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Polydopamine Modified Rice Husk-derived Silicon Carbon Black Used as Green Filler in Natural Rubber/Butadiene Rubber: Design, Processing and Properties

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Abstract

The green filler PDA-SiCB was prepared by grafting polydopamine (PDA) to rice husk-derived silicon carbon black (SiCB). The effect of PDA-SiCB as a renewable filler on the properties of natural rubber/butadiene rubber (NR/BR) composites was studied in detail. The PDA coating formed on the surface of SiCB could not only improve the surface activity of the SiCB and promote the dispersion of the SiCB, but also effectively solved the problem of compatibility between the SiCB and the matrix, greatly improved the interface strength, thus effectively improving the properties of rubber composites. As a result, the tensile strength of NR/BR/PDA-SiCB composites prepared by mechanical blending with dopamine modified filler was greatly improved, reaching 23.1 MPa, which are 63 % and 106 % higher than that of NR/BR/SiCB composite and NR/BR rubber. And compared with NR/BR/SiCB, the elongation at break and glass transition temperature (Tg) of NR/BR/PDA-SiCB were increased by 30 % and 3.87 oC, respectively, and the thermal stability was also improved.

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Acknowledgment

This work was financially supported by the Project of Jilin Provincial Scientific and Technological Department (20190302055GX, 20190302037GX); the China Postdoctoral Science Foundation (2017M611321).

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Authors and Affiliations

  1. Key Laboratory of Automobile Materials, Ministry of Education, and College of Materials Science and Engineering, Jilin University, Changchun, 130025, China

    Jicai Liang, Leiming Sun, Kaifeng Yu, Wenming Jin & Ce Liang

  2. Roll Forging Research Institute, Jilin University, Changchun, 130025, Jilin, China

    Jicai Liang, Leiming Sun & Wenming Jin

  3. College of Chemistry, Jilin University, Changchun, 130012, Jilin, China

    Miaomiao Qian

Authors
  1. Jicai Liang
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  2. Leiming Sun
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  3. Kaifeng Yu
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  4. Miaomiao Qian
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  5. Wenming Jin
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  6. Ce Liang
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Correspondence to Wenming Jin or Ce Liang.

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Liang, J., Sun, L., Yu, K. et al. Polydopamine Modified Rice Husk-derived Silicon Carbon Black Used as Green Filler in Natural Rubber/Butadiene Rubber: Design, Processing and Properties. Fibers Polym 22, 3144–3152 (2021). https://doi.org/10.1007/s12221-021-1302-5

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  • DOI: https://doi.org/10.1007/s12221-021-1302-5

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