (MART) is proposed. First, the limb radiance, measured over a range of tangent heights, is processed using the DOAS technique to recover the effective column densities of atmospheric ozone. Second, these effective column densities along the lines of sight (LOSs) are inverted using the MART coupled with a forward model SCIATRAN (radiative transfer model for SCIAMACHY) to derive the ozone profiles. This method is applied to Optical Spectrograph and Infra Red Imager System (OSIRIS) radiance, using the wavelength windows 571–617 nm. Vertical ozone profiles between 10 and 48 km are derived with a vertical resolution of 1 km. The results illustrate a good agreement with the cloud-free coincident SCanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY) ozone measurements, with deviations less than ±10% (±5% for altitudes from 17 to 47 km). Furthermore, sensitivities of retrieved ozone to aerosol, cloud parameters and NO2 concentration are also investigated.
Similar content being viewed by others
References
Bourassa, A. E., 2007: Stratospheric aerosol retrieval from OSIRIS limb scattered sunlight spectra. Ph.D Thesis, Department of Physics and Engineering Physis, Univeristy of Saskatchewan, Saskatoon, 175 pp.
Brinksma, E. J., A. Bracher, D. E. Lolkema, et al., 2006: Geophysical validation of SCIAMACHY Limb Ozone Profiles. Atmos. Chem. Phys., 6(1), 197–209.
Chen Hongbin, 2009: An overview of the space-based observations for upper atomospheric research. Adv. Earth Sci., 24(3), 229–241. (in Chinese)
Chu, W. P., and M. P. McCormick, 1989: SAGE II inversion algorithm. J. Geophys. Res., 94(D6), 8339–8351.
Degenstein, D. A., A. E. Bourassa, C. Z. Roth, et al., 2008: Limb scatter ozone retrieval from 10 to 60 km using a multiplicative algebraic reconstruction technique. Atmos. Chem. Phys. Discuss, 8, 11853–11877.
—, E. J. Llewellyn, and N. D. Lloyd, 2003: Volume emission rate tomography from a statellite platform. Appl. Opt., 42(8), 1441–1450.
—, —, and —, 2004.: Tomographic retrieval of the oxygen infrared atmospheric band with the OSIRIS infrared imager. Can. J. Phys., 82, 501–515.
Eichmann, K. -U., J. W. Kaiser, C. v. Savigny, et al., 2004: SCIAMACHY limb measurements in the UV/Vis spectral region: first results. Adv. Space Res., 34, 775–779.
Evans, W. F. J., and E. J. Llewellyn, 1972: Measurements of mesospheric ozone from observations of the 1.27 µ band. Radio Sci., 7(1), 45–50.
Flittner, D. E., P. K. Bhartia, and B. M. Herman, 2000: O3 profiles retrieved from limb scatter measurements: Theory. Geophys. Res. Lett., 27(17), 2601–2604.
Gottwald, M., H. Bovensmann, G. Lichtenberg, et al., 2006: SCIAMACHY, Monitoring the Changing Earth’s Atmosphere. DLR, Institut fur Methodik der Fernerkundung, Freiburger.
Haley, C. S., S. M. Brohede, and C. E. Sioris, 2004: Retrieval of stratospheric O3 and NO2 profiles from Odin Optical Spectrograph and Infrared Imager System (OSIRIS) limb-scattered sunlight measurements. J. Geophys. Res., 109(D16303), 1–19.
Heue, K. P., A. Richter, M. Brun, et al., 2005: Validation of SCIAMACHY tropospheric NO2-columns with AMAXDOAS measurements. Atmos. Chem. Phys., 5, 1039–1051.
Kaiser, J. W., 2001: Atmospheric parameter retrieval from UV-vis-NIR limb scattering measurements. PhD thesis, Instiute of Environmental Physics / Institute of Remote Sensing, University of Bremen, Bremen, 10 pp.
Khabibrakhmanov, I. K., D. A. Degenstein, and E. J. Llewenllyn, 2002: Mesospheric ozone determination from orbit with the OSIRIS instrument on Odin. Can. J. Phys, 80, 493–504.
McPeters, R. D., S. J. Janz, E. Hilsenrath, et al., 2000: The retrieval of O3 profiles from limb scatter measurements: Results from the shuttle ozone limb sounding experiment. Geophys. Res. Lett., 27, 2597–2600.
Piters, A. J. M., K. Bramstedt, J.-C. Lambert, et al., 2006: Overview of SCIAMACHY validataion: 2002–2004. Atmos. Chem. Phys., 6, 127–148.
Qi Jin, 2007: Retrieval of nitrogen dioxide total column over China from SCIAMACHY/ENVISAT data. M.S Thesis, Chinese Academy of Meteorological Sciences, Beijing, 73 pp. (in Chinese)
Roth, C. Z., D. A. Degenstein, A. E. Bourassa, et al., 2007: The retrieval of vertical profiles of the ozone number density using Chappuis band absorption information and a multiplicative algebraic reconstruction technique. Can. J. Phys., 85, 1225–1243.
Rozanov, A., V. Rozanov, M. Buchwitz, et al., 2005: SCIATRAN 2.0-A new radiative transfer model for geophysical applications in the 175–2400 nm spectral region. Adv. Space Res., 36, 1015–1019.
Rusch, D. W., G. H. Mount, C. A. Barth, et al., 1984: Solar measospheric explorer ulttraviolet spectrometer: Measurements of ozone in the 1.0–0.1 mbar region. J. Geophys. Res., 89(D7), 11677–11687.
Strong, K., B. M. Joseph, R. Dosanjh, et al., 2002: Retrieval of vertical concentration profiles from OSIRIS UV-Visible limb spectra. Can. J. Phys., 80, 409–434.
Thomas, R. J., C. A. Barth, D. W. Rusch, et al., 1984: Solar mesosphere explorer near-Infrared spectrometer: measurements of 1.27-µm radiances and the inference of mesospheric ozone. J. Geophys. Res., 89(D6), 9569–9580.
Thomason, L. W., J. R. Moore, M. C. Pitts, et al., 2010: An evaluation of the SAGE III version 4 aerosol extinction coefficient and water vapor data products. Atmos. Chem. Phys., 10(6), 2159–2173.
von Savigny, C., C. S. Haley, C. E. Sioris, et al., 2003: Stratospheric ozone profiles retrieved from limb scattered sunlight radiance spectra measured by the OSIRIS instrument on the Odin satellite. Geophys. Res. Lett., 30(14), 1755–1758.
Wang Zijun, 2008: Simulation on atmospheric volume emission from limb scattering. M. S Thesis, College of Geoexploration Science and Technology, Jilin University, Changchun, 76 pp. (in Chinese)
Weitkamp, C., R. Baumgart, A. Behrendt, et al., 2001: Lidar ozone measurements in the marine and terrestrial atmosphere from the ground to the tropopause. Geoscience and Remote Sensing Symposium, IGARSS’ 01. IEEE 2001 International, 3, 1023–1025.
Author information
Authors and Affiliations
Corresponding author
Additional information
Supported by the National High Tech Research and Development (863) Program of China (2006AA12Z102) and Graduate Innovation Fund of Jilin University (20091023).
Rights and permissions
About this article
Cite this article
Wang, Z., Chen, S., Yang, C. et al. A method for retrieving vertical ozone profiles from limb scattered measurements. Acta Meteorol Sin 25, 659–668 (2011). https://doi.org/10.1007/s13351-011-0509-6
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s13351-011-0509-6