Abstract
Measurement of radium (226Ra) and thorium (232Th) content, and exhalation rate of radon (222Rn) and thoron (220Rn) from soil and building materials are important in the context of modeling indoor radon and thoron concentration. In this study, exhalation rates of radon and thoron from commonly used building materials in India were measured using active measurement techniques. Also the activity concentrations of 226Ra, 232Th and potassium (40K) in building materials were measured by HPGe gamma spectrometric technique. The activity concentration of 226Ra, 232Th and 40K varied from 16.4 ± 4.4 to 114.7 ± 3.4, 13.3 ± 1.5 to 153.9 ± 16.6 and below detection limit to 1,007 ± 40 Bq/kg with arithmetic mean 40.3, 61.9 and 822 Bq/kg, respectively, for the examined building material samples. The radon exhalation rates from the building materials varied from 0.5 ± 0.01 to 62.9 ± 12.5 mBq/kg/h for powder samples, 73 ± 5 to 6,000 ± 310 mBq/m2/h for structural building materials while the thoron exhalation rates varied from 0.07 ± 0.27 to 15.03 ± 2.1 mBq/kg/h for samples in powder form. Radium equivalent activity calculated for coarse aggregate and brick powder samples ranged between 73 and 343 Bq/kg.
Similar content being viewed by others
References
Bavarnegin E, Fathabadi N, Moghaddam MV, Farahani MV, Moradi M, Babakhni A (2013) Radon exhalation rate and natural radionuclide content in building materials of high background areas of Ramsar, Iran. J Environ Radioact 117:36–40
Cevik U, Kara A, Celik N, Karabidak M, Celik A (2011) Radon survey and exposure assessment in Karaca and Çal Caves, Turkey. Water Air Soil Pollut 214:461–469
Chen J, Rahman NM, Atiya IA (2010) Radon exhalation from building materials for decorative use. J Environ Radioact 101:317–322
Csige I, Szabó Z, Szabo C (2013) Experimental technique to measure thoron generation rate of building material samples using RAD7 detector. Radiat measurements 59:201–204
Faheem M, Mujahid SA, Matiullah (2008) Assessment of radiological hazards due to the natural radioactivity in soil and building material samples collected from six districts of the Punjab province-Pakistan. Radiat Measurements 43:1443–1447
Gaware JJ, Sahoo BK, Sapra BK, Mayya YS (2011) Indigenous development and networking of online radon monitors in the underground uranium mine. Radiat Protect Environ 34:37–40
Gupta M, Chauhan RP (2011) Estimating radiation dose from building materials, Iran. J Radiat Res 9:187–194
Gupta M, Chauhan RP, Sonkawade RG, Kant K (2010) Contribution of TENORM towards indoor radioactivity. ISST J Appl Phys 1:75–79
Hassan NM, Ishikawa T, Hosoda M, Iwaoka K, Sorimachi A, Sahoo SK, Janik M, Kranrod C, Yonehara H, Fukushi M, Tokonami S (2011) The effect of water content on the radon emanation coefficient for some building materials used in Japan. Radiat Measurements 46:232–237
IAEA (1989) Regional workshop on environmental sampling and measurements of radioactivity for monitoring purpose, Kalpakkam, India, vol 9., pp 85–92
Kanse SD, Sahoo BK, Sapra BK, Gaware JJ, Mayya YS (2013) Powder sandwich technique: a novel method for determining the thoron emanation potential of powders bearing high 224Ra content. Radiat Measurements 48:82–87
Khan HM, Ismail M, Khan K, Akhter P (2011) Measurement of radionuclides and gamma-ray dose rate in soil and transfer of radionuclides from soil to vegetation, vegetable of some northern area of Pakistan using γ-ray spectrometry. Water Air Soil Pollut 219:129–142
Kovler K (2011) Legislative aspects of radiation hazards from both gamma emitters and radon exhalation of concrete containing coal fly ash. Constr Build Mater 25:3404–3409
Krishnamoorthy N, Mullainathan S, Mehra R, Chaparro MAE, Chaparro MAE (2014) Radiation impact assessment of naturally occurring radionuclides and magnetic mineral studies of Bharathapuzha river sediments, South India. Environ Earth Sci 71:3593–3604
Krisiuk EM, Tarasov SI, Shamov VP, Shlak NI, Lisachenko EP, Gomslsky LG (1971) A study of radioactivity in building materials. Research Institute of Radiation Hygeine, Leningrad
Kumar A, Chauhan RP (2013) Active and passive measurements of radon diffusion coefficient from building construction materials. Environ Earth Sci 72:251–257
Kumar A, Chauhan RP, Joshi M, Sahoo BK (2014) Modeling of indoor radon concentration from radon exhalation rates of building materials and validation through measurements. J Environ Radioact 127:50–55
Maged AF, Ashraf FA (2005) Radon exhalation rate of some building materials used in Egypt. Environ Geochem Health 27:485–489
Nain M, Chauhan RP, Chakarvarti SK (2006) Alpha radioactivity in Indian cement samples. Iran J Radiat Res 3:171–176
Nazaroff WW, Nero AV Jr (1988) Radon and its decay products in indoor air. Wiley, New York
Ningappa (2009) Studies on natural background radiation levels in granite qurries around Banglore rural district. PhD Thesis University of Manglore, Mysore
OECD (1979) Nuclear Energy Agency. Exposure to radiation from natural radioactivity in building materials. Report by NEA Group of Experts, OECD, Paris
Petropoulos NP, Anagnostakis MJ, Simopoulos SE (2001) Building materials radon exhalation rate: ERRICCA intercomparison exercise results. Sci Total Environ 272:109–118
Sahoo BK, Nathwani D, Eappen KP, Ramachandran TV, Gaware JJ, Mayya YS (2007) Estimation of radon emanation factor in Indian building materials. Radiat Measurements 42:1422–1425
Sahoo BK, Sapra BK, Gaware JJ, Kanse SD, Mayya YS (2011) A model to predict radon exhalation from walls to indoor air based on the exhalation from building material samples. Sci Total Environ 409:2635–2641
Sakoda A, Hanamoto K, Ishimori Y, Nagamatsu T, Yamaoka K (2008) Radioactivity and radon emanation fraction of the granites sampled at Misasa and Badgastein. Appl Radiat Isot 66:648–652
Steiner V, Kovler K, Perevalov A, Kelm H (2005) Estimation of the radon dose in buildings by measuring the exhalation rate from building materials. Int Congress Ser 1276:397–398
Stoulos S, Manolopoulou M, Papastefanou C (2003) Assessment of natural radiation exposure and radon exhalation from building materials in Greece. J Environ Radioact 69:225–240
Stranden E (1976) Some aspects on radioactivity of building materials. Phys Norv 1976(8):167–173
Sumesh CG, Kumar AV, Tripathi RM, Nair RN, Puranik VD (2013) Impact of flow rate on sensitivity of semiconductor type thoron monitor. Radiat Measurement 59:241–244
Trevisi R, Nuccetelli Risica S (2013) Screening tools to limit the use of building materials with enhanced/elevated levels of natural radioactivity: analysis and application of index criteria. Constr Build Mater 49:448–454
Turhan S, Gunduz L (2008) Determination of specific activity of 226Ra, 232Th and 40K for assessment of radiation hazards from Turkish pumice samples. J Environ Radioact 99:332–342
Ujic P, Celikovic I, Kandic A, Zunic Z (2008) Standardization and difficulties of the thoron exhalation rate measurements using an accumulation chamber. Radiat Measurements 43:1396–1401
UNSCEAR (2000) United Nations Scientific Committee on the effects of atomic radiation. Sources and effects of ionizing radiation, vol I. United Nations, New York
Uyanik NA, Uyanik O, Gur F, Aydin I (2013) Natural radioactivity of bricks and brick material in the Salihli-Turgutlu area of Turkey. Environ Earth Sci 68:499–506
Acknowledgments
The authors are thankful to Board of Research in Nuclear Science, Department of Atomic Energy, Mumbai, India, for providing the financial support in form of project 2011/36/25-BRNS to carry out this work.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Kumar, A., Chauhan, R.P., Joshi, M. et al. Estimation of radionuclides content and radon–thoron exhalation from commonly used building materials in India. Environ Earth Sci 74, 1539–1546 (2015). https://doi.org/10.1007/s12665-015-4146-8
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s12665-015-4146-8