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Corrosion Mechanism of Three-Dimensional Network Configuration SiC–Fe Composites in Deep Mine Environment

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Abstract

With the development and depletion of shallow coal resources, deep coal mining has gradually become normalized. In the face of increasingly severe corrosion environment of coal mining, it is urgent to develop new materials with excellent corrosion resistance for key parts of coal mining equipment. In this paper, SiC, Al2O3 and SiO2 were used as raw materials to prepare three-dimensional network configuration SiC ceramics by organic foam impregnation method. Then the three-dimensional network configuration SiC-Fe composite was prepared by atmospheric pressure casting process. And by electrochemical test, static immersion corrosion test, scanning electron microscope and first-principles simulation calculation, the corrosion resistance of three-dimensional network configuration SiC-Fe composite in harsh mine water environment was characterized, meanwhile the corrosion resistance mechanism was analyzed. The results show that the corrosion potential increases from - 495.756 mV to -379.626 mV, and the corrosion current density decreases from 3.6864 μA/cm2 to 2.1709 μA/cm2 when the SiC ceramic reinforcement is added. The inhibition efficiency based on polarization curve measurement is increased by 41.11%. The charge transfer resistance increases from 5417 Ω·cm2 to 6437 Ω·cm2, and the capacitance value drops from 159.96 μF·cm−2 to 90.12 μF·cm−2. The inhibition efficiency based on electrochemical impedance spectroscopy is increased by 18.83%. First principles calculations show that the addition of SiC reinforcement showed a greater resistance in preventing the migration of corrosive media to the surface of the Fe substrate and can effectively slow down corrosion, which was consistent with the experimental results.

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Acknowledgements

This work was supported by The Tribology Science Fund of State Key Laboratory of Tribology (No. SKLTKF20B11), and supported by National Training Program of Innovation and Entrepreneurship for Undergraduates (No.202304058).

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Authors and Affiliations

  1. School of Mechanical and Electrical Engineering, China University of Mining and Technology (Beijing), Beijing, China

    Lei Fan, Fatao Wang, Yirui Bai, Xingshuai Fan, Neng Yang & Denglin Ran

  2. Coal Industry Engineering Research Center of Top-Coal Caving Mining, China University of Mining and Technology (Beijing), Beijing, China

    Lei Fan & Fatao Wang

  3. Zhengzhou Coal Mining Machinery Group Co Ltd, Zhengzhou, China

    Lei Fan, Neng Yang & Denglin Ran

  4. State Key Laboratory of Tribology in Advanced Equipment, Tsinghua University, Beijing, China

    Lei Fan

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  1. Lei Fan
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Fan, L., Wang, F., Bai, Y. et al. Corrosion Mechanism of Three-Dimensional Network Configuration SiC–Fe Composites in Deep Mine Environment. Trans Indian Inst Met (2024). https://doi.org/10.1007/s12666-023-03251-2

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