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The effect of platinum decoration on the sensing characterisation of AlP nanosheets towards mercaptopurine drug

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Abstract

The density functional B3LYP was utilised for scrutinising the effect of Pt-decoration on the sensing performance of an AlP nanosheet (AlPNS) in detecting mercaptopurine (MP). Pure AlPNS has a weak interaction with MP, and the sensing response is \(\sim \) 2.4. There was an increase in the energy of adsorption (\(E_{\mathrm{ad}})\) for MP from \(-6.2\) to \(-24.1\) kcal/mol when the surface of AlPNS was decorated with a Pt atom. There was also a dramatic increase in the sensing response to 77.4. The recovery time (RT) for the desorption of MP from the AlPNS surface that was decorated with Pt at 298 K was 36.4 s. The solvent H\(_{2}\)O decreased \(E_{\mathrm{ad}}\) for MP to \(-19.9\) kcal/mol. These values suggest that AlPNS decorated with Pt can be used as an MP sensor because of its high sensitivity and shorter RT.

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Acknowledgements

Authors extend their appreciation to the Deanship of Scientific Research at King Khalid University for supporting this work through the research project programme under grant number R.G.P.2/107/42.

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Authors and Affiliations

  1. Spectroscopy Department, Physics Research Institute, National Research Centre, Dokki, Giza, 12622, Egypt

    A A Menazea

  2. Laser Technology Unit, National Research Centre, Dokki, Giza, 12622, Egypt

    A A Menazea

  3. Chemistry Department, Faculty of Science, King Khalid University, P.O. Box 9004, Abha, 61413, Saudi Arabia

    Nasser S Awwad

  4. Biology Department, Faculty of Science, King Khalid University, P.O. Box 9004, Abha 61413, Saudi Arabia

    Hala A Ibrahium

  5. Department of Semi Pilot Plant, Nuclear Materials Authority, P.O. Box 530, El Maadi, Egypt

    Hala A Ibrahium

  6. Physics Department, Faculty of Science, King Khalid University, P.O. Box 9004, Abha, 61413, Saudi Arabia

    H Elhosiny Ali

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  1. A A Menazea
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  2. Nasser S Awwad
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  3. Hala A Ibrahium
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Menazea, A.A., Awwad, N.S., Ibrahium, H.A. et al. The effect of platinum decoration on the sensing characterisation of AlP nanosheets towards mercaptopurine drug. Pramana - J Phys 96, 100 (2022). https://doi.org/10.1007/s12043-022-02334-x

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