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Assessment of an arid region soil capacity on natural attenuation of municipal treated wastewater: a column experiment using soil of Varamin area, Iran

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Abstract

Soil aquifer treatment (SAT) is an effective indirect technique for wastewater reuse. The present study aims at assessing the soil capacity in arid region of Varamin on natural attenuation of inorganic constituents of municipal treated wastewater of Tehran City. In order to simulate SAT pond, four columns of 30 cm in height and 4 cm in diameter were filled with sandy loam soil taken from artificial recharge pond in Varamin plain. These columns were recharged by secondary treated wastewater from Shahre-Rey treatment plant under the plan of 12-h wetting and drying cycles. During the experiment, 50 pore volume passed through each column. The pH, EC, TDS, SAL, SAR, major ions, nitrate, phosphate and trace elements were measured in influent and effluent samples. The concentration of Na+, Ca2+, Mg2+, Cl and SO42− increased in effluent samples due to a washout process and dissolution of minerals. The soil could only attenuate NO3, K+, Rb and PO43− with the percentage of 18.4, 24.6, 67.7 and 83.6, respectively. The soil of studied area is rich in Cr, Ni, Sr, Pb, Cu, Zn, Ba and Rb. The concentrations of all mentioned trace elements, with the exception of Rb, have increased in the effluent samples with respect to influent. Also, the quality indices of TDS, SAL and SAR have increased 10.6, 25.2 and 8.7%, respectively, in effluent. Soil column samples, at the end of experiment, contain high amounts of major and trace elements. Consequently, there is a potential risk for groundwater contamination in long-term recharge.

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References

  • Abel CDT, Sharma SK, Malolo YN et al (2012) Attenuation of bulk organic matter, nutrients (N and P), and pathogen indicators during soil passage: effect of temperature and redox conditions in simulated soil aquifer treatment (SAT). Water Air Soil Pollut 223:5205–5220

    Article  Google Scholar 

  • Appelo CAJ, Postma D (2004) Geochemistry, groundwater and pollution. CRC Press, Boca Raton

    Google Scholar 

  • Azaroual M, Pettenati M, Ollivier P et al (2013) Reactive transfer of pollutants through the unsaturated soil zone during an artificial aquifer recharge process. Proc Earth Planet Sci 7:40–43

    Article  Google Scholar 

  • Becerra-Castro C, Lopes AR, Vaz-Moreira I et al (2015) Wastewater reuse in irrigation: a microbiological perspective on implications in soil fertility and human and environmental health. Environ Int 75:117–135. https://doi.org/10.1016/j.envint.2014.11.001

    Article  Google Scholar 

  • Bekele E, Toze S, Patterson B, Higginson S (2011) Managed aquifer recharge of treated wastewater: water quality changes resulting from infiltration through the vadose zone. Water Res 45:5764–5772

    Article  Google Scholar 

  • Bennett EM, Carpenter SR, Caraco NF (2001) Human impact on erodable phosphorus and eutrophication: a global perspective: increasing accumulation of phosphorus in soil threatens rivers, lakes, and coastal oceans with eutrophication. Bioscience 51:227–234

    Article  Google Scholar 

  • Bouwer H, Pyne RDG, Goodrich JA (1990) Recharging ground water. Civ Eng 60:63

    Google Scholar 

  • Brissaud F (2003) Groundwater recharge with recycled municipal wastewater: criteria for health related guidelines. State of the art report health risks in aquifer recharge using reclaimed water Water, Sanitation and Health Protection and the Human Environment World Health Organization Geneva and WHO Regional Office for Europe Copenhagen, Denmark, vol 2, pp 10–15

  • Bürger DA, Piquetc M, Moreno BF et al (2010) Impact of soil organic carbon content on soil filtering capacity solutes. In: Proceedings of the 19th world congress of soil science: soil solutions for a changing world, Brisbane, Australia, 1–6 August 2010. Symposium 3.2. 2 Improved water and soil management using lysimeters. International Union of Soil Sciences (IUSS), c/o Institut für Bodenforschung, Universität für Bodenkultur, pp 36–39

  • Close M (2010) Critical review of contaminant transport time through the Vadose Zone. Environment Canterbury

  • Conley DJ, Paerl HW, Howarth RW et al (2009) Controlling eutrophication: nitrogen and phosphorus. Science 323:1014–1015

    Article  Google Scholar 

  • Crook J, Surampalli RY (1996) Water reclamation and reuse criteria in the US. Water Sci Technol 33:451–462

    Google Scholar 

  • de Vries GE, Lopez A (2013) Wastewaters are not wastes. In: Living with water. Springer, New York, pp 101–141

  • Drewes JE, Heberer T, Rauch T, Reddersen K (2003) Fate of pharmaceuticals during ground water recharge. Groundw Monit Remediat 23:64–72

    Article  Google Scholar 

  • Dutta T, Carles-Brangarí A, Fernàndez-Garcia D et al (2015) Vadose zone oxygen (O2) dynamics during drying and wetting cycles: an artificial recharge laboratory experiment. J Hydrol 527:151–159

    Article  Google Scholar 

  • Flores AN, Sola FM, Navarro Flores A, Martínez Sola F (2010) Evaluation of metal attenuation from mine tailings in SE Spain (Sierra Almagrera): a soil-leaching column study. Mine Water Environ 29:53–67. https://doi.org/10.1007/s10230-010-0099-z

    Article  Google Scholar 

  • Fox P (2001) Soil aquifer treatment for sustainable water reuse. American Water Works Association, New York

    Google Scholar 

  • Gupta SC, Larson WE (1979) Estimating soil water retention characteristics from particle size distribution, organic matter percent, and bulk density. Water Resour Res 15:1633–1635

    Article  Google Scholar 

  • Han FX, Singer A (2007) Solution chemistry of trace elements in arid zone soils. In: Biogeochemistry of trace elements in arid environments. Springer Netherlands, pp 69–105

  • Hanson B, Grattan SR, Fulton A (1999) Agricultural salinity and drainage. University of California Irrigation Program, University of California Davis

  • Harman CJ, Rao PSC, Basu NB et al (2011) Climate, soil, and vegetation controls on the temporal variability of vadose zone transport. Water Resour Res 47(10):W00J13. https://doi.org/10.1029/2010WR010194

  • He Y, DeSutter T, Casey F et al (2015) Field capacity water as influenced by Na and EC: implications for subsurface drainage. Geoderma 245:83–88

    Article  Google Scholar 

  • Heberer T (2006) Occurrence, transport, attenuation and removal of pharmaceutical residues in the aquatic environment and their relevance to drinking water supply in urban areas, in recharge systems for protecting and enhancing groundwater resources. In: Proceedings of the 5th international symposium on management of aquifer recharge, pp 529–534

  • Hentati O, Chaker S, Wali A et al (2014) Effects of long-term irrigation with treated wastewater on soil quality, soil-borne pathogens, and living organisms: case study of the vicinity of El Hajeb (Tunisia). Environ Monit Assess 186:2671–2683

    Article  Google Scholar 

  • Holman IP, Whelan MJ, Howden NJK et al (2008) Phosphorus in groundwater—an overlooked contributor to eutrophication? Hydrol Process 22:5121–5127

    Article  Google Scholar 

  • Huber DP (2011) Re-evaluating effects of water quality changes on soil hydraulic properties, Doctoral dissertation, Colorado State University

  • IMOE I (2010) Environmental criteria of treated waste water and return flow reuse. Iranian Ministry of Energy (IMOE), No, 535

  • Izbicki JA, Flint AL, O’Leary DR et al (2015) Storage and mobilization of natural and septic nitrate in thick unsaturated zones, California. J Hydrol 524:147–165

    Article  Google Scholar 

  • Jarvis NJ (2007) A review of non-equilibrium water flow and solute transport in soil macropores: principles, controlling factors and consequences for water quality. Eur J Soil Sci 58:523–546

    Article  Google Scholar 

  • Johnson JS, Baker LA, Fox P (1999) Geochemical transformations during artificial groundwater recharge: soil–water interactions of inorganic constituents. Water Res 33:196–206

    Article  Google Scholar 

  • Kaboosi K (2016) The assessment of treated wastewater quality and the effects of mid-term irrigation on soil physical and chemical properties (case study: Bandargaz-treated wastewater). Appl Water Sci 7(5):2385–2396

    Article  Google Scholar 

  • Kalavrouziotis IK, Koukoulakis PH (2012) Soil pollution under the effect of treated municipal wastewater. Environ Monit Assess 184:6297–6305

    Article  Google Scholar 

  • Kodešová R, Vignozzi N, Rohošková M et al (2009) Impact of varying soil structure on transport processes in different diagnostic horizons of three soil types. J Contam Hydrol 104:107–125

    Article  Google Scholar 

  • Kowalkowski T, Tutu H, Cozmuta LM et al (2010) Assessment of mobility of heavy metals in two soil types by use of column leaching experiments and chemometric evaluation of elution curves. Int J Environ Anal Chem 90:797–811

    Article  Google Scholar 

  • Lazarova V, Cirelli G, Jeffrey P et al (2000) Enhancement of integrated water management and water reuse in Europe and the Middle East. Water Sci Technol 42:193–202

    Google Scholar 

  • Lennartz B, Haria AH, Johnson AC (2007) Flow regime effects on reactive and non-reactive solute transport. Soil Sediment Contam 17:29–40

    Article  Google Scholar 

  • Lin C, Shacahr Y, Banin A (2004) Heavy metal retention and partitioning in a large-scale soil-aquifer treatment (SAT) system used for wastewater reclamation. Chemosphere 57:1047–1058

    Article  Google Scholar 

  • Lin C, Negev I, Eshel G, Banin A (2008) In situ accumulation of copper, chromium, nickel, and zinc in soils used for long-term waste water reclamation. J Environ Qual 37:1477–1487

    Article  Google Scholar 

  • Mahmoudi N, Nakhaei M, Porhemmat J (2017) Assessment of hydrogeochemistry and contamination of Varamin deep aquifer, Tehran Province, Iran. Environ Earth Sci 76:370

    Article  Google Scholar 

  • Mansell J, Drewes JE (2004) Fate of steroidal hormones during soil aquifer treatment. Groundw Monit Remediat 24:94–101

    Article  Google Scholar 

  • Miller GW (2006) Integrated concepts in water reuse: managing global water needs. Desalination 187:65–75

    Article  Google Scholar 

  • Montgomery-Brown J, Drewes JE, Fox P, Reinhard M (2003) Behavior of alkylphenol polyethoxylate metabolites during soil aquifer treatment. Water Res 37:3672–3681

    Article  Google Scholar 

  • Mulligan CN, Yong RN (2004) Natural attenuation of contaminated soils. Environ Int 30:587–601

    Article  Google Scholar 

  • Nahra JA (2006) Modeling phosphorus transport in soil and water, Doctoral dissertation, Ph. D. thesis, Department of Bioresource Engineering, McGill University, Montreal, QC

  • Pais I, Jones JB Jr (1997) The handbook of trace elements. CRC Press, Boca Raton

    Google Scholar 

  • Parkhurst DL, Appelo CAJ (1999) User’s guide to PHREEQC (version 2): a computer program for speciation, batch-reaction, one-dimensional transport, and inverse geochemical calculations. ceres.udc.es

  • Pierzynski GM, Vance GF, Sims JT (2005) Soils and environmental quality. CRC Press, Boca Raton

    Google Scholar 

  • Quanrud DM, Carroll SM, Gerba CP, Arnold RG (2003a) Virus removal during simulated soil-aquifer treatment. Water Res 37:753–762

    Article  Google Scholar 

  • Quanrud DM, Hafer J, Karpiscak MM et al (2003b) Fate of organics during soil-aquifer treatment: sustainability of removals in the field. Water Res 37:3401–3411

    Article  Google Scholar 

  • Rao SM, Gaurave K, Sarvanan A (2013) Lead retention by soils at field moisture contents. Soil Sediment Contam Int J 22:208–222

    Article  Google Scholar 

  • Sánchez-Martin MJ, Lorenzo LF, Sanchez-Camazano M (2001) Leaching of Cd, Zn, Pb, and Cu in packed and undisturbed columns of soils affected by the spill from a pyrite mine in the south of Spain. Soil Sediment Contam 10:359–373

    Article  Google Scholar 

  • Schäfer A, Ustohal P, Harms H et al (1998) Transport of bacteria in unsaturated porous media. J Contam Hydrol 33:149–169

    Article  Google Scholar 

  • Smičiklas I, Jović M, Šljivić-Ivanović M et al (2015) Correlation of Sr 2+ retention and distribution with properties of different soil types. Geoderma 253:21–29

    Article  Google Scholar 

  • Soriano-Disla JM, Gómez I, Navarro-Pedreño J (2011) The influence of soil properties on the mobility of metals following a single application of polluted sewage sludge to seventy agricultural topsoils: a laboratory column study. Soil Sediment Contam Int J 20:961–976

    Article  Google Scholar 

  • Sposito G (2008) The chemistry of soils. Oxford University Press, Oxford

    Google Scholar 

  • Tabatabaei SH, Najafi P (2009) Effects of irrigation with treated municipal wastewater on soil properties in arid and semi-arid regions. Irrig Drain 58:551–560

    Article  Google Scholar 

  • Todd DK, Mays LW (2005) Groundwater hydrology, 3rd edn. Wiley, Hoboken

    Google Scholar 

  • Toze S, Hanna J, Smith T et al (2004) Determination of water quality improvements due to the artificial recharge of treated effluent. IAHS Publ Ser Proc Rep 285:53–60

    Google Scholar 

  • Usepa U (2004) Guidelines for water reuse. EPA/625/R–04/108. USEPA and US Agency for International Development, Washington, DC

  • Vanderzalm JL, Page DW, Barry KE, Dillon PJ (2010) A comparison of the geochemical response to different managed aquifer recharge operations for injection of urban stormwater in a carbonate aquifer. Appl Geochem 25:1350–1360

    Article  Google Scholar 

  • Vohla C, Alas R, Nurk K et al (2007) Dynamics of phosphorus, nitrogen and carbon removal in a horizontal subsurface flow constructed wetland. Sci Total Environ 380:66–74

    Article  Google Scholar 

  • Xue S, Zhao Q-L, Wei L-L, Ren N-Q (2009) Behavior and characteristics of dissolved organic matter during column studies of soil aquifer treatment. Water Res 43:499–507

    Article  Google Scholar 

  • Zhang J, Lo IMC (2008) Centrifuge study of long term transport behavior and fate of copper in soils at various saturation of water, compaction and clay content. Soil Sediment Contam 17:237–255

    Article  Google Scholar 

  • Zhang J, Huang X, Liu C et al (2005) Nitrogen removal enhanced by intermittent operation in a subsurface wastewater infiltration system. Ecol Eng 25:419–428

    Article  Google Scholar 

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Acknowledgements

The authors would like to thank the Kharazmi University for the financial support which helped to carry out this research work.

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Correspondence to Nina Mahmoudi.

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Mahmoudi, N., Nakhaei, M. & Porhemmat, J. Assessment of an arid region soil capacity on natural attenuation of municipal treated wastewater: a column experiment using soil of Varamin area, Iran. Environ Earth Sci 77, 140 (2018). https://doi.org/10.1007/s12665-018-7292-y

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