Abstract
Technological advancement towards the quantum era requires secure communication, quantum computation and ultra-sensitive sensing capabilities. Layered quantum materials (LQMs) have remarkable optoelectronic and quantum properties that can usher us into the quantum era. Electron microscopy is the tool of choice for measuring these LQMs at an atomic and nanometre scale. On the other hand, electron-irradiation of LQMs can modify various material properties, including the creation of structural defects. We review different types of structural defects, as well as electron elastic- and inelastic-scattering induced processes. Controlled modification of optoelectronic and quantum properties of LQMs using electron-irradiation, including creation of single-photon emitters is discussed. Protection of electron-irradiation induced damage of LQMs via encapsulation by other layered materials is encouraged. We finally give insights into challenges and opportunities, including creating novel structures using an electron beam.
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References
Arute F, Arya K, Babbush R, Bacon D, Bardin J C, Barends R et al 2019 Nature 574 505
Gisin N and Thew R 2007 Nat. Photonics 1 165
Pirandola S, Bardhan B R, Gehring T, Weedbrook C and Lloyd S 2018 Nat. Photonics 12 724
Degen C L, Reinhard F and Cappellaro P 2017 Rev. Mod. Phys. 89 035002
Preskill J 2018 Quantum 2 79
Singh A, Tran K, Kolarczik M, Seifert J, Wang Y, Hao K et al 2016 Phys. Rev. Lett. 117 257402
O’Brien J L 2007 Science 318 1567
Liao W, Huang Y, Wang H and Zhang H 2019 Appl. Mater. Today 16 435
Chakraborty C, Vamivakas N and Englund D 2019 Nanophotonics 8 2017
Butler S Z, Hollen S M, Cao L, Cui Y, Gupta J A, Gutiérrez H R et al 2013 ACS Nano 7 2898
Wilson J A and Yoffe A D 1969 Adv. Phys. 18 193
Singh A, Jo S S, Li Y, Wu C, Li M and Jaramillo R 2020 ACS Photonics 7 3270
Liu Y, Weiss N O, Duan X, Cheng H-C, Huang Y and Duan X 2016 Nat. Rev. Mater. 1 1
Datta I, Chae S H, Bhatt G R, Tadayon M A, Li B, Yu Y et al 2020 Nat. Photonics 14 256
Zhu C R, Zhang K, Glazov M, Urbaszek B, Amand T, Ji Z W et al 2014 Phys. Rev. B 90 161302
Wang G, Bouet L, Lagarde D, Vidal M, Balocchi A, Amand T et al 2014 Phys. Rev. B 90 075413
Qiu H, Xu T, Wang Z, Ren W, Nan H, Ni Z et al 2013 Nat. Commun. 4 2642
van der Zande A M, Huang P Y, Chenet D A, Berkelbach T C, You Y, Lee G-H et al 2013 Nat. Mater. 12 554
Chen Y, Xi J, Dumcenco D O, Liu Z, Suenaga K, Wang D et al 2013 ACS Nano 7 4610
Singh A, Li Y, Fodor B, Makai L, Zhou J, Xu H et al 2019 Appl. Phys. Lett. 115 161902
Mleczko M J, Zhang C, Lee H R, Kuo H-H, Magyari-Köpe B, Moore R G et al 2017 Sci. Adv. 3 e1700481
Kalinin S V and Dyck O 2019 Adv. Funct. Mater. 29 1908267
Mahjouri-Samani M, Lin M-W, Wang K, Lupini A R, Lee J, Basile L et al 2015 Nat. Commun. 6 7749
Hu Z, Wu Z, Han C, He J, Ni Z and Chen W 2018 Chem. Soc. Rev. 47 3100
Chen J, Shao K, Yang W, Tang W, Zhou J, He Q et al 2019 ACS Appl. Mater. Interfaces 11 19381
Li H, Jia X, Zhang Q and Wang X 2018 Chem 4 1510
Nan H, Wang Z, Wang W, Liang Z, Lu Y, Chen Q et al 2014 ACS Nano 8 5738
Lin Z, Carvalho B R, Kahn E, Lv R, Rao R, Terrones H et al 2016 2D Mater. 3 022002
Zhang K, Feng S, Wang J, Azcatl A, Lu N, Addou R et al 2015 Nano Lett. 15 6586
Xia Y, Wei L, Deng J, Zong L, Wang C, Chen X et al 2020 Adv. Mater. Technol. 5 2000307
Eftekhari A 2017 J. Mater. Chem. A 5 18299
Wu Z and Ni Z 2017 Nanophotonics 6 1219
Ly T H, Chiu M-H, Li M-Y, Zhao J, Perello D J, Cichocka M O et al 2014 ACS Nano 8 11401
Lin J, Pantelides S T and Zhou W 2015 ACS Nano 9 5189
Zhou W, Zou X, Najmaei S, Liu Z, Shi Y, Kong J et al 2013 Nano Lett. 13 2615
Najmaei S, Liu Z, Zhou W, Zou X, Shi G, Lei S et al 2013 Nat. Mater. 12 754
Egerton R F, Li P and Malac M 2004 Micron 35 399
Komsa H-P, Kotakoski J, Kurasch S, Lehtinen O, Kaiser U and Krasheninnikov A V 2012 Phys. Rev. Lett. 109 035503
Liu K, Feng J, Kis A and Radenovic A 2014 ACS Nano 8 2504
Kretschmer S, Lehnert T, Kaiser U and Krasheninnikov A V 2020 Nano Lett. 20 2865
Ke J-A, Garaj S and Gradečak S 2019 ACS Appl. Mater. Interfaces 11 26228
Komsa H-P, Kurasch S, Lehtinen O, Kaiser U and Krasheninnikov A V 2013 Phys. Rev. B 88 035301
Lin Y-C, Dumcenco D O, Huang Y-S and Suenaga K 2014 Nat. Nanotechnol. 9 391
Egerton R F 2013 Ultramicroscopy 127 100
Hobbs L W 1987 Ultramicroscopy 23 339
Reimer L 1998 Scanning electron microscopy (Berlin, Heidelberg: Springer) p 529
Everhart T E and Hoff P H 1971 J. Appl. Phys. 42 5837
Skowron S T, Roberts S L, Khlobystov A N and Besley E 2019 Micron 120 96
Refaely-Abramson S, Qiu D Y, Louie S G and Neaton J B 2018 Phys. Rev. Lett. 121 167402
Parkin W M, Balan A, Liang L, Das P M, Lamparski M, Naylor C H et al 2016 ACS Nano 10 4134
Moody G, Tran K, Lu X, Autry T, Fraser J M, Mirin R P et al 2018 Phys. Rev. Lett. 121 057403
Choi S, Tran T T, Elbadawi C, Lobo C, Wang X, Juodkazis S et al 2016 ACS Appl. Mater. Interfaces 8 29642
Barthelmi K, Klein J, Hötger A, Sigl L, Sigger F, Mitterreiter E et al 2020 Appl. Phys. Lett. 117 070501
Qian Q, Peng L, Perea-Lopez N, Kazunori Fujisawa K, Zhang K, Zhang X et al 2020 Nanoscale 12 2047
Mignuzzi S, Pollard A J, Bonini N, Brennan B, Gilmore I S, Pimenta M A et al 2015 Phys. Rev. B 91 195411
Shi W, Lin M-L, Tan Q-H, Qiao X-F, Zhang J and Tan P-H 2016 2D Mater. 3 025016
Koperski M, Molas M R, Arora A, Nogajewski K, Slobodeniuk A O, Faugeras C et al 2017 Nanophotonics 6 1289
Ayari S, Smiri A, Hichri A, Jaziri S and Amand T 2018 Phys. Rev. B 98 205430
Moody G, Kavir Dass C, Hao K, Chen C-H, Li L-J, Singh A et al 2015 Nat. Commun. 6 8315
Koperski M, Nogajewski K, Arora A, Cherkez V, Mallet P, Veuillen J-Y et al 2015 Nat. Nanotechnol. 10 503
He Y-M, Clark G, Schaibley J R, He Y, Chen M-C, Wei Y-J et al 2015 Nat. Nanotechnol. 10 497
Chakraborty C, Goodfellow K M and Vamivakas A N 2016 Opt. Mater. Express 6 2081
Srivastava A, Sidler M, Allain A V, Lembke D S, Kis A and Imamoğlu A 2015 Nat. Nanotechnol. 10 491
Kimble H J, Dagenais M and Mandel L 1977 Phys. Rev. Lett. 39 691
Tran T T, Elbadawi C, Totonjian D, Lobo C J, Grosso G, Moon H et al 2016 ACS Nano 10 7331
Klein J, Lorke M, Florian M, Sigger F, Sigl L, Rey S et al 2019 Nat. Commun. 10 2755
Branny A, Kumar S, Proux R and Gerardot B D 2017 Nat. Commun. 8 15053
Palacios-Berraquero C, Kara D M, Montblanch A R-P, Barbone M, Latawiec P, Yoon D et al 2017 Nat. Commun. 8 15093
Parto K, Banerjee K and Moody G 2020 arXiv:2009.07315 [physics, physics:quant-ph]
Zhao X, Dan J, Chen J, Ding Z, Zhou W, Loh K P et al 2018 Adv. Mater. 30 1707281
Lin J, Zhang Y, Pantelides S T and Zhou W 2015 Microscopy Microanal. 21 433
Zhao X, Kotakoski J, Meyer J C, Sutter E, Sutter P, Krasheninnikov A V et al 2017 MRS Bull. 42 667
Ahn S, Kim G, Nayak P K, Yoon S I, Lim H, Shin H-J et al 2016 ACS Nano 10 8973
Kobayashi K and Yasuda H 2018 Mater. Res. Express 5 085006
Singh A, Lee H Y and Gradečak S 2020 Nano Res. 13 1363
Zan R, Ramasse Q M, Jalil R, Georgiou T, Bangert U and Novoselov K S 2013 ACS Nano 7 10167
Cho H, Jones M R, Nguyen S C, Hauwiller M R, Zettl A and Alivisatos A P 2017 Nano Lett. 17 414
Wang J I-J, Yang Y, Chen Y-A, Watanabe K, Taniguchi T, Churchill H O H et al 2015 Nano Lett. 15 1898
Lee G-H, Cui X, Kim Y D, Arefe G, Zhang X, Lee C-H et al 2015 ACS Nano 9 7019
Zheng S, So J-K, Liu F, Liu Z, Zheludev N and Fan H J 2017 Nano Lett. 17 6475
Kufer D and Konstantatos G 2015 Nano Lett. 15 7307
Tran K, Moody G, Wu F, Lu X, Choi J, Kim K, Rai A et al 2019 Nature 567 71
Kotakoski J, Jin C H, Lehtinen O, Suenaga K and Krasheninnikov A V 2010 Phys. Rev. B 82 113404
Caturla M J, Soneda N, Diaz de la Rubia T and Fluss M 2006 J. Nuclear Mater. 351 78
Deng J, Deng D and Bao X 2017 Adv. Mater. 29 1606967
Lin J, Cretu O, Zhou W, Suenaga K, Prasai D, Bolotin K I et al 2014 Nat. Nanotechnol. 9 436
Acknowledgements
AS would like to acknowledge funding from Indian Institute of Science start-up grant, and from SERB Start-up research grant SRG-2020-000133. KSK would like to acknowledge DST-INSPIRE fellowship. AKD would like acknowledge Prime Minister's Research Fellowship (PMRF).
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This article is part of the special issue on ‘Quantum materials and devices’.
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Dash, A.K., Mondal, M., Verma, M. et al. Effect of electron-irradiation on layered quantum materials. Bull Mater Sci 44, 227 (2021). https://doi.org/10.1007/s12034-021-02516-0
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DOI: https://doi.org/10.1007/s12034-021-02516-0