Abstract
Recently, we achieved atomic-resolution optical imaging with near-field scanning optical microscopy using photon-induced force detection. In this technique, the surface photovoltage of the silicon-tip apex induced by the optical near field on the surface is measured as the electrostatic force. We demonstrated atomicresolution imaging of the near field on the α-Al2O3 (0001) surface of a prism. We investigated the spatial distribution of the near field by scanning at different tip-sample distances and found that the atomic corrugation of the near-field signal was observed at greater distances than that of the atomic force microscopy signal. As the tip-sample distance increased, the normalized signal-to-noise ratio of the near field is in a gradual decline almost twice that of the frequency shift (Δf).
Similar content being viewed by others
References
Pohl, D. W.; Denk, W.; Lanz, M. Optical stethoscopy: Image recording with resolution λ/20. Appl. Phys. Lett. 1984, 44, 651–653.
Betzig, E.; Trautman, J. K.; Harris, T. D.; Weiner, J. S.; Kostelak, R. L. Breaking the diffraction barrier: Optical microscopy on a nanometric scale. Science 1991, 251, 1468–1470.
Fischer, U. Ch.; Pohl, D. W. Observation of single-particle plasmons by near-field optical microscopy. Phys. Rev. Lett. 1989, 62, 458–461.
Zenhausern, F.; Martin, Y.; Wickramasinghe, H. K. Scanning interferometric apertureless microscopy: Optical imaging at 10 angstrom resolution. Science 1995, 269, 1083–1085.
Hecht, B.; Bielefeldt, H.; Inouye, Y.; Pohl, D. W.; Novotny, L. Facts and artifacts in near-field optical microscopy. J. Appl. Phys. 1997, 81, 2492–2498.
Sánchez, E. J.; Novotny, L.; Xie, X. S. Near-field fluorescence microscopy based on two-photon excitation with metal tips. Phys. Rev. Lett. 1999, 82, 4014–4017.
Stöckle, R. M.; Suh, Y. D.; Deckert, V.; Zenobi, R. Nanoscale chemical analysis by tip-enhanced Raman spectroscopy. Chem. Phys. Lett. 2000, 318, 131–136.
Ichimura, T.; Hayazawa, N.; Hashimoto, M.; Inoue, Y.; Kawata, S. Tip-enhanced coherent anti-stokes Raman scattering for vibrational nanoimaging. Phys. Rev. Lett. 2004, 92, 220801.
Zhang, R.; Zhang, Y.; Dong, Z. C.; Jiang, S.; Zhang, C.; Chen, L. G.; Zhang, L.; Liao, Y.; Aizpurua, J.; Luo, Y. et al. Chemical mapping of a single molecule by plasmonenhanced Raman scattering. Nature 2013, 498, 82–86.
Binnig, G.; Quate, C. F.; Gerber, Ch. Atomic force microscopy. Phys. Rev. Lett. 1986, 56, 930–933.
Giessibl, F. J. Atomic resolution of the silicon (111)-(7×7) surface by atomic force microscopy. Science 1995, 267, 68–71.
Mertz, J.; Hipp, M.; Mlynek, J.; Marti, O. Optical near-field imaging with a semiconductor probe tip. Appl. Phys. Lett. 1994, 64, 2338–2340.
Abe, M.; Sugawara, Y.; Sawada, K.; Andoh, Y.; Morita, S. Near-field optical imaging using force detection with new tip-electrode geometry. Appl. Surf. Sci. 1999, 140, 383–387.
Ma, Z. M.; Kou, L. L.; Naitoh, Y.; Li, Y. J.; Sugawara, Y. The stray capacitance effect in kelvin probe force microscopy using FM, AM and heterodyne A Mmodes. Nanotechnology 2013, 24, 225701.
Sugawara, Y.; Yamanishi, J.; Tokuyama, T.; Naitoh, Y.; Li, Y. J. Atomic-resolution imaging of the optical near field based on the surface photovoltage of a silicon probe tip. Phys. Rev. Appl. 2015, 3, 044020.
Sadewadder, S.; Jelinek, P.; Fang C.-K.; Custance, O.; Yamada, Y.; Sugimoto Y.; Abe, M.; Morita, S. New insights on atomic-resolution frequency-modulation kelvin-probe force-microscopy imaging of semiconductors. Phys. Rev. Lett. 2009, 103, 266103.
Sadeghi, A.; Baratoff, A.; Ghasemi, S. A.; Goedecker, S.; Glatzel, T.; Kawai, S.; Meyer, E. Multiscale approach for simulations of kelvin probe force microscopy with atomic resolution. Phys. Rev. B 2012, 86, 075407.
Giessibl, F. J. Forces and frequency shifts in atomicresolution dynamic-force microscopy. Phys. Rev. B 1997, 56, 16010–16015.
Albrecht, T. R.; Grütter, P.; Horne, D.; Rugar, D. Frequency modulation detection using high-Q cantilevers for enhanced force microscope sensitivity. J. Appl. Phys. 1991, 69, 668–673.
Vilfan, I.; Lanç on, F.; Villain, J. Rotational reconstruction of sapphire (0001). Surf. Sci. 1997, 392, 62–68.
Barth, C.; Reichling, M. Imaging the atomic arrangements on the high-temperature reconstructed a-Al2O3(0001) surface. Nature 2001, 414, 54–57.
Lauritsen, J. V.; Jensen, M. C. R.; Venkataramani, K.; Hinnemann, B.; Helveg, S.; Clausen, B. S.; Besenbacher, F. Atomic-scale structure and stability of the v31×v31 R° surface of Al2O3(0001). Phys. Rev. Lett. 2009, 103, 076103.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Yamanishi, J., Tokuyama, T., Naitoh, Y. et al. Distance dependence of atomic-resolution near-field imaging on α-Al2O3 (0001) surface with respect to surface photovoltage of silicon probe tip. Nano Res. 9, 530–536 (2016). https://doi.org/10.1007/s12274-015-0934-4
Received:
Revised:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s12274-015-0934-4