Abstract
The Einstein–Debye approximation was used with the help of Simpson’s 3/8th rule to develop a method for the temperature dependence of heat capacity at constant volume and constant pressure of actinide dioxide nuclear fuels. The Debye model approximates the acoustic modes of the lattice while the Einstein model approximates the optical modes. Based on Simpson’s 3/8th rule, a simple mathematical expression was used to calculate the isochoric and isobaric heat capacities of nuclear fuels for arbitrary temperature values. When compared to prior published studies of nuclear fuels, such as UO\({}_{2}\) and PuO\({}_{2}\), the dependability, efficiency and precision of the present method are satisfactory. The obtained results are consistent with the literature, demonstrating the validity of the method.
Similar content being viewed by others
References
J T White and A T Nelson, J. Nucl. Mater. 443, 342 (2013)
E Yakub, C Ronchi and D Staicu, J. Nucl. Mater. 400, 189 (2010)
Y Yun and P M Oppeneer, Mater. Res. Soc. (MRS) Bull. 36, 178 (2011)
V Khokhlov, I Korzun, V Dokutovich and E Filatov, J. Nucl. Mater. 410, 32 (2011)
K Morimoto, M Kato, M Ogasawara and M Kashimura, J. Nucl. Mater. 389, 179 (2009)
H Koç, E Eser and B A Mamedov, Nucl. Eng. Design 241, 3678 (2011)
J K Fink, J. Nucl. Mater. 279, 1 (2000)
H E Schmidt, C Sari, K Richter and P Gerontopoulos, J. Less Common Met. 121, 621 (1986)
M Katayama, J Adachi, K Kurosaki, M Uno, S Miwa, M Osaka, K Tanaka and S Yamanaka, Mater. Res. Soc. Symp. Proc. (Warrendale, PA, 2007) Vol. 1043E, 1043-T09-06.
T Nishi, A Itoh, M Takano, M Numata, M Akabori, Y Arai and K Minato, J. Nucl. Mater. 376, 78 (2008)
K Kurosaki, M Imamura, I Sato, T Namekawa, M Uno and S Yamanaka, J. Alloys Compd. 387, 9 (2005)
S Saygi, AIP Adv. 4, 027102 (2014)
C B Basak, A K Sengupta and H S Kamath, J. Alloys Compd. 360, 210 (2003)
J A Webb and I Charit, J. Nucl. Mater. 427, 87 (2012)
L Vlahovic, D Staicu, A Küst and R J M Konings, J. Nucl. Mater. 499, 504 (2018)
V Sobolev and S Lemehov, J. Nucl. Mater. 352, 300 (2006)
Yu N Devyatko, V V Novikov, V I Kuznetsov, O V Khomyakov and D A Chulkin, IOP Conf. Ser. Mater. Sci. Eng.130, 012061 (2016)
T Balcerzak, K Szałowski and M Jǎšcur, J. Phys. Condens. Matter 22, 425401 (2010)
D Belmonte, G Ottonello and M Vetuschi Zuccolini, J. Chem. Phys. 138, 064507 (2013)
M H G Jacobs, R Schmid-Fetzer and A P van den Berg, Phys. Chem. Miner. 20, 207 (2013)
B A Mamedov, Nucl. Eng. Design 276, 124 (2014)
C G S Pillai and P Raj, J. Nucl. Mater. 277, 116 (2000)
K Kurosaki, K Yamada, M Uno, S Yamanaka, K Yamamoto and T Namekawa, J. Nucl. Mater. 294, 160 (2001)
P Ruello, L Desgranges, G Baldinozzi, G Calvarin, T Hansen, G Petot-Ervas and C Petot, J. Phys. Chem. Solids 66, 823 (2006)
H Serizawa, Y Arai and Y Suzuki, J. Nucl. Mater. 280, 99 (2000)
S Li, R Ahuja and B Johansson, High Press. Res. 22, 471 (2002)
M Cankurtaran and V Askerov, Phys. Status Solidi B 194, 499 (1996)
T Arima, S Yamasaki, Y Inagaki and K Idemitsu, J. Alloys. Comd. 415, 43 (2006)
Y Yun, D Legut and P M Oppeneer, J. Nucl. Mater. 426, 109 (2012)
J P Hiernaut, G J Hyland and C Ronchi, Int. J. Thermophys. 14, 259 (1993)
E Eser, B Duyuran, M H Bölükdemir and H Koç, Nucl. Eng. Technol. 52, 1208 (2020)
J J Carbajo, G L Yoder, S G Popov and V K Ivanov, J. Nucl. Mater. 299, 181 (2001)
O L Kruger and H J Savage, J. Chem. Phys. 49, 4540 (1968)
M Chu, D Meng, S Xiao, W Wang and Q Chen, J. Alloys Compd. 539, 7 (2012)
N I Kolev, Multiphase flow dynamics, in: Nuclear thermal hydraulics (Springer-Verlag, Berlin, 2009)
Acknowledgements
IAA thanks CVR for constructing a computational program in the Python language.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Ansari, I.A., Rao, C.V. Analytical evaluation of isochoric and isobaric heat capacities for actinide dioxide nuclear fuels. Pramana - J Phys 97, 79 (2023). https://doi.org/10.1007/s12043-023-02557-6
Received:
Revised:
Accepted:
Published:
DOI: https://doi.org/10.1007/s12043-023-02557-6